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In this article, a previously published amplifier-less potentiostat architecture is further examined. Starting with a linearized model, the impact of the most important parameters is studied taking in account the electrodes-solution…

Systems and Control · Electrical Eng. & Systems 2025-04-30 Andrea Sannino , David-Peter Wiens , Maurits Ortmanns , José I. Artigas , Aránzazu Otín

This paper proposes the linearized physics-based model of a lithium-ion battery that can be incorporated into the optimization framework for power system economic studies. The proposed model is a linear approximation of the single particle…

Systems and Control · Electrical Eng. & Systems 2022-07-08 Anton V. Vykhodtsev , Darren Jang , Qianpu Wang , William Rosehart , Hamidreza Zareipour

Non-destructive characterization of lithium-ion batteries provides critical insights for optimizing performance and lifespan while preserving structural integrity. Optimizing electrolyte design in commercial LIBs requires consideration of…

We develop a mathematical framework to analyze electrochemical impedance spectra in terms of a distribution of diffusion times (DDT) for a parallel array of random finite-length Warburg (diffusion) or Gerischer (reaction-diffusion) circuit…

Chemical Physics · Physics 2018-03-21 Juhyun Song , Martin Z. Bazant

The unified 3D phase-field model for the description of the lithium-ion cell as a whole is developed. The model takes into account the realistic distribution of particles in porous electrodes, percolative transport of ions, and the…

Disordered Systems and Neural Networks · Physics 2021-05-11 Pavel E. L'vov , Mikhail Yu. Tikhonchev , Renat T. Sibatov

Currently, the characterization of electric energy storage units used for power system operation and planning models relies on two major assumptions: charge and discharge efficiencies, and power limits are constant and independent of the…

Systems and Control · Electrical Eng. & Systems 2024-12-20 Alvaro Gonzalez-Castellanos , David Pozo , Aldo Bischi

Numerical simulations are a powerful tool for the development and improvement of Li-ion batteries. Modeling the mass transport of the involved electrolytic solutions requires precise determination of the corresponding electrolyte…

Chemical Physics · Physics 2024-11-21 Lukas Lehnert , Maryam Nojabaee , Arnulf Latz , Birger Horstmann

Fracture of lithium-ion battery electrodes is found to contribute to capacity fade and reduce the lifespan of a battery. Traditional fracture models for batteries are restricted to consideration of a single, idealised particle; here,…

This paper investigates the identification of observable low-frequency (LF) parameters of battery cell's equivalent circuit models (ECMs) using time-domain voltage and current measurements sampled at low frequency by built-in battery…

Systems and Control · Electrical Eng. & Systems 2026-05-29 Vladimir Sovljanski , Mario Paolone

Battery aging is a natural process that contributes to capacity and power fade, resulting in a gradual performance degradation over time and usage. State of Charge (SOC) and State of Health (SOH) monitoring of an aging battery poses a…

Systems and Control · Electrical Eng. & Systems 2021-06-25 Anirudh Allam , Simona Onori

To further improve Lithium-ion batteries (LiBs), a profound understanding of complex battery processes is crucial. Physical models offer understanding but are difficult to validate and parameterize. Therefore, automated machine-learning…

Chemical Physics · Physics 2024-10-28 Micha C. J. Philipp , Yannick Kuhn , Arnulf Latz , Birger Horstmann

The Doyle-Fuller-Newman (DFN) model is a common mechanistic model for lithium-ion batteries. The reaction rate constant and diffusivity within the DFN model are key parameters that directly affect the movement of lithium ions, thereby…

Systems and Control · Electrical Eng. & Systems 2025-04-15 Marc D. Berliner , Minsu Kim , Xiao Cui , Vivek N. Lam , Patrick A. Asinger , Martin Z. Bazant , William C. Chueh , Richard D. Braatz

We build a transient multidimensional multiphysical model based on continuum theories, involving the coupled mechanical, thermal and electrochemical phenomena occurring simultaneously in the discharge or charge of lithium-ion batteries. The…

Numerical Analysis · Mathematics 2024-03-26 Jaime Mora-Paz

Thermal electrochemical models for porous electrode batteries (such as lithium ion batteries) are widely used. Due to the multiple scales involved, solving the model accounting for the porous microstructure is computationally expensive,…

Chemical Physics · Physics 2020-04-14 Matthew J. Hunt , Ferran Brosa Planella , Florian Theil , W. Dhammika Widanage

The response of a model micro-electrochemical system to a time-dependent applied voltage is analyzed. The article begins with a fresh historical review including electrochemistry, colloidal science, and microfluidics. The model problem…

Soft Condensed Matter · Physics 2009-11-10 Martin Z. Bazant , Katsuyo Thornton , Armand Ajdari

Electrochemical Impedance Spectroscopy (EIS) is a crucial technique for assessing corrosion of a metallic materials. The analysis of EIS hinges on the selection of an appropriate equivalent circuit model (ECM) that accurately characterizes…

In this paper, we study a suitable experimental design of electrochemical impedance spectroscopy (EIS) to reduce the number of frequency points while not significantly affecting the uncertainties of the estimated cell's equivalent circuit…

Systems and Control · Electrical Eng. & Systems 2025-01-13 Vladimir Sovljanski , Mario Paolone , Sylvain Tant , Damien Pierre Sainflou

Lithium-ion battery (LIB) sources have played an essential role in self-sustained transportation energy systems and have been widely deployed in the last few years. To realize reliable battery maintenance, identifying its electrochemical…

Systems and Control · Electrical Eng. & Systems 2023-03-15 Yuxuan Gu , Jianxiao Wang , Yuanbo Chen , Kedi Zheng , Zhongwei Deng , Qixin Chen

This paper proposes a fully unsupervised methodology for the reliable extraction of latent variables representing the characteristics of lithium-ion batteries (LIBs) from electrochemical impedance spectroscopy (EIS) data using information…

Signal Processing · Electrical Eng. & Systems 2021-07-14 Seongyoon Kim , Yun Young Choi , Jung-Il Choi

The penetrations of lithium-ion batteries in transport, energy and communication systems are increasing rapidly. A meticulous model applicable for precise in-situ monitoring and convenient online controlling is in sought to bridge the gap…

Systems and Control · Electrical Eng. & Systems 2022-03-22 Yuxuan Gu , Jianxiao Wang , Yuanbo Chen , Zhongwei Deng , Hongye Guo , Kedi Zheng , Qixin Chen