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The pump-probe experiments enabled by X-ray free-electron lasers (XFEL) will allow us to directly observe correlated electronic motion with attosecond time resolution by detecting photoelectron pairs in coincidence. In helium, the…

We propose a new scenario to apply IR-pump-XUV-probe schemes to resolving strong field ionization induced and attosecond pulse driven electron-hole dynamics and coherence in real time. The coherent driving of both the infrared laser and the…

Atomic Physics · Physics 2016-02-26 Jing Zhao , Jianmin Yuan , Zengxiu Zhao

A two-dimensional model atom is employed to study the ionization behavior of initially excited atomic states in highly-frequent intense laser pulses beyond the dipole approximation. An additional regime of ionization suppression is found at…

Atomic Physics · Physics 2009-11-11 Andreas Staudt , Christoph H. Keitel , John S. Briggs

Stimulated by a recent measurement of coherent control in photoionization of atomic barium, we have calculated one- and two-photon ionization cross sections of the aligned 6s6p^1P_1 state of barium in the energy range between the 5d_{3/2}…

Expression for the probability of the spontaneous emission of high-order harmonics when the emitter phases are synchronized and are obtained in the region where the multiphoton approximation is applicable to the description of the…

Atomic Physics · Physics 2017-09-12 K. V. Ivanyan

Fano resonances are ubiquitous phenomena appearing in many fields of physics, e.g. atomic or molecular photoionization, or electron transport in quantum dots. Recently, attosecond interferometric techniques have been used to measure the…

We investigate the angle-resolved photoelectron spectra from laser-assisted photoionization for helium and neon atoms using an \textit{ab initio} method based on time-dependent surface flux and configuration interaction singles. We find…

Atomic Physics · Physics 2020-08-26 Mattias Bertolino , David Busto , Felipe Zapata , Jan Marcus Dahlström

Clusters and nanodroplets hold the promise of enhancing high-order nonlinear optical effects due to their high local density. However, only moderate enhancement has been demonstrated to date. Here, we report the observation of energetic…

We study high-order harmonic generation in aligned molecules close to the ionization threshold. Two distinct contributions to the harmonic signal are observed, which show very different responses to molecular alignment and ellipticity of…

Atomic Physics · Physics 2011-09-16 H. Soifer , P. Botheron , D. Shafir , A. Diner , O. Raz , B. D. Bruner , Y. Mairesse , B. Pons , N. Dudovich

We report on the observation, characterization, and control of the electron dynamics in ionized argon atoms. We utilized an intense mid-infrared (MIR) pulse to create a coherent superposition of the spin-orbit split ground state of the ion.…

Energy coupling during relativistically intense laser-matter interactions is encoded in the attosecond motion of strongly driven electrons at the pre-formed plasma-vacuum boundary. Studying and controlling this motion can reveal details…

We present fully ab initio simulations of attosecond streaking for ionization of helium accompanied by shake-up of the second electron. This process represents a prototypical case for strongly correlated electron dynamics on the attosecond…

Atomic Physics · Physics 2013-05-24 Renate Pazourek , Stefan Nagele , Johannes Feist , Joachim Burgdörfer

Above-threshold ionization spectra from cesium are measured as a function of the carrier-envelope phase (CEP) using laser pulses centered at 3.1 $\mu$m wavelength. The directional asymmetry in the energy spectra of backscattered electrons…

Fully quantum treatment explicitly presents the high harmonic generation as a three-stage process: above threshold ionization (ATI) is followed by the continuum electron propagation in a laser field and subsequent stimulated recombination…

Atomic Physics · Physics 2009-10-31 M. Yu. Kuchiev , V. N. Ostrovsky

We have examined the profile of an isolated autoionizing resonance driven by a pulse of short duration and moderately strong field. The analysis has been based on stochastic differential equations governing the time evolution of the density…

Atomic Physics · Physics 2018-03-06 G. Mouloudakis , P. Lambropoulos

Phase-shift differences and amplitude ratios of the outgoing $s$ and $d$ continuum wave packets generated by two-photon ionization of helium atoms are determined from the photoelectron angular distributions obtained using velocity map…

The photoionization of a helium atom by short intense laser pulses is studied theoretically in the vicinity of the $2s2p\,^1P$ doubly-excited state with the intention to investigate the impact of the intensity and duration of the exciting…

Atomic Physics · Physics 2017-09-20 Anton N. Artemyev , Lorenz S. Cederbaum , Philipp V. Demekhin

Isolated attosecond pulses (IAPs) produced through laser-driven high-harmonic generation (HHG) hold promise for unprecedented insight into biological processes via attosecond x-ray diffraction with tabletop sources. However, efficient…

High harmonic light sources make it possible to access attosecond time-scales, thus opening up the prospect of manipulating electronic wave packets for steering molecular dynamics. However, two decades after the birth of attosecond physics,…

Ionization by relativistically intense short laser pulses is studied in the framework of strong-field quantum electrodynamics. Distinctive patterns are found in the energy probability distributions of photoelectrons. Except of the already…

Atomic Physics · Physics 2018-03-14 F. Cajiao Vélez , J. Z. Kamiński , K. Krajewska