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Colloidal particles or nanoparticles, with equal affinity for two fluids, are known to adsorb irreversibly to the fluid-fluid interface. We present large-scale computer simulations of the demixing of a binary solvent containing such…

Soft Condensed Matter · Physics 2007-05-23 K. Stratford , R. Adhikari , I. Pagonabarraga , J. -C. Desplat , M. E. Cates

Deformable colloids and macromolecules adsorb at interfaces, as they decrease the interfacial energy between the two media. The deformability, or softness, of these particles plays a pivotal role in the properties of the interface. In this…

We study, using Monte Carlo simulations, the interaction between charged colloidal particles confined to the air-water interface. The dependence of force on ionic strength and counterion valence is explored. For 1:1 electrolyte, we find…

Soft Condensed Matter · Physics 2018-02-05 Matheus Girotto , Alexandre P. dos Santos , Yan Levin

Interfacial hydrodynamic slippage of water depends on both on surface chemistry and roughness. This study tries to connect the effect of chemical property and the physical structure of the surface on the interfacial slippage of water. By…

Fluid Dynamics · Physics 2016-05-10 Chinmay Anand Misra , Chirodeep Bakli

Liquids in contact with solids are submitted to intermolecular forces making liquids heterogeneous and stress tensors are not any more spherical as in homogeneous bulks. The aim of this article is to show that a square-gradient functional…

Classical Physics · Physics 2017-08-23 Henri Gouin

Within a general framework we study the effective, deformation-induced interaction between two colloids trapped at a fluid interface. As an application, we consider the interface deformation owing to the electrostatic field of charged…

Soft Condensed Matter · Physics 2007-05-23 Alvaro Dominguez , Martin Oettel , Siegfried Dietrich

We analyze the effective potential for nanoparticles trapped at a fluid interface within a simple model which incorporates surface and line tensions as well as a thermal average over interface fluctuations (capillary waves). For a single…

Soft Condensed Matter · Physics 2010-09-06 H. Lehle , M. Oettel

We investigate the equilibrium properties of a colloidal solution in contact with a soft interface. As a result of symmetry breaking, surface effects are generally prevailing in confined colloidal systems. In this Letter, particular…

Statistical Mechanics · Physics 2015-06-24 Hamid Kaidi , Thomas Bickel , Mabrouk Benhamou

A systematically designed study has been conducted to understand and clearly demarcate the degree of contribution by the constituting elements to the surface tension of nanocolloids. The effects of elements such as surfactants, particles…

Soft Condensed Matter · Physics 2016-10-20 A R Harikrishnan , Purbarun Dhar , PK Agnihotri , Sateesh Gedupudi , Sarit K Das

Surface roughness affects many properties of colloids, from depletion [1] and capillary interactions [2], to their dispersibility [3] and use as emulsion stabilizers [4]. It also impacts particle-particle frictional contacts, which have…

Soft Condensed Matter · Physics 2018-07-04 Chiao-Peng Hsu , Shivaprakash N. Ramakrishna , Michele Zanini , Nicholas D. Spencer , Lucio Isa

We report experimental and computational observations of dynamic contact networks for colloidal suspensions undergoing shear thickening. The dense suspensions are comprised of sterically stabilized poly(methyl methacrylate) hard sphere…

Soft Condensed Matter · Physics 2021-10-13 Shravan Pradeep , Mohamad Nabizadeh , Alan R. Jacob , Safa Jamali , Lilian C. Hsiao

Charged colloidal monolayers at the interface between water and air (or oil) are used in a large number of chemical, physical and biological applications. Although a considerable experimental and theoretical effort has been devoted in the…

Soft Condensed Matter · Physics 2018-12-03 Aviv Karnieli , Tomer Markovich , David Andelman

Reactions at solid-water interfaces play a foundational role in water treatment systems, catalysis, chemical separations, and in predicting chemical fate and transport in the environment. Over the last century, experimental measurements and…

Chemical Physics · Physics 2022-12-14 Anastasia G. Ilgen , Kevin Leung , Louise J. Criscenti , Jeffery A. Greathouse

We study the sliding of elastic solids in adhesive contact with flat and rough interfaces. We consider the dependence of the sliding friction on the elastic modulus of the solids. For elastically hard solids with planar surfaces with…

Soft Condensed Matter · Physics 2007-05-23 V. N. Samoilov , C. Yang , U. Tartaglino , B. N. J. Persson

It is proposed that lubricant molecules adsorbed on an interface between two asperities in contact, which is rough on the atomic scale, can switch the interface from the strong to weak pinning regime, resulting in a large reduction in the…

Materials Science · Physics 2007-05-23 J. B. Sokoloff

The influence of the external pressure and surface energy on the wetting transition at nanotextured interfaces is studied using molecular dynamics and continuum simulations. The surface roughness of the composite interface is introduced via…

Soft Condensed Matter · Physics 2018-07-12 Bishal Bhattarai , Nikolai V. Priezjev

Responsive poly-N-isopropylacrylamide-based microgels are commonly used as model colloids with soft repulsive interactions. It has been shown that the microgel-microgel interaction in solution can be easily adjusted by varying the…

Soft Condensed Matter · Physics 2021-09-06 Steffen Bochenek , Cathy E. McNamee , Michael Kappl , Hans Juergen Butt , Walter Richtering

The effect of surface roughness on the structure of liquid crystalline fluids near solid substrates is studied by Monte Carlo simulations. The liquid crystal is modelled as a fluid of soft ellipsoidal molecules and the substrate is modelled…

Soft Condensed Matter · Physics 2009-11-11 David Cheung , Friederike Schmid

We investigate the impact of nanoparticle roughness on the phase behaviour of suspensions in models of calcium carbonate nanoparticles. We use a Derjaguin approach that incorporates roughness effects and interactions between the…

Soft Condensed Matter · Physics 2020-05-12 Juan D. Olarte-Plata , Gøran Brekke-Svaland , Fernando Bresme

We consider the surface pressure of a colloid-laden liquid interface. As micron-sized particles of suitable wettability can be irreversibly bound to the liquid interface on experimental timescales, we use the canonical ensemble to derive an…

Soft Condensed Matter · Physics 2022-03-07 R. Mears , I. Muntz , J. H. J. Thijssen
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