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We study dynamics of incoherent exciton formation under interband photoexcitation in Cu$_2$O using time-and angle-resolved photoemission spectroscopy at 90 K. Hot electrons injected by allowed optical transitions with 3.40-eV photons show…

Mesoscale and Nanoscale Physics · Physics 2019-10-23 H. Tanimura , K. Tanimura , P. H. M. van Loosdrecht

Transport of elementary excitations is a fundamental property of 2D semiconductors, important for wide-ranging emergent phenomena and device applications. While exciton transport reported in 2D materials barely exceeds 1-2 $\mu$m, coherent…

Optics · Physics 2025-06-03 Xin Xie , Qiuyang Li , Chenxi Liu , Yuze Liu , Chulwon Lee , Kai Sun , Hui Deng

The growth of single crystals of MoS2 and WS2 by materials transport through a liquid salt flux made from a low melting mixture of NaCl and CsCl is described. The crystals are characterized by single crystal X-ray diffraction, which reveals…

We study the photoluminescence dynamics of ultra-cold indirect excitons optically created in a double quantum well heterostructure. Above a threshold laser excitation, our experiments reveal the apparition of the so-called inner…

Mesoscale and Nanoscale Physics · Physics 2012-02-10 M. Alloing , A. Lemaitre , E. Galopin , F. Dubin

In heterostructures consisting of different transition-metal dichalcogenide monolayers, a staggered band alignment can occur, leading to rapid charge separation of optically generated electron-hole pairs into opposite monolayers. These…

Photogenerated carrier transport and recombination in metal halide perovskites are critical to device performance. Despite considerable efforts, sample quality issues and measurement techniques have limited the access to their intrinsic…

Perovskites have attracted much attention due to their remarkable optical properties. While it is well established that excitons dominate their optical response, the impact of higher excitonic states and formation of phonon sidebands in…

Mesoscale and Nanoscale Physics · Physics 2020-11-04 David Feldstein , Raul Perea-Causin , Shuli Wang , Mateusz Dyksik , Kenji Watanabe , Takashi Taniguchi , Paulina Plochocka , Ermin Malic

Reflectance and magneto-reflectance experiments together with theoretical modelling based on the $\mathbf{k\cdot p}$ approach have been employed to study the evolution of direct bandgap excitons in MoS$_2$ layers with a thickness ranging…

Mesoscale and Nanoscale Physics · Physics 2019-03-01 A. O. Slobodeniuk , Ł. Bala , M. Koperski , M. R. Molas , P. Kossacki , K. Nogajewski , M. Bartos , K. Watanabe , T. Taniguchi , C. Faugeras , M. Potemski

In transition metal dichalcogenides layers of atomic scale thickness, the electron-hole Coulomb interaction potential is strongly influenced by the sharp discontinuity of the dielectric function across the layer plane. This feature results…

We study the effect of one-dimensional (1D) photonic crystal heterojunction (h-PhC) on the light absorption and light emission of monolayer molybdenum disulfide (MoS$_{2}$), and obtained the analytical solution of the light absorption and…

Mesoscale and Nanoscale Physics · Physics 2017-09-15 Liu Jiang-tao , Tong Hong , Wu Zhen-Hua , Huang Jin-Bao , Zhou Yun-Song

The dynamics of excess protons in the protic ionic liquid ethylammonium formate (EAF) have been investigated from femtosecond to microseconds using visible pump mid-infrared probe spectroscopy. The pH-jump following visible photoexcitation…

We present a systematic study of the exciton/electron-hole plasma photoluminescence dynamics in bulk GaAs for various lattice temperatures and excitation densities. The competition between the exciton and electron-hole pair recombination…

Materials Science · Physics 2009-11-22 A. Amo , M. D. Martin , L. Vina , A. I. Toropov , K. S. Zhuravlev

Time-resolved photoluminescence spectra after nonresonant excitation show a distinct 1s resonance, independent of the existence of bound excitons. A microscopic analysis identifies excitonic and electron-hole plasma contributions. For low…

Condensed Matter · Physics 2009-11-10 S. Chatterjee , C. Ell , S. Mosor , G. Khitrova , H. M. Gibbs , W. Hoyer , M. Kira , S. W. Koch , J. P. Prineas , H. Stolz

The excitonic luminescence of an isolated polydiacetylene polymer chain in its monomer matrix is studied by micro-photoluminescence. These chains behave as perfect 1D excitonic systems with the expected 1/sqrt{E} density of states between 5…

Materials Science · Physics 2007-05-23 F. Dubin

In recent years it has become clear that the transport of excitons and charge carriers in molecular systems can be enhanced by coherent coupling with photons, giving rise to the formation of hybrid excitations known as polaritons. Such…

Materials Science · Physics 2023-01-19 M. Balasubrahmaniyam , Arie Simkovich , Adina Golombek , Guy Ankonina , Tal Schwartz

The interplay of optics, dynamics and transport is crucial for the design of novel optoelectronic devices, such as photodetectors and solar cells. In this context, transition metal dichalcogenides (TMDs) have received much attention. Here,…

Mesoscale and Nanoscale Physics · Physics 2019-11-04 Raul Perea-Causin , Samuel Brem , Roberto Rosati , Roland Jago , Marvin Kulig , Jonas D. Ziegler , Jonas Zipfel , Alexey Chernikov , Ermin Malic

We investigate excitonic transitions in a h-BN encapsulated monolayer $\textrm{MoS}_2$ phototransistor by photocurrent spectroscopy at cryogenic temperature (T = 5 K). The spectra presents excitonic peaks with linewidths as low as 8 meV,…

The optical responses of semiconducting transition metal dichalcogenides are dominated by excitons. Being able to strongly interact with light and other materials excitations, excitons in semiconductors are prototypes for investigating…

Mesoscale and Nanoscale Physics · Physics 2021-01-28 Xuke Jiang , Masoud Taleb , Florian Diekmann , Kai Rossnagel , Nahid Talebi

Light emission from higher-order correlated excitonic states has been recently reported in hBN-encapsulated monolayer WSe2 and WS2 upon optical excitation. These exciton complexes are found to be bound states of excitons residing in…

Mesoscale and Nanoscale Physics · Physics 2019-04-19 Matthias Paur , Aday J. Molina-Mendoza , Rudolf Bratschitsch , Kenji Watanabe , Takashi Taniguchi , Thomas Mueller

Light emitters in vicinity of a hyperbolic metamaterial (HMM) show a range of quantum optical phenomena from spontaneous decay rate enhancement to strong coupling. In this study, we integrate monolayer Molybdenum disulfide (MoS$_2$) emitter…

Optics · Physics 2022-08-05 Harshavardhan R. Kalluru , Jaydeep K. Basu