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Related papers: Spin-orbit interaction in the HD$^+$ ion

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Improved values of hyperfine coefficients related to the electronic spin-orbit and electron-nucleus spin-spin tensor interactions in the HD$^+$ molecular ion are obtained through numerical calculation of relativistic corrections at the…

Atomic Physics · Physics 2022-11-09 Mohammad Haidar , Vladimir I. Korobov , Laurent Hilico , Jean-Philippe Karr

We consider higher-order corrections to hyperfine coefficients related to the spin-orbit and spin-spin tensor interactions in hydrogen molecular ions. The $m\alpha^7 \ln(\alpha)$-order radiative correction is derived in the NRQED framework.…

Atomic Physics · Physics 2022-09-14 Mohammad Haidar , Vladimir I. Korobov , Laurent Hilico , Jean-Philippe Karr

The largest hyperfine interaction coefficients in the hydrogen molecular ion HD$^+$, i.e. the electron-proton and electron-deuteron spin-spin scalar interactions, are calculated with estimated uncertainties slightly below 1~ppm. The…

A complete effective Hamiltonian for relativistic corrections at orders $m\alpha^6$ and $m\alpha^6(m/M)$ in a one-electron molecular system is derived from the NRQED Lagrangian. It includes spin-independent corrections to the energy levels…

Atomic Physics · Physics 2020-08-25 Vladimir Korobov , Jean-Philippe Karr , Mohammad Haidar , Zhen-Xiang Zhong

Precise numerical calculation of radiofrequency intervals between hyperfine sublevels of the $(37,35)$ state of the antiprotonic helium-4 atom is presented. Theoretical consideration includes the QED corrections of order $m\alpha^6$ to the…

Atomic Physics · Physics 2014-02-11 Vladimir I. Korobov , Zhen-Xiang Zhong

The nuclear spin--rotation interaction in the hyperfine structure of the hydrogen molecular ion is investigated. The interaction constants are determined and are found to differ in sign and magnitude compared to another theory, but they are…

atom-ph · Physics 2008-02-03 James F. Babb

We present a comprehensive analysis of all currently available high-accuracy frequency measurements of rotational and rovibrational transitions in the hydrogen molecular ion HD$^+$. Our analysis utilises the theoretically calculated…

Atomic Physics · Physics 2023-05-11 Jean-Philippe Karr , Jeroen C. J. Koelemeij

We investigate interactions between the proton spin, the deuteron spin, and the orbital angular momentum in the electronic ground state of the HD molecule. These interactions lead to hyperfine splittings of molecular energy levels. Our…

Chemical Physics · Physics 2020-07-29 Jacek Komasa , Mariusz Puchalski , Krzysztof Pachucki

Theoretical investigations of the hyperfine structure of the hydrogen molecular ion (one electron and two protons) are discussed. The nuclear spin-rotation interaction has been found to be of the same sign as in the hydrogen molecule and…

Atomic Physics · Physics 2008-02-03 J. F. Babb

We present accurate ab initio and quantum scattering calculations on a prototypical hybrid ion-atom system Yb$^+$-Rb, recently suggested as a promising candidate for the experimental study of open quantum systems, quantum information…

Atomic Physics · Physics 2016-09-29 Timur V. Tscherbul , Paul Brumer , Alexei A. Buchachenko

We reconsider the calculation of rovibrational transition frequencies in hydrogen molecular ions. Some previously neglected contributions, such as the deuteron polarizability, are included into consideration in comparison with our previous…

Atomic Physics · Physics 2021-09-15 Vladimir I. Korobov , Jean-Philippe Karr

We derive a spin-orbital Hamiltonian for a triangular lattice of e_g orbital degenerate (Ni^{3+}) transition metal ions interacting via 90 degree superexchange involving (O^{2-}) anions, taking into account the on-site Coulomb interactions…

Strongly Correlated Electrons · Physics 2009-11-11 Albert J. W. Reitsma , Louis F. Feiner , Andrzej M. Oles'

High-precision variational calculations of the operators for the relativistic corrections in the leading $m\alpha^4$ order are presented. The ro-vibrational states in the range of the total orbital angular momentum $L\!=\!0\!-\!4$ and…

Atomic Physics · Physics 2019-01-09 D. T. Aznabayev , A. K. Bekbaev , V. I. Korobov

The magnetic dipole transitions in the homonuclear molecular ion H$_2^+$ are obtained for a wide range of $v$ and $L$, vibrational and total orbital momentum quantum numbers, respectively. Calculations are performed in the nonrelativistic…

Atomic Physics · Physics 2023-11-09 D. T. Aznabayev , A. K. Bekbaev , V. I. Korobov

The m\alpha^6(m/M) order corrections to the hyperfine splitting in the H_2^+ ion are calculated. That allows to reduce uncertainty in the frequency intervals between hyperfine sublevels of a given rovibrational state to about 10 ppm.…

Atomic Physics · Physics 2009-05-12 V. I. Korobov , L. Hilico , J. -Ph. Karr

The relativistic second-order corrections at orders $m\alpha^6$ and $m\alpha^6(m/M)$ in hydrogen molecular ions are calculated. Convergence of numerical results is studied, which allows estimating the relative numerical uncertainty to be…

Atomic Physics · Physics 2025-06-30 Vladimir I. Korobov , Jean-Philippe Karr , Zhen-Xiang Zhong

We revisit the $m \alpha^6 (m/M)$ order corrections to the hyperfine splitting in the H$_2^+$ ion, and find a hitherto unrecognized second-order relativistic contribution associated with the vibrational motion of the nuclei. Inclusion of…

The OH$^+$ ($X ^3\Sigma^-$) radical cation has been investigated by combining a 4 K 22-pole ion trap apparatus with high-resolution IR and THz radiation sources. Applying different types of action spectroscopic methods, the fundamental…

Spin-orbit coupling in crystals is known to lead to unusual direction dependent exchange interactions, however understanding of the consequeces of such effects in molecular crystals is incomplete. Here we perform four component relativistic…

Strongly Correlated Electrons · Physics 2017-04-19 A. C. Jacko , A. L. Khosla , J. Merino , B. J. Powell

We review recent experiments on HD$^+$ spectroscopy. The reduced proton-deuteron mass to electron mass ratio, $\mu_{pd}/m_e$, is inferred from the comparison of theory and experiment. Theoretical issues related to the calculations of the…

Atomic Physics · Physics 2022-09-07 Vladimir I. Korobov
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