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The search for high-quality transition metal dichalcogenides mono- and multi-layers grown on large areas is still a very active field of investigation nowadays. Here, we use molecular beam epitaxy to grow 15$\times$15 mm large WSe$_2$ on…

We report on the growth of epitaxial ZnO thin films and ZnO based heterostructures on sapphire substrates by laser molecular beam epitaxy (MBE). We first discuss some recent developments in laser-MBE such as flexible ultra-violet laser beam…

Materials Science · Physics 2014-01-14 Matthias Opel , Stephan Geprägs , Matthias Althammer , Thomas Brenninger , Rudolf Gross

We report on the growth of epitaxial Sr2RuO4 films using a hybrid molecular beam epitaxy approach in which a volatile precursor containing RuO4 is used to supply ruthenium and oxygen. The use of the precursor overcomes a number of issues…

Materials Science · Physics 2017-10-05 Patrick B. Marshall , Honggyu Kim , Kaveh Ahadi , Susanne Stemmer

Iron(II) monoxide (FeO) is thermodynamically stable in the halite (w\"ustite) structure only at elevated temperatures in a typically non-stoichiometric, Fe-deficient, Fe$_{1-z}$O form that tends to phase separate and/or transform into…

The stoichiometric "111" iron-based superconductor, LiFeAs, has attacted great research interest in recent years. For the first time, we have successfully grown LiFeAs thin film by molecular beam epitaxy (MBE) on SrTiO3(001) substrate, and…

Materials Science · Physics 2015-03-12 Kai Chang , Peng Deng , Teng Zhang , Hai-Cheng Lin , Kun Zhao , Shuai-Hua Ji , Lili Wang , Ke He , Xu-Cun Ma , Xi Chen , Qi-Kun Xue

In this study, high-quality thin films of the topological semimetal phase NiTe$_2$ were prepared using molecular beam epitaxy (MBE) technique, confirmed through X-ray diffraction with pronounced Laue oscillations. Electrical transport…

Materials Science · Physics 2024-08-05 Liguo Zhang , Dapeng Zhao , Xiangyang Liu , Junwen Lai , Junhai Ren , Qin Wang , Haicheng Lin , Yan Sun , Katsumi Tanigaki

Epitaxial La doped BaSnO3 films were grown in an adsorption controlled regime by molecular beam epitaxy, where the excess volatile SnOx desorbs from the film surface. A film grown on a (001) DyScO3 substrate exhibited a mobility of 183 cm^2…

Rutile GeO$_2$ is a promising ultra-wide bandgap semiconductor for future power electronic devices whose alloy with the wide bandgap semiconductor rutile-SnO$_2$ enables bandgap engineering and the formation of heterostructure devices. The…

Materials Science · Physics 2025-01-23 Wenshan Chen , Kingsley Egbo , Joe Kler , Andreas Falkenstein , Jonas Lähnemann , Oliver Bierwagen

By employing a mixed SnO$_2$+Sn source, we demonstrate suboxide molecular beam epitaxy growth of phase-pure single crystalline metastable SnO(001) thin films at a growth rate of ~1.0nm/min without the need for additional oxygen. These films…

In this work we investigate the growth of $\beta$-Ga2O3 homoepitaxial layers on top of (100) oriented substrates via indium-assisted metal exchange catalyzed molecular beam epitaxy (MEXCAT-MBE) which have exhibited prohibitively low growth…

Materials Science · Physics 2020-12-21 Piero Mazzolini , Andreas Falkenstein , Zbigniew Galazka , Manfred Martin , Oliver Bierwagen

We have investigated a method for substituting oxygen with nitrogen in EuO thin films, which is based on molecular beam epitaxy distillation with NO gas as the oxidizer. By varying the NO gas pressure, we produce crystalline, epitaxial…

Materials Science · Physics 2012-05-23 R. Wicks , S. G. Altendorf , C. Caspers , H. Kierspel , R. Sutarto , L. H. Tjeng , A. Damascelli

BaTiO3 is a technologically relevant material in the perovskite oxide class with above room temperature ferroelectricity and a very large electro optical coefficient, making it highly suitable for emerging electronic and photonic devices.…

To advance fundamental understanding, and ultimate application, of transition-metal dichalcogenide (TMD) monolayers, it is essential to develop capabilities for the synthesis of high-quality single-layer samples. Molecular beam epitaxy…

Materials Science · Physics 2020-01-22 Akhil Rajan , Kaycee Underwood , Federico Mazzola , Philip D. C. King

Materials informatics exploiting machine learning techniques, e.g., Bayesian optimization (BO), has the potential to offer high-throughput optimization of thin-film growth conditions through incremental updates of machine learning models in…

High temperatures promote kinetic processes which can drive crystal synthesis towards ideal thermodynamic conditions, thereby realizing samples of superior quality. While accessing very high temperatures in thin-film epitaxy is becoming…

Materials Science · Physics 2024-11-06 Jeong Rae Kim , Sandra Glotzer , Adrian Llanos , Salva Salmani-Rezaie , Joseph Falson

Atomically thin transition metal dichalcogenide films with distorted trigonal (1T$^\prime$) phase have been predicted to be candidates for realizing quantum spin Hall effect. Growth of 1T$^\prime$ film and experimental investigation of its…

Materials Science · Physics 2019-12-04 Xue Zhou , Zeyu Jiang , Kenan Zhang , Wei Yao , Mingzhe Yan , Hongyun Zhang , Wenhui Duan , Shuyun Zhou

As-grown superconducting MgB_2 thin films have been grown on SrTiO_3(001), MgO(001), and Al_2O_3(0001) substrates by a molecular beam epitaxy (MBE) method with novel co-evaporation conditions of low deposition rate in ultra-high vacuum. The…

Superconductivity · Physics 2009-11-10 Y. Harada , M. Udsuka , Y. Nakanishi , M. Yoshizawa

We studied structural, optical and magnetic properties of high-quality 5 and 15% Co-doped ZnO films grown by plasma-assisted molecular beam epitaxy (MBE) on (0001)-sapphire substrates. Magnetic force microscopy (MFM) and magnetic…

The growth of wafer-scale van der Waals (vdW) thin films and heterostructures by molecular beam epitaxy (MBE) is important for future applications in quantum technologies, next generation optoelectronic devices, and fundamental physics…

Materials Science · Physics 2025-08-13 Qihua Zhang , Maria Hilse , Stephanie Law

Materials with perpendicular magnetic anisotropy (PMA) effect with high Curie temperature ($T_C$) is essential in applications. In this work, $Cr_2Te_3$ thin films showing PMA with $T_C$ ranging from 165 K to 295 K were successfully grown…

Materials Science · Physics 2019-12-24 Hongxi Li , Linjing Wang , Tao Yu , Liang Zhou , Yang Qiu , Hongtao He , Fei Ye , Iam Keong Sou , Gan Wang