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We introduce an approach for performing spectrally resolved electron microscopy without the need for an electron spectrometer. The method involves an electron beam prepared as a coherent superposition of multiple paths, one of which passes…

Materials Science · Physics 2025-04-24 F. Javier García de Abajo , Cruz I. Velasco

In this paper we describe an ultrafast scanning electron microscope setup developed for the research of inelastic scattering of electrons at optical near-fields of periodic dielectric nanostructures. Electron emission from the Schottky…

Applied Physics · Physics 2018-08-01 M. Kozák , J. McNeur , N. Schönenberger , J. Illmer , A. Li , A. Tafel , P. Yousefi , T. Eckstein , P. Hommelhoff

We report on the development of an ultrafast Transmission Electron Microscope based on a laser-driven cold-field emission source. We first describe the instrument before reporting on numerical simulations of the laser-driven electron…

Optics · Physics 2019-11-27 G. M. Caruso , F. Houdellier , S. Weber , M. Kociak , A. Arbouet

Free electron beams such as those employed in electron microscopes have evolved into powerful tools to investigate photonic nanostructures with an unrivaled combination of spatial and spectral precision through the analysis of electron…

Quantum Physics · Physics 2021-04-22 F. Javier García de Abajo , Valerio Di Giulio

Electron-photon quantum entanglement in an electron microscope paves the way for a new quantum platform, enabling the integration of quantum functionalities into electron microscopy and opening opportunities for quantum imaging and quantum…

Quantum Physics · Physics 2026-05-25 Tatsuro Yuge , Ryo Okamoto , Takumi Sannomiya , Keiichirou Akiba

In this manuscript we present a theoretical framework and its numerical implementation to simulate the out-of-equilibrium electron dynamics induced by the interaction of ultrashort laser pulses in condensed-matter systems. Our approach is…

The ability to tailor laser light on a chip using integrated photonics has allowed for extensive control over fundamental light-matter interactions in manifold quantum systems including atoms, trapped ions, quantum dots, and defect centers.…

Electron microscopy based on high-energy electrons allows nanoscopic analytical imaging taking advantage of secondarily generated particles. Especially for cathodoluminescence, the correlation between primary incident electrons and emitted…

Instrumentation and Detectors · Physics 2025-01-28 Sotatsu Yanagimoto , Naoki Yamamoto , Tatsuro Yuge , Hikaru Saito , Keiichirou Akiba , Takumi Sannomiya

Entangled photon spectroscopy is a nascent field that has important implications for measurement and imaging across chemical, biology, and materials fields. Entangled photon spectroscopy potentially offers improved spatial and…

Optics · Physics 2021-07-07 Szilard Szoke , Manni He , Bryce P. Hickam , Scott K. Cushing

Ultrafast electron beams are essential for many applications, yet space-charge interactions in high-intensity beams lead to energy dissipation, coherence loss, and pulse broadening. Existing techniques mitigate these effects by using…

Optics · Physics 2025-07-02 Hao Geng , Qiaofei Pan , Jian Kang , Yiming Pan

Spontaneous processes triggered in a sample by free electrons are commonly regarded as incoherent, and therefore unable to interfere with external light sources. Here, we challenge this concept by showing through first-principles theory…

Efficient coupling between light and bulk plasmons (BPs) remains a central challenge because of their inherent mode mismatch, limited penetration depth, and pronounced resonant energy mismatch between visible-range photons and BPs. In this…

Coherent control of ultrafast quantum phenomena benefits from pulse-shaping capabilities allowing to modulate the envelope and instantaneous phase of optical fields on femtosecond time scales. While such control is available for optical…

Optics · Physics 2026-02-05 Nelin Laštovičková Streshkova , Martin Kozák

Nonlinear optical phenomena such as parametric amplification and frequency conversion are typically driven by external optical fields. Free electrons can also act as electromagnetic sources, offering unmatched spatial precision. Combining…

Mesoscale and Nanoscale Physics · Physics 2025-08-04 Leila Prelat , Eduardo J. C. Dias , F. Javier García de Abajo

In this paper we study photon emission in the interaction of the laser beam with an under-dense target and the attached reflecting plasma mirror. Photons are emitted due to the inverse Compton scattering when accelerated electrons interact…

Plasma Physics · Physics 2020-07-17 M. Jirka , O. Klimo , Y. J. Gu , S. Weber

Progress in electron-beam spectroscopies has recently enabled the study of optical excitations with combined space, energy and time resolution in the nanometer, millielectronvolt and femtosecond domain, thus providing unique access into…

Optics · Physics 2019-11-13 Albert Polman , Mathieu Kociak , F. Javier García de Abajo

The generation of quantum entanglement between phonons in photoirradiated remote electron-phonon systems is numerically studied. Upon excitation by a visible/ultraviolet laser pulse, the entanglement of electrons is immediately generated…

Mesoscale and Nanoscale Physics · Physics 2021-10-13 Kunio Ishida , Hiroaki Matsueda

We propose and theoretically demonstrate a technique that allows one to compensate for chromatic aberrations of traditional electron lenses in ultrafast electron microscopes. The technique is based on space- and time-dependent phase…

Advancing quantum information, communication and sensing relies on the generation and control of quantum correlations in complementary degrees of freedom. Here, we demonstrate the preparation of electron-photon pair states using the…

We report on the development of an ultrafast Transmission Electron Microscope based on a cold field emission source which can operate in either DC or ultrafast mode. Electron emission from a tungsten nanotip is triggered by femtosecond…

Instrumentation and Detectors · Physics 2017-11-15 Florent Houdellier , Giuseppe M. Caruso , Sébastien Weber , Mathieu Kociak , Arnaud Arbouet
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