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A fundamental issue that limits the efficiency of many photoelectrochemical systems is that the photon absorption length is typically much longer than the electron diffusion length. Various photon management schemes have been developed to…

Topological phase transitions in condensed matter systems have shown extremely rich physics, unveiling such exotic states of matter as topological insulators, superconductors and superfluids. Photonic topological systems open a whole new…

Conformational phases of a semiflexible off-lattice homopolymer model near an attractive substrate are investigated by means of multicanonical computer simulations. In our polymer-substrate model, nonbonded pairs of monomers as well as…

Computational Physics · Physics 2009-07-20 Monika Möddel , Michael Bachmann , Wolfhard Janke

The transport of charged particles or photons in a scattering medium can be modelled with a Boltzmann equation. The mathematical treatment for scattering in such scenarios is often simplified if evaluated in a frame where the scattering…

Plasma Physics · Physics 2024-02-27 Nils W. Schween , Brian Reville

A necessary first step in the development of technologies such as artificial photosynthesis is understanding the photoexcitation process within the basic building blocks of naturally-occurring light harvesting complexes (LHCs). The most…

Mesoscale and Nanoscale Physics · Physics 2019-07-30 María Rosa Preciado-Rivas , Duncan John Mowbray , Keenan Lyon , Ask Hjorth Larsen , Bruce Forbes Milne

Heterogeneous catalysis of adsorbates on metallic surfaces mediated by plasmon has potential high photoelectric conversion efficiency and controllable reaction selectivity. Theoretical modeling of dynamical reaction processes provides…

Chemical Physics · Physics 2023-06-05 Xiaoyan Wu , Tammo van der Heide , Thomas Frauenheim , Sergei Tretiak , ChiYung Yam , Yu Zhang

The use of eco-friendly materials for the environment has been addressed as a critical issue in the development of systems for renewable energy applications. In this regard, the investigation of organic photovoltaic (OPV) molecules for the…

Chemical Physics · Physics 2017-01-13 Alfredo Guillén-López , Miguel Robles , Jesús Muñiz

The Bruggeman formalism for the homogenization of particulate composite materials is used to predict the effective permittivity dyadic of a two-constituent composite material with one constituent having the ability to display the Pockels…

Optics · Physics 2009-11-13 Akhlesh Lakhtakia , Tom G. Mackay

Charged particle optics, the description of particle trajectories in the vicinity of some optical axis, describe the imaging properties of particle optics devices. Here, we present a complete and compact description of charged particle…

Optics · Physics 2021-06-16 Felix Kern , Jonas Krehl , Arsha Thampi , Axel Lubk

The recently suggested possibility that weak vibronic transitions can be excitonically enhanced in light-harvesting complexes is studied in detail. A vibronic exciton dimer model which includes ground state vibrations is investigated using…

Chemical Physics · Physics 2014-10-09 Jan Schulze , Magne Torbjörnsson , Oliver Kühn , Tõnu Pullerits

Topological photonics is a rapidly emerging field of research in which geometrical and topological ideas are exploited to design and control the behavior of light. Drawing inspiration from the discovery of the quantum Hall effects and…

The study of the formation of molecular hydrogen on low temperature surfaces is of interest both because it allows to explore elementary steps in the heterogeneous catalysis of a simple molecule and because of the applications in…

Chemical Physics · Physics 2008-11-21 G. Vidali , V. Pirronello , L. Li , J. Roser , G. Manico , R. Mehl , A. Lederhendler , H. B. Perets , J. R. Brucato , O. Biham

In this work, a novel ring polymer representation for multi-level quantum system is proposed for thermal average calculations. The proposed presentation keeps the discreteness of the electronic states: besides position and momentum, each…

Chemical Physics · Physics 2017-05-24 Jianfeng Lu , Zhennan Zhou

Controlling thin film formation is technologically challenging. The knowledge of physical properties of the film and of the atoms in the surface vicinity can help improve control over the film growth. We investigate the use of the…

In this paper we analyze how Transformation Optics recipes can be applied to control the flow of surface plasmons on metal-dielectric interfaces. We study in detail five different examples: a cylindrical cloak, a beam shifter, a right-angle…

We propose an 'automatic' approach to analyze the results of the on-the-fly trajectory surface hopping simulation on the multi-channel nonadiabatic photoisomerization dynamics by considering the trajectory similarity and the configuration…

Chemical Physics · Physics 2019-01-30 Xusong Li , Deping Hu , Yu Xie , Zhenggang Lan

Generally, the normal displacement-based formation control has a sensing mode that requires the agent not only to have certain knowledge of its direction, but also to gather its local information characterized by nonnegative coupling…

Optimization and Control · Mathematics 2023-06-06 Zhen Li , Yang Tang , Yongqing Fan , Tingwen Huang

With light-matter interaction extending into strong regime, as well as rapid development of laser technology, systems subjecting to a time-periodic perturbation are attracted broad attention. Floquet theorem and Floquet time-independent…

Quantum Physics · Physics 2023-09-25 Yu Wang , Vahid Mosallanejad , Wei Liu , Wenjie Dou

We propose a general theoretical description of chemical reactions occurring on a catalytic surface with heterogeneous reactivity. The propagator of a diffusion-reaction process with eventual absorption on the heterogeneous partially…

Chemical Physics · Physics 2019-11-05 Denis S. Grebenkov

We study theoretically the simultaneous, photo-induced two-particle excitations of strongly correlated systems on the basis of the Hubbard model. Under certain conditions specified in this work, the corre- sponding transition probability is…

Strongly Correlated Electrons · Physics 2015-05-18 B. D. Napitu , J. Berakdar