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Chiral phonons are desirable for applications in spintronics but their generation and control remains a challenge.Here we demonstrate the emergence of truly chiral phonons from selective magnon-phonon coupling in inversion-symmetric…

Circularly polarized phonons conventionally carry an angular momentum and a magnetic moment arising from circular motions of the atoms. Here, we present three anomalous cases that lead to phonon magnetic moments, which cannot be described…

Materials Science · Physics 2026-02-24 Swati Chaudhary , Carl P. Romao , Dominik M. Juraschek

We have developed a microscopic theory on phonon energy dispersion in chiral crystals within a harmonic approximation. One of the main issues is about the splitting of sound velocity of acoustic phonons with opposite ``crystal'' angular…

Strongly Correlated Electrons · Physics 2023-02-01 Hirokazu Tsunetsugu , Hiroaki Kusunose

Chiral phonons, quantized lattice vibrations with circular polarization and non-zero angular momentum, offer new perspectives for phononic and quantum device engineering. Graphyne could be a promising candidate due to its unique lattice…

Mesoscale and Nanoscale Physics · Physics 2025-08-18 Subhendu Mishra , Arpan Chakraborty , Douglas S. Galvao , Pedro A. S. Autreto , Abhishek Kumar Singh

Phonon angular momentum in chiral materials has been widely studied in spintronics and condensed matter physics. In chiral crystals, this is not the conserved quantity in contrast to the pseudo-angular momentum. To highlight this point and…

Materials Science · Physics 2023-06-30 Akihito Kato , Jun-ichiro Kishine

In this Letter, we predict a structural phase transition unique to chiral crystals with screw symmetry. In chiral crystals, the phonon frequency renormalized by the electron-phonon coupling depends on the handedness of circular…

Strongly Correlated Electrons · Physics 2026-04-21 Shun Asano , Youichi Yanase

Chiral phonons, circularly polarized lattice vibrations carrying intrinsic angular momentum, offer unprecedented opportunities for controlling heat flow, manipulating quantum states through spin-phonon coupling, and realizing exotic…

The second-order nonlinear optical coefficients associated with chirality differ in sign for the two mirror-image forms (enantiomers) of a chiral material. Structures comprised of alternating stacks of the enantiomers can therefore be used…

Chemical Physics · Physics 2019-05-16 Bertrand Busson , Martti Kauranen , Colin Nuckolls , Thomas Katz , André Persoons

Lattice vibrations carrying angular momentum, known as chiral phonons, have emerged as a promising route to control and understand complex material properties, yet their deterministic manipulation remains largely unexplored. Here we…

In nature, $\alpha$-quartz crystals frequently form contact twins - two adjacent crystals with the same chemical structure but different crystallographic orientation, sharing a common lattice plane. As $\alpha$-quartz crystallises in a…

Materials Science · Physics 2023-07-03 Juan D. F. Pottecher , Gunnar F. Lange , Cameron Robey , Bartomeu Monserrat , Bo Peng

The concept of chirality makes ubiquitous appearance in nature. Particularly, both a structure and its collective excitations may acquire well defined chiralities. In this work, we reveal an intrinsic connection between the chiralities of a…

Materials Science · Physics 2024-05-21 Hao Chen , Weikang Wu , Jiaojiao Zhu , Weikang Gong , Weibo Gao , Shengyuan A. Yang , Lifa Zhang

The Raman selection rules arise from the crystal symmetry and then determine the Raman activity and polarization of scattered phonon modes. However, these selection rules can be broken in resonant process due to the strong electron-phonon…

Materials Science · Physics 2021-02-09 Qing-Hai Tan , Kai-Xuan Xu , Yu-Jia Sun , Xue-Lu Liu , Yuan-Fei Gao , Shu-Liang Ren , Ping-Heng Tan , Jun Zhang

The concept of chirality is of great relevance in nature, from chiral molecules such as sugar to parity transformations in particle physics. In condensed matter physics, recent studies have demonstrated chiral fermions and their relevance…

Hyperbolic crystals like {\alpha}-MoO$_3$ can support large wavevectors and photon density as compared to the commonly used dielectric crystals, which makes them a highly desirable platform for compact photonic devices. The extreme…

Chiral properties have seen increasing use in recent years, leading to the emerging fields of chiral quantum optics, plasmonics, and phononics. While these fields have achieved manipulation of the chirality of light and lattice vibrations,…

Materials Science · Physics 2025-04-08 Carl P. Romao , Dominik M. Juraschek

In recent studies, it has been discovered that phonons can carry angular momentum, leading to a series of investigations into systems with 3-fold rotation symmetry. However, for systems with 2-fold screw rotational symmetry, such as…

Materials Science · Physics 2024-04-01 Meiqi Li , Zhibing Li , Huanjun Chen , Weiliang Wang

We have found that the polarization dependence of Raman scattering in organic crystals at finite temperatures can only be described by a fourth-rank formalism. This generalization of the second-rank Raman tensor $\mathcal{R}$ stems from the…

We theoretically introduce a scheme to perform Ramsey spectroscopy on a racemic mixture of chiral molecules, simultaneously extracting the transition frequencies of the left- and right-handed molecules, known as enantiomers. By taking the…

Atomic Physics · Physics 2023-11-07 Itay Erez , Eliana Ruth Wallach , Yuval Shagam

We predict high-order harmonics in which the polarization within the spectral bandwidth of each harmonic varies continuously and significantly. For example, the interaction of counter-rotating circularly-polarized bichromatic drivers having…

Optics · Physics 2014-10-24 Avner Fleischer , Ofer Kfir , Pavel Sidorenko , Oren Cohen

Chirality, the breaking of improper rotational symmetry, is a fundamental concept spanning diverse scientific domains. In condensed matter physics, chiral phonons, originating from circular atomic motions that carry angular momentum, have…