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Large-scale quantum networks rely on optical fiber networks and photons as so-called flying qubits for information transport. While dispersion and absorption of optical fibers are minimum at the infrared telecom wavelengths, most atomic and…

In large-area quantum networks based on optical fibers, photons are the fundamental carriers of information as so-called flying qubits. They may also serve as the interconnect between different components of a hybrid architecture, which…

Quantum Physics · Physics 2024-12-05 Anica Hamer , Frank Vewinger , Thorsten Peters , Michael H. Frosz , Simon Stellmer

Large-area quantum networks based on optical fibers allow photons at near-infrared wavelengths to travel with minimal loss. Quantum frequency conversion is a method to alter the wavelength of a single photon while maintaining its quantum…

Quantum Physics · Physics 2025-06-09 Anica Hamer , Frank Vewinger , Michael H. Frosz , Simon Stellmer

Optical spectroscopy and imaging of microscopic samples have opened up a wide range of applications throughout the physical, chemical, and biological sciences. High chemical specificity may be achieved by directly interrogating the…

Coherent anti-Stokes Raman scattering (CARS) spectroscopy with time-delayed ultrashort pulses and a single-pixel photodetector has shown great potential for spectroscopic imaging and transient studies in chemistry and biological research.…

Optics · Physics 2023-12-05 Tianjian Lv , Bing Han , Ming Yan , Zhaoyang Wen , Kun Huang , Kangwen Yang , Heping Zeng

Practical implementations of quantum information networks require frequency conversion of individual photons. Approaches based on a molecular gas as the nonlinear medium cover a wide range of the optical spectrum and promise high efficiency…

Quantum Physics · Physics 2025-06-09 Anica Hamer , Frank Vewinger , Michael H. Frosz , Simon Stellmer

Coherent anti-Stokes Raman scattering (CARS) microspectroscopy has demonstrated significant potential for biological and materials imaging. To date, however, the primary mechanism of disseminating CARS spectroscopic information is through…

Optics · Physics 2015-10-08 Charles H. Camp , Young Jong Lee , Marcus T. Cicerone

We have developed an interferometric implementation of coherent anti-Stokes Raman scattering (CARS) which enables broadband coherent Raman spectroscopy free from non-resonant background (NRB), with a signal strength proportional to…

Optics · Physics 2014-02-25 Brad Littleton , Thomas Kavanagh , Frederic Festy , David Richards

Frequency modulation coherent anti-Stokes Raman scattering (FM CARS) is presented, using a compact as well as fast and widely tunable fiber-based light source. With this light source Raman resonances between 700 cm$^{-1}$ and 3200 cm$^{-1}$…

Broadband-tunable sources of circularly-polarized light are crucial in fields such as laser science, biomedicine and spectroscopy. Conventional sources rely on nonlinear wavelength conversion and polarization control using standard optical…

Optics · Physics 2019-04-16 S. Davtyan , D. Novoa , Y. Chen , M. H. Frosz , P. St. J. Russell

When a laser pump beam of sufficient intensity is incident on a Raman-active medium such as hydrogen gas, a strong Stokes signal, red-shifted by the Raman transition frequency {\Omega}$_R$, is generated. This is accompanied by the creation…

We present a unified view of the frequency dependence of the various scattering processes involved when a neutral hydrogen atom interacts with a monochromatic, linearly-polarized photon. A computational approach is employed of the atom…

Atomic Physics · Physics 2016-06-06 Swaantje J. Grunefeld , Michael W. J. Bromley , Yongjun Cheng

We experimentally demonstrate frequency translation of a nonclassical optical field via the Bragg scattering four-wave mixing process in a photonic crystal fiber (PCF). The high nonlinearity and the ability to control dispersion in PCF…

Quantum Physics · Physics 2010-09-08 H. J. McGuinness , M. G. Raymer , C. J. McKinstrie , S. Radic

We report coherent association of atoms into a single weakly bound NaCs molecule in an optical tweezer through an optical Raman transition. The Raman technique uses a deeply bound electronic excited intermediate state to achieve a large…

We present a quantum-mechanical model that describes fiber-based frequency conversion by four-wave-mixing Bragg scattering in the presence of Raman interactions. In the case of continuous-wave pumps we find closed-form expressions for the…

Quantum Physics · Physics 2024-06-06 Mathias Linde Holst Korsgaard , Jacob Gade Koefoed , Karsten Rottwitt

Molecular hydrogen is a benchmark system for bound state quantum calculation and tests of quantum electrodynamical effects. While spectroscopic measurements on the stable species have progressively improved over the years, high resolution…

Atomic Physics · Physics 2017-11-22 M. Schlösser , X. Zhao , M. Trivikram , W. Ubachs , E. J. Salumbides

We report a resource-efficient scheme in which a single pump laser was used to achieve frequency conversion by Bragg-scattering four-wave mixing in a photonic crystal fiber. We demonstrate bidirectional conversion of coherent light between…

We experimentally demonstrate efficient Raman conversion to respective Stokes and anti-Stokes fields in both pulsed and continuous modes with a Rb-87 atomic vapor cell. The conversion efficiency is about 40-50% for the Stokes field and…

Atomic Physics · Physics 2012-10-19 Bing Chen , Kai Zhang , Chun-Hua Yuan , Chengling Bian , Cheng Qiu , L. Q. Chen , Z. Y. Ou , Weiping Zhang

Quantum frequency conversion, the process of shifting the frequency of an optical quantum state while preserving quantum coherence, can be used to produce non-classical light at otherwise unapproachable wavelengths. We present experimental…

Quantum Physics · Physics 2021-08-30 Hugo Kerdoncuf , Jesper B. Christensen , Mikael Lassen

The unique ring-shaped intensity patterns and helical phase fronts of optical vortices make them useful in many applications. Here we report for the first time efficient Raman frequency conversion between vortex modes in twisted…

Optics · Physics 2020-04-22 S. Davtyan , Y. Chen , M. H. Frosz , P. ST. J. Russell , D. Novoa
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