Related papers: Terahertz spin dynamics in rare-earth orthoferrite…
The magnetic circular dichroism and the Faraday rotation are the fundamental phenomena of great practical importance arising from the breaking of the time reversal symmetry by a magnetic field. In most materials the strength and the sign of…
Spintronics, a transformative field of research, leverages the spin of electron to revolutionize electronic devices, offering significant advantages over traditional charge-based systems. This chapter highlights the critical role of novel…
Narrowband terahertz (THz) radiation is crucial for high-resolution spectral identification, but a narrowband THz source driven by femtosecond (fs) laser has remained scarce. Here, it is computationally predicted that a…
Electronic excitations in a ferromagnet can trigger ultrafast spin dynamics with potential applications in a speed increase in magnetic recording. The project investigates ultrafast magnetization dynamics, which is driven in metallic layers…
Coherent radiation with frequencies ranging from 0.3 to 30 THz has recently become accessible by femtosecond laser technology. Terahertz (THz) waves have already found many applications in spectroscopy and imaging, and they can be…
A pair of circularly polarized laser pulses of opposite helicities are shown to control the route of spin reorientation phase transition in rare-earth antiferromagnetic orthoferrite (Sm$_{0.55}$Tb$_{0.45}$)FeO$_3$. The route can be…
Strong-field terahertz (THz) excitations enable dynamic control over electronic, lattice and symmetry degrees of freedom in quantum materials. Here, we uncover pronounced terahertz-induced symmetry modulations and coherent phonon dynamics…
Antiferromagnetic (AFM) materials possess a well-recognized potential for ultrafast data processing thanks to their intrinsic ultrafast spin dynamics, absence of stray fields, and large spin transport effects. The very same properties,…
Spin-orbit-torque-driven dynamics have recently gained interest in the field of magnetism due to the reduced requirement of current densities and an increase in efficiency, as well as the ease of implementation of different devices and…
State-of-the-art metallic terahertz (THz) emitters rely predominantly on spintronic heterostructures, where heavy metals serve as passive spin-to-charge converters. Here, we demonstrate efficient THz radiation from standalone Pt nanofilms…
Spin-transfer torque and spin Hall effects combined with their reciprocal phenomena, spin-pumping and inverse spin Hall (ISHE) effects, enable the reading and control of magnetic moments in spintronics. The direct observation of these…
We report a comprehensive study of spin dynamics in the (Mo2/3Tb1/3)2AlC i-MAX compound using ac susceptibility measurements across a range of magnetic fields. Unique behaviors were observed, including spin dynamics in the kHz range between…
Recent observations of topological spin textures brought spintronics one step closer to new magnetic memories. Nevertheless, the existence of Skyrmions, as well as their stabilization, require very specific intrinsic magnetic properties…
Femtosecond laser excitation of materials that exhibit magnetic spin textures promises advanced magnetic control via the generation of ultrafast and non-equilibrium spin dynamics. We explore such possibilities in ferrimagnetic [Fe(0.35…
We report on terahertz (THz) electron paramagnetic resonance generalized spectroscopic ellipsometry (THz-EPR-GSE). Measurements of the field and frequency dependencies of the magnetic response due to the spin transitions associated with the…
Magneto-terahertz phenomena are the main focus of the thesis. This work started as supporting research for the science of an X-ray laser (SwissFEL). X-ray lasers have recently drawn great attention as an unprecedented tool for scientific…
The unique functionalities of antiferromagnets offer promising routes to advance information technology. Their compensated magnetic order leads to spin resonances in the THz-regime, which suggest the possibility to coherently control…
Magnetic polarons can generate colossal magnetoresistance in magnetic semiconductors, yet their terahertz electrodynamics remain largely unexplored. Here we report magneto-terahertz spectroscopy of the Eu-based Zintl antiferromagnet…
Recent studies in spintronics have highlighted ultrathin magnetic metallic multilayers as a novel and very promising class of broadband terahertz radiation sources. Such spintronic multilayers consist of ferromagnetic (FM) and non-magnetic…
Near-infrared (NIR) pump-terahertz (THz) probe spectroscopy is used to investigate the charge and spin exciations in a strongly correlated electron compound Na0.5CoO2. This compound exhibits a coexistence of various charge and spin orders…