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For the large and chemically diverse GMTKN55 benchmark suite, we have studied the performance of density-corrected density functional theory (HF-DFT), compared to self-consistent DFT, for several pure and hybrid GGA and meta-GGA…

Chemical Physics · Physics 2021-03-29 Golokesh Santra , Jan M. L. Martin

We present the self-consistent implementation of current-dependent (hybrid) meta generalized gradient approximation (mGGA) density functionals using London atomic orbitals. A previously proposed generalized kinetic energy density is…

Dynamic Voltage and Frequency Scaling is essential for enhancing energy efficiency in mobile platforms. However, traditional heuristic-based governors are increasingly inadequate for managing the complexity of heterogeneous System-on-Chip…

Distributed, Parallel, and Cluster Computing · Computer Science 2025-09-30 Jinqi Yan , Fang He , Qianlong Sang , Bifeng Tong , Peng Sun , Yili Gong , Chuang Hu , Dazhao Cheng

For 6-DOF (degrees of freedom) interactive virtual acoustic environments (VAEs), the spatial rendering of diffuse late reverberation in addition to early (specular) reflections is important. In the interest of computational efficiency, the…

Audio and Speech Processing · Electrical Eng. & Systems 2021-11-30 Christoph Kirsch , Josef Poppitz , Torben Wendt , Steven van de Par , Stephan D. Ewert

In this work, we present the first derivation and implementation of analytic gradient methods for the computation of the atomic axial tensors (AATs) required for simulations of vibrational circular dichroism (VCD) spectra using…

Chemical Physics · Physics 2025-11-03 Brendan M. Shumberger , T. Daniel Crawford

The vdW-DF-cx0 exchange-correlation hybrid design has a truly nonlocal correlation component and aims to facilitate concurrent descriptions of both covalent and non-covalent molecular interactions. The vdW-DF-cx0 design mixes a fixed ratio,…

Chemical Physics · Physics 2018-06-13 Yang Jiao , Elsebeth Schröder , Per Hyldgaard

Stein Variational Gradient Descent (SVGD) is a widely used sampling algorithm that has been successfully applied in several areas of Machine Learning. SVGD operates by iteratively moving a set of interacting particles (which represent the…

Machine Learning · Computer Science 2024-06-24 Victor Priser , Pascal Bianchi , Adil Salim

The power spectrum and voxel intensity distribution (VID) are two summary statistics that can be applied to condense the information encoded in line-intensity maps. The information contained in both summary statistics is highly…

Cosmology and Nongalactic Astrophysics · Physics 2024-04-18 Vivian I. Sabla , José Luis Bernal , Gabriela Sato-Polito , Marc Kamionkowski

We assess the performance of nonempirical, truly nonlocal and semi-local functionals with regard to structural and thermal properties of $3d$, $4d$, and $5d$ non-magnetic transition metals. We focus on constraint-based functionals and…

Materials Science · Physics 2021-01-14 Leili Gharaee , Paul Erhart , Per Hyldgaard

The squared Brunt-V\"{a}is\"{a}l\"{a} Frequency (BVF) is computed in terms of the moist entropy potential temperature recently defined in Marquet (2011). Both homogeneously saturated and non-saturated versions of $N^2$ (the squared BVF) are…

Atmospheric and Oceanic Physics · Physics 2014-01-15 Pascal Marquet , Jean-François Geleyn

The van der Waals (vdW) density functional (vdW-DF) method [ROPP 78, 066501 (2015)] describes dispersion or vdW binding by tracking the effects of an electrodynamic coupling among pairs of electrons and their associated exchange-correlation…

Strongly Correlated Electrons · Physics 2018-02-21 Yang Jiao , Elsebeth Schröder , Per Hyldgaard

Since the development of the nonlocal correlation functional vdW-DF, the family of van der Waals density functionals has grown to better describe a wide variety of systems. A recent generation of the vdW-DF family, vdW-DF3, featured a…

Materials Science · Physics 2025-09-03 Trevor Jenkins , Kristian Berland , Timo Thonhauser

A simple and computationally efficient scheme to calculate approximate imaginary-frequency dependent polarizability, hence asymptotic van der Waals coefficient, within density functional theory is proposed. The dynamical dipolar…

Materials Science · Physics 2009-04-20 Huy-Viet Nguyen , Stefano de Gironcoli

The vibrational dynamics of adsorbate molecules in single-molecule junctions depend critically on the geometric structure and electronic interactions between molecule and substrate. Vibrations, excited mechanochemically or by external…

Mesoscale and Nanoscale Physics · Physics 2025-09-17 Lukas Hörmann , Reinhard J. Maurer

The fractional quantum Hall effect remains a captivating area in condensed matter physics, characterized by strongly correlated topological order, which manifests as fractionalized excitations and anyonic statistics. Numerical simulations,…

Strongly Correlated Electrons · Physics 2025-10-27 Yi Yang , Yayun Hu , Zi-Xiang Hu

The alternative separation of exchange and correlation energies proposed by Toulouse et al. [Theor. Chem. Acc. 114, 305 (2005)] is explored in the context of multi-configuration range-separated density-functional theory. The new…

Density functional calculations on atoms are often used for determining accurate initial guesses as well as generating various types of pseudopotential approximations and efficient atomic-orbital basis sets for polyatomic calculations. To…

Computational Physics · Physics 2023-10-30 Susi Lehtola

A two-parameter extension of the density-scaled double hybrid approach of Sharkas et al. [J. Chem. Phys. 134, 064113 (2011)] is presented. It is based on the explicit treatment of a fraction of multideterminantal exact exchange. The…

Chemical Physics · Physics 2012-01-12 Emmanuel Fromager

Long-range exchange and correlation effects, responsible for the failure of currently used approximate density functionals in describing van der Waals forces, are taken into account explicitly after a separation of the electron-electron…

Materials Science · Physics 2009-11-11 Janos G. Angyan , Iann C. Gerber , Andreas Savin , Julien Toulouse

We present a new video compression framework (ViSTRA2) which exploits adaptation of spatial resolution and effective bit depth, down-sampling these parameters at the encoder based on perceptual criteria, and up-sampling at the decoder using…

Image and Video Processing · Electrical Eng. & Systems 2021-06-22 Fan Zhang , Mariana Afonso , David R. Bull