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We consider harmonics generation and wave-mixing by two-color multi photon resonant excitation of three-level atoms/molecules in strong laser fields. The coherent part of the spectra corresponding to multicolor harmonics generation is…

Atomic Physics · Physics 2016-08-24 H. K. Avetissian , B. R. Avchyan , G. F. Mkrtchian

Microscopic nonlinear quantum theory of interaction of coherent electromagnetic radiation with gapped bilayer graphene is developed. The Liouville-von Neumann equation for the density matrix is solved numerically at the multiphoton…

Mesoscale and Nanoscale Physics · Physics 2019-05-21 H. K. Avetissian , A. K. Avetissian , A. G. Ghazaryan , Kh. V. Sedrakian , G. F. Mkrtchian

High-order harmonic generation (HHG) results from strong-field laser matter interaction and it is one of the main processes that are used to extract electron structural and dynamical information about the atomic or molecular targets with…

In the past two decades high-harmonic generation (HHG) has become a key process in ultra-fast science due to the extremely short time-structure of the underlying electron dynamics being imprinted in the emitted harmonic light bursts. After…

Atomic Physics · Physics 2012-01-25 Markus C. Kohler , Thomas Pfeifer , Karen Z. Hatsagortsyan , Christoph H. Keitel

We employ the two-band density-matrix equations and time-dependent density functional theory to calculate high-order harmonic generation (HOHG) in graphene under a femtosecond laser irradiation. Our investigation uncovers a striking…

Atomic Physics · Physics 2023-07-25 Fulong Dong , Qinzhi Xia , Jie Liu

Using Time-Dependent Density Functional Theory (TDDFT) nonlinear nonperturbative response of the molecular system is studied for photoisomerization reaction. The 1,3-cyclohexadiene photoisomerization is probed by the high-harmonic…

Chemical Physics · Physics 2024-08-06 Lauren Bauerle , Agnieszka Jaron

High-harmonic generation (HHG) in condensed-matter systems is both a source of fundamental insight into quantum electron motion and a promising candidate to realize compact ultraviolet and ultrafast light sources. Here we argue that the…

Mesoscale and Nanoscale Physics · Physics 2017-03-08 Joel D. Cox , Andrea Marini , F. Javier García de Abajo

Strongly driven systems of emitters offer an attractive source of light over broad spectral ranges up to the X-ray region. A key limitation of these systems is that the light they emit is for the most part classical. We challenge this…

Quantum Physics · Physics 2023-06-06 Andrea Pizzi , Alexey Gorlach , Nicholas Rivera , Andreas Nunnenkamp , Ido Kaminer

We theoretically investigate correlated electron dynamics in high-harmonic generation (HHG), using all-electron \emph{ab initio} simulations for three-dimensional real alkali-metal atoms. The resulting harmonic spectra exhibit a plateau…

Atomic Physics · Physics 2019-04-10 Yang Li , Takeshi Sato , Kenichi L. Ishikawa

Quantum-optical descriptions of strong-field processes have attracted significant attention in recent years. Typically, the theoretical modeling has been conducted in the Schr\"odinger picture, where results are only obtainable under…

High-order harmonic generation (HHG) in simultaneous intense near-infrared (NIR) laser light and brilliant x rays above an inner-shell absorption edge is examined. A tightly bound inner-shell electron is transferred into the continuum.…

High harmonic generation (HHG) enables extreme ultraviolet radiation with table-top setups. Its exceptional properties, such as coherence and (sub)-femtosecond pulse durations, have led to a diversity of applications. Some of these require…

Several correlation and interference effects in strong-field physics are investigated. We show that the interference of continuum wave packets can be the dominant mechanism of high-harmonic generation (HHG) in the over-the-barrier regime.…

High-harmonic generation (HHG) in solids has rapidly emerged as a promising platform for creating compact attosecond sources and probing ultrafast electron dynamics. Resonant metasurfaces are essential for enhancement of the otherwise small…

We present derivation and implementation of the Multi-Configurational Strong-Field Approximation with Gaussian nuclear Wave Packets (MC-SFA-GWP) -- a version of the molecular strong-field approximation which treats all electronic and…

Chemical Physics · Physics 2017-11-10 Serguei Patchkovskii , Michael S. Schuurman

Nonlinear light-matter interaction and, in particular, high-harmonic generation (HHG) are fundamentally interesting and frequently discussed as versatile probes of quantum materials with potential for optical information processing…

Mesoscale and Nanoscale Physics · Physics 2026-04-15 Jessica O. de Almeida , Wilton J. M. Kort-Kamp , Mathias S. Scheurer

We present a study of photon statistics associated with high-order harmonic generation (HHG) involving one-mode and intermodal correlations of the high harmonic photons. The aim of the paper is to give insight into the nonclassical…

Quantum Physics · Physics 2021-09-15 Ákos Gombkötő , Péter Földi , Sándor Varró

We explore the roles of electronic band structure and Coulomb interactions in solid-state HHG by studying the optical response of linear atomic chains and carbon nanotubes to intense ultrashort pulses. Specifically, we simulate electron…

Mesoscale and Nanoscale Physics · Physics 2020-03-18 Sandra de Vega , Joel D. Cox , Fernando Sols , F. Javier García de Abajo

We study high-harmonic generation (HHG) in the one-dimensional Hubbard model in order to understand its relation to elementary excitations as well as the similarities and differences to semiconductors. The simulations are based on the…

Strongly Correlated Electrons · Physics 2021-01-13 Yuta Murakami , Shintaro Takayoshi , Akihisa Koga , Philipp Werner

We theoretically demonstrate x-ray second harmonic generation (SHG) with strong-field-driven high harmonic generation (HHG) from core electrons in gas-phase atoms, highlighting its potential as a powerful spectroscopic tool for studying…

Atomic Physics · Physics 2025-03-31 Xinhua Xie