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In semiconductors, exciton or charge carrier diffusivity is typically described as an inherent material property. Here, we show that the transport of excitons (i.e., bound electron-hole pairs) in CsPbBr3 perovskite nanocrystals (NCs)…

Exciton-phonon interactions govern the energy level spectrum and thus the optical response in semiconductors. In this respect, lead-halide perovskite nanocrystals represent a unique system, for which the interaction with optical phonons is…

We calculate the shift in emission frequency of the trion and biexciton (relative to that of the single exciton) for nanocrystals (NCs) of inorganic perovskites CsPbBr3 and CsPbI3. The calculations use an envelope-function k.p model…

Mesoscale and Nanoscale Physics · Physics 2020-03-26 T. P. T. Nguyen , S. A. Blundell , C. Guet

Layered halide perovskites are solution-processed natural heterostructures where quantum and dielectric confinement effects down to the nanoscale strongly influence the optical properties, leading to stabilization of bound excitons.…

Materials Science · Physics 2022-12-09 Claudio Quarti , Giacomo Giorgi , Claudine Katan , Jacky Even , Maurizia Palummo

Halide perovskite quantum dots exhibit cooperative optical phenomena that are absent in conventional semiconductor nanocrystals, including exciton superradiance, superabsorption, and biexciton superradiance within individual dots. Here we…

Optics · Physics 2026-02-25 Priya Nagpal , Patanjali Kambhampati

Advances in opto-electronics require the development of materials with novel and engineered characteristics. A class of materials that has garnered tremendous interest is metal-halide perovskites, stimulated by meteoric increases in…

Bose-Fermi systems such as mixtures of electrons with excitons or exciton-polaritons are extensively discussed as candidates to host a variety of intriguing phenomena, including polaron formation, drag effects, supersolidity, and…

Mesoscale and Nanoscale Physics · Physics 2023-08-09 Andrey S. Plyashechnik , Alexey A. Sokolik , Nina S. Voronova , Yurii E. Lozovik

We carry out a detailed theoretical study of the electronic and optical properties of bulk and monolayer bismuth triiodide (BiI$_{3}$), a layered metal halide, using the ab initio GW+BSE scheme with a full spinorial formulation. We discuss…

The correlation between the shift current mechanism for the bulk photovoltaic effect (BPVE) and the structural and electronic properties of ferroelectric perovskite oxides is not well understood. Here, we study and engineer the shift…

Materials Science · Physics 2015-03-03 Fenggong Wang , Steve M. Young , Fan Zheng , Ilya Grinberg , Andrew M. Rappe

To fully explore exciton-based applications and improve their performance, it is essential to understand the exciton behavior in anisotropic materials. Here, we investigate the optical properties of anisotropic excitons in GeS encapsulated…

All-inorganic halide perovskites have attracted a great interest as a promising light harvester of perovskite solar cells due to their enhanced chemical stability. In this work we investigate the material properties of solid solutions…

Materials Science · Physics 2020-04-22 Chol-Jun Yu , Un-Hyok Ko , Suk-Gyong Hwang , Yun-Sim Kim , Un-Gi Jong , Yun-Hyok Kye , Chol-Hyok Ri

A comprehensive study of excitonic properties of 2D layered perovskites is provided, with an emphasis on understanding and controlling the exciton fine structure. First, an overview of the optical properties is presented, discussing the…

We report a comprehensive first-principles study of the electronic and optical properties of recently identified exfoliable one-dimensional semiconducting materials, focusing on chalcogenide-based atomic chains derived from van der…

Topological polaritons, combining the robustness of the topological protected edge states to defects and disorder with the strong nonlinear properties of polariton bosons, represent an excellent platform to investigate novel photonic…

Mesoscale and Nanoscale Physics · Physics 2024-01-09 Jiahuan Ren , Teng Long , Chunling Gu , Hongbing Fu , Dmitry Solnyshkov , Guillaume Malpuech , Qing Liao

We report on the observation of spin dependent optically dressed states and optical Stark effect on an individual Mn spin in a semiconductor quantum dot. The vacuum-to-exciton or the exciton-to-biexciton transitions in a Mn-doped quantum…

Mesoscale and Nanoscale Physics · Physics 2012-06-18 C. Le Gall , A. Brunetti , H. Boukari , L. Besombes

For a neutral system of positive and negative charges, such as atoms in a crystal, increasing the density causes the Mott transition from bound electrons to free electrons. The density of optically generated electron-hole systems can be…

We study the dynamics of interacting superfluid bosons in a one dimensional vertical optical lattice after a sudden increase of the lattice potential depth. We show that this system can be exploited to investigate the effects of strong…

Quantum Gases · Physics 2014-05-23 K. W. Mahmud , L. Jiang , E. Tiesinga , P. R. Johnson

Halide double perovskites with alternating silver and pnictogen cations are an emerging family of photoabsorber materials with robust stability and band gaps in the visible range. However, the nature of optical excitations in these systems…

Materials Science · Physics 2021-02-12 Raisa-Ioana Biega , Marina R. Filip , Linn Leppert , Jeffrey B. Neaton

The tendency of identical bosons to bunch, seen in the Hanbury Brown-Twiss effect and Bose-Einstein condensation, is a hallmark of quantum statistics. This bunching can enhance the rates of fundamental processes such as atom-atom and…

Metal halide perovskites exhibit a materials physics that is distinct from traditional inorganic and organic semiconductors. While materials such as CH3NH3PbI3 are non-magnetic, the presence of heavy elements (Pb and I) in a…

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