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Frequency comb spectroscopy provides broadband access to molecular fingerprints with mode-defined spectral resolution. However, its deployment in non-cooperative gas sensing remains challenging because conventional implementations require…

Frequency comb spectroscopy has significantly advanced molecular spectroscopy across scientific research and diverse applications. Among its key performance metrics especially for time-resolved studies, sensitivity and measurement speed are…

Absorption spectroscopy is a widely used technique that permits the detection and characterization of gas species at low concentrations. We propose a sensing strategy combining the advantages of frequency modulation spectroscopy with the…

Quantum Physics · Physics 2023-03-30 Alexandre Belsley

We achieve a quantum-noise-limited absorption sensitivity of 1.7/times10$^{-12}$ cm$^{-1}$ per spectral element at 400 s of acquisition time with cavity-enhanced frequency comb spectroscopy, the highest demonstrated for a comb-based…

High finesse frequency combs (HFC) with large ratio of the frequency spacing to the width of the spectral components have demonstrated remarkable results in many applications such as precision spectroscopy and metrology. We found that low…

The broadband, coherent nature of narrow-linewidth fiber frequency combs is exploited to measure the full complex spectrum of a molecular gas through multi-heterodyne spectroscopy. We measure the absorption and phase shift experienced by…

Optics · Physics 2009-11-13 Ian Coddington , William C. Swann , Nathan R. Newbury

The frequency comb of a multimode interferometer offers exceptional scalability potential for field-encoded quantum information. However, the staple field detection method, homodyne detection, cannot access quantum information in the whole…

Quantum Physics · Physics 2026-03-11 Bakhao Dioum , Virginia D'Auria , Alessandro Zavatta , Olivier Pfister , Giuseppe Patera

We suggest an all-optical scheme for the storage, retrieval and processing of a single-photon wave packet through its off-resonant Raman interaction with a series of coherent control beams. These control beams, each with distinct carrier…

Quantum Physics · Physics 2016-12-09 Xiwen Zhang , Alexey Kalachev , Philip Hemmer , Olga Kocharovskaya

Sensing platforms based upon photonic integrated circuits have shown considerable promise; however, they require corresponding advancements in integrated optical readout technologies. Here, we present an on-chip spectrometer that leverages…

Optical frequency-comb-based-high-resolution spectrometers offer enormous potential for spectroscopic applications. Although various implementations have been demonstrated, the lack of suitable mid-infrared comb sources has impeded…

Frequency combs have revolutionized the field of optical spectroscopy, enabling researchers to probe molecular systems with a multitude of accurate and precise optical frequencies. While there have been tremendous strides in direct…

Computational techniques have gained significant traction in photonics, enabling the co-design of hardware and data processing algorithms to drastically simplify optical system architectures and improve their performance. However, their…

Optics · Physics 2026-01-19 J. J. Navarro-Alventosa , A. Aupart-Acosta , V. Duran

Frequency combs based on nonlinear-optical phenomena in integrated photonics are a versatile light source that can explore new applications, including frequency metrology, optical communications, and sensing. We demonstrate robust…

Fourier transform spectroscopy based on incoherent light sources is a well-established tool in research fields from molecular spectroscopy and atmospheric monitoring to material science and biophysics. It provides broadband molecular…

We have demonstrated a new technique that provides massively parallel comb spectroscopy sensitive specifically to ions through the combination of cavity-enhanced direct frequency comb spectroscopy with velocity modulation spectroscopy.…

Atomic Physics · Physics 2015-05-28 Laura C. Sinclair , Kevin C. Cossel , Tyler Coffey , Jun Ye , Eric A. Cornell

Optical frequency combs have had a remarkable impact on precision spectroscopy. Enabling this technology in the x-ray domain is expected to result in wide-ranging applications, such as stringent tests of astrophysical models and quantum…

Dual-comb spectroscopy is emerging as one of the most appealing applications of mid-infrared frequency combs for high-resolution molecular spectroscopy, as it leverages on the unique coherence properties of frequency combs combined with the…

We formulate theoretically and demonstrate experimentally an all-optical method for reconstruction of the amplitude, phase and coherence of frequency combs from a single-shot measurement of the spectral intensity. Our approach exploits…

Astronomical spectrographs require frequency calibration through sources like hollow-cathode lamps or absorption-gas cells. Laser frequency combs (LFCs) provide highest accuracy but are facing operational challenges. We aim to provide a…

Instrumentation and Methods for Astrophysics · Physics 2024-09-05 Ansgar Reiners , Michael Debus , Sebastian Schäfer , Eberhard Tiemann , Mathias Zechmeister

Dual-comb spectroscopy is a powerful technique for real-time, broadband optical sampling of molecular spectra which requires no moving components. Recent developments with microresonator-based platforms have enabled frequency combs at the…

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