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Electron-electron correlation effects play an instrumental role in our understanding of sequential (SDI) and non-sequential double ionization (NSDI) mechanisms. Here, we present a theoretical study of NSDI driven by plasmonic-enhanced…

Solid electrolytes with fast ion transport are one of the key challenges for solid state lithium metal batteries. To improve ion conductivity, chemical doping has been the most effective strategy, and atomistic simulation with…

Orbit-based methods are widespread in strong-field laser-matter interaction. They provide a framework in which photoelectron momentum distributions can be interpreted as the quantum interference between different semi-classical pathways the…

Atomic Physics · Physics 2024-10-03 T. Rook , D. Habibović , C. Figueira de Morisson Faria

We present an implementation of a time-dependent multiconfiguration self-consistent-field (TD-MCSCF) method [R. Anzaki et al., Phys. Chem. Chem. Phys. 19, 22008 (2017)] with the full configuration interaction expansion for coupled…

Atomic Physics · Physics 2021-10-08 Yang Li , Takeshi Sato , Kenichi L. Ishikawa

A theoretical study of the K-shell ionization of hydrogen-like ions, colliding with bare nuclei, is performed within the framework of the time-dependent Dirac equation. Special emphasis is placed on the ionization probability that is…

Atomic Physics · Physics 2023-04-20 O. Novak , R. Kholodov , A. Surzhykov , A. N. Artemyev , Th. Stöhlker

We derive an analytical formula for the ionization rate of neutral atoms and molecules in a strong monochromatic field. Our model is based on the strong-field approximation with transition amplitudes calculated by an extended saddle point…

Atomic Physics · Physics 2007-05-23 Thomas Kim Kjeldsen , Lars Bojer Madsen

The strong-field approximation can be and has been applied in both length gauge and velocity gauge with quantitatively conflicting answers. For ionization of negative ions with a ground state of odd parity, the predictions of the two gauges…

Quantum Physics · Physics 2009-11-11 D. Bauer , D. B. Milosevic , W. Becker

Attosecond dynamics in strong-field tunnel ionization are encoded in intricate holographic patterns in the photoelectron momentum distributions (PMDs). These patterns show the interference between two or more superposed quantum electron…

The orientation-dependent strong-field ionization of CO molecules is investigated using the fully propagated three-dimensional time-dependent Hartree-Fock theory. The full ionization results are in good agreement with recent experiments.…

Atomic Physics · Physics 2013-10-30 Bin Zhang , Jianmin Yuan , Zengxiu Zhao

A simple, analytical, nonrelativistic ionization rate formula for atoms and positive ions in intense ultraviolet and x-ray electromagnetic fields is derived. The rate is valid at arbitrary values of the Keldysh parameter and confirmed by…

Atomic Physics · Physics 2009-11-13 S. V. Popruzhenko , V. D. Mur , V. S. Popov , D. Bauer

Electron dynamics of anatase TiO$_2$ under the influence of ultrashort and intense laser field is studied using the real-time time-dependent density functional theory (TDDFT). Our findings demonstrate the effectiveness of TDDFT calculations…

We review the semiclassical two-step model for strong-field ionization. The semiclassical two-step model describes quantum interference and accounts for the ionic potential beyond the semiclassical perturbation theory. We discuss…

Atomic Physics · Physics 2021-05-05 N. I. Shvetsov-Shilovski

We present a novel ab-initio single-electron approach to correlated electron dynamics in strong laser fields. By writing the electronic wavefunction as a product of a marginal one-electron wavefunction and a conditional wavefunction, we…

Atomic Physics · Physics 2016-02-02 Axel Schild , E. K. U. Gross

Time-dependent quantum chemical methods coupled to Gaussian basis sets are gaining popularity in modeling the electron dynamics of atoms and molecules interacting with intense laser fields. Two approaches most widely used for this purpose,…

Chemical Physics · Physics 2023-01-18 Aleksander P. Woźniak , Maciej Lewenstein , Robert Moszyński

Double electron ionisation process occurs when an intense laser pulse interacts with atoms or molecules. Exact {\it ab initio} numerical simulation of such a situation is extremely computer resources demanding, thus often one is forced to…

We study single-photon ionization of aligned H$_2^+$ in low-intensity near-circular laser fields with lower photon energy numerically and analytically. The photoelectron momentum distribution (PMD) within the laser polarization plane,…

Atomic Physics · Physics 2025-05-13 Z. Y. Chen , S. Q. Shen , M. Q. Liu , J. Y. Che , Y. J. Chen

A versatile semiclassical approximation for intense laser-atom processes is presented. This uniform approximation is no more complicated than the frequently-used multi-dimensional saddle-point approximation and far superior, since it…

Atomic Physics · Physics 2016-09-08 C. Figueira de Morisson Faria , H. Schomerus , W. Becker

We investigate differential electron distributions in nonsequential double ionization (NSDI) with linearly polarized, few-cycle pulses, using a classical model based on a laser-assisted inelastic $(e^-,2e^-)$ rescattering mechanism. We show…

Atomic Physics · Physics 2009-11-10 X. Liu , C. Figueira de Morisson Faria

A time-dependent formulation for electron-hole excitations in extended finite systems, based on the Bethe-Salpeter equation (BSE), is developed using a stochastic wave function approach. The time-dependent formulation builds on the…

Materials Science · Physics 2015-02-11 Eran Rabani , Roi Baer , Daniel Neuhauser

We analytically describe the strong-field light-electron interaction using a quantized coherent laser state with arbitrary photon number. We obtain a light-electron wave function which is a closed-form solution of the time-dependent…

Atomic Physics · Physics 2017-03-20 I. A. Gonoskov , N. Tsatrafyllis , I. K. Kominis , P. Tzallas