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Related papers: Higher-order corrections to the spin-orbit and spi…

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We consider higher-order corrections to hyperfine coefficients related to the spin-orbit and spin-spin tensor interactions in hydrogen molecular ions. The $m\alpha^7 \ln(\alpha)$-order radiative correction is derived in the NRQED framework.…

Atomic Physics · Physics 2022-09-14 Mohammad Haidar , Vladimir I. Korobov , Laurent Hilico , Jean-Philippe Karr

The largest hyperfine interaction coefficients in the hydrogen molecular ion HD$^+$, i.e. the electron-proton and electron-deuteron spin-spin scalar interactions, are calculated with estimated uncertainties slightly below 1~ppm. The…

We report on progress in calculation of the spin-orbit interaction for the HD$^+$ molecular ion. This interaction is currently the largest source of theoretical uncertainty in determination of the hyperfine structure of rovibrational…

Atomic Physics · Physics 2022-11-09 Vladimir I. Korobov , Jean-Philippe Karr

A complete effective Hamiltonian for relativistic corrections at orders $m\alpha^6$ and $m\alpha^6(m/M)$ in a one-electron molecular system is derived from the NRQED Lagrangian. It includes spin-independent corrections to the energy levels…

Atomic Physics · Physics 2020-08-25 Vladimir Korobov , Jean-Philippe Karr , Mohammad Haidar , Zhen-Xiang Zhong

Precise numerical calculation of radiofrequency intervals between hyperfine sublevels of the $(37,35)$ state of the antiprotonic helium-4 atom is presented. Theoretical consideration includes the QED corrections of order $m\alpha^6$ to the…

Atomic Physics · Physics 2014-02-11 Vladimir I. Korobov , Zhen-Xiang Zhong

The relativistic second-order corrections at orders $m\alpha^6$ and $m\alpha^6(m/M)$ in hydrogen molecular ions are calculated. Convergence of numerical results is studied, which allows estimating the relative numerical uncertainty to be…

Atomic Physics · Physics 2025-06-30 Vladimir I. Korobov , Jean-Philippe Karr , Zhen-Xiang Zhong

High-precision variational calculations of the operators for the relativistic corrections in the leading $m\alpha^4$ order are presented. The ro-vibrational states in the range of the total orbital angular momentum $L\!=\!0\!-\!4$ and…

Atomic Physics · Physics 2019-01-09 D. T. Aznabayev , A. K. Bekbaev , V. I. Korobov

The major goal of the high-precision studies of ro-vibrational states in the hydrogen molecular ions is to provide an alternative way for improving the electron-to-proton mass ratio, or the atomic mass of electron. By now the complete set…

Atomic Physics · Physics 2008-04-16 V. I. Korobov

The m\alpha^6(m/M) order corrections to the hyperfine splitting in the H_2^+ ion are calculated. That allows to reduce uncertainty in the frequency intervals between hyperfine sublevels of a given rovibrational state to about 10 ppm.…

Atomic Physics · Physics 2009-05-12 V. I. Korobov , L. Hilico , J. -Ph. Karr

We investigate interactions between the proton spin, the deuteron spin, and the orbital angular momentum in the electronic ground state of the HD molecule. These interactions lead to hyperfine splittings of molecular energy levels. Our…

Chemical Physics · Physics 2020-07-29 Jacek Komasa , Mariusz Puchalski , Krzysztof Pachucki

We present a comprehensive analysis of all currently available high-accuracy frequency measurements of rotational and rovibrational transitions in the hydrogen molecular ion HD$^+$. Our analysis utilises the theoretically calculated…

Atomic Physics · Physics 2023-05-11 Jean-Philippe Karr , Jeroen C. J. Koelemeij

The complete second-order hyperfine-interaction correction is calculated for centroid energy levels of H, D, and $^3$He atoms. For $^3$He, the corrections of $-2.075$~kHz and $-0.305$~kHz beyond the leading hyperfine-mixing contribution are…

Atomic Physics · Physics 2024-12-10 Krzysztof Pachucki , Vojtěch Patkóš , Vladimir A. Yerokhin

We reconsider the calculation of rovibrational transition frequencies in hydrogen molecular ions. Some previously neglected contributions, such as the deuteron polarizability, are included into consideration in comparison with our previous…

Atomic Physics · Physics 2021-09-15 Vladimir I. Korobov , Jean-Philippe Karr

Expectation values of the Breit operators and the $Q$ terms are calculated for HD$^+$ with the vibrational number $v=0-4$ and the total angular momentum $L=0-4$. Relativistic and radiative corrections to some ro-vibrational transition…

Atomic Physics · Physics 2013-01-07 Zhen-Xiang Zhong , Pei-pei Zhang , Zong-Chao Yan , Ting-Yun Shi

The effective Hamiltonian of $m\alpha^6$ and $m\alpha^6(m/M)$ order corrections for hydrogen molecular ions has been derived in [ Z.-X. Zhong, \emph{et al.}, Phys. Rev. A {\bf98}, 032502(2018).], in this work we express the energy…

Atomic Physics · Physics 2026-03-17 Zhen-Xiang Zhong , Ping Yang , Vladimir I. Korobov , Chun Li , Ting-Yun Shi

The OH$^+$ ($X ^3\Sigma^-$) radical cation has been investigated by combining a 4 K 22-pole ion trap apparatus with high-resolution IR and THz radiation sources. Applying different types of action spectroscopic methods, the fundamental…

We revisit the $m \alpha^6 (m/M)$ order corrections to the hyperfine splitting in the H$_2^+$ ion, and find a hitherto unrecognized second-order relativistic contribution associated with the vibrational motion of the nuclei. Inclusion of…

The indirect nuclear spin-spin coupling tensor, $\mathbf J$, between mercury nuclei in Hg-containing systems can be of the order of few kHz and one of the largest measured. We conduct an analysis of the physics behind the electronic…

We present a nonrelativistic calculation of the rotation-vibration levels of the molecular ions H2+, D2+ and HD+, relying on the diagonalization of the exact three-body Hamiltonian. The J=2 levels are obtained with a very high accuracy of…

Quantum Physics · Physics 2017-02-20 Jean-Philippe Karr , Laurent Hilico

The static dipole polarizability for the hydrogen molecular ions H$_2^+$, HD$^+$, and D$_2^+$ are calculated. These new data for polarizability takes into account the leading order relativistic corrections to the wave function of the…

Atomic Physics · Physics 2017-02-01 D. T. Aznabayev , A. K Bekbaev , S. A. Zhaugasheva , V. I. Korobov
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