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Nonlinear phononics relies on the resonant optical excitation of infrared-active lattice vibrations to coherently induce targeted structural deformations in solids. This form of dynamical crystal-structure design has been applied to control…

Applied Physics · Physics 2021-05-19 Meredith Henstridge , Michael Först , Edward Rowe , Michael Fechner , Andrea Cavalleri

The bulk photovoltaic effect (BPVE) refers to current generation due to illumination by light in a homogeneous bulk material lacking inversion symmetry. In addition to the intensively studied shift current, the ballistic current, which…

Materials Science · Physics 2021-05-05 Zhenbang Dai , Aaron M. Schankler , Lingyuan Gao , Liang Z. Tan , Andrew M. Rappe

Ultrafast photocurrent experiments are performed on semiconducting, single-walled carbon nanotubes under a resonant optical excitation of their subbands. The photogenerated excitons are dissociated at large electric fields and the resulting…

Mesoscale and Nanoscale Physics · Physics 2017-04-19 Christoph Karnetzky , Lukas Sponfeldner , Max Engl , Alexander W. Holleitner

The interplay between crystal symmetry and its optical responses is at the heart of tremendous recent advances in light-matter interactions and applications. Nonlinear optical processes that produce electric currents, for example bulk…

Materials Science · Physics 2021-10-27 Yongliang Shi , Jian Zhou

Photodetection is an indispensable function of optoelectronic devices in modern communication and sensing systems. Contrary to the near-infrared/visible regions, the fast and sensitive photodetectors operated at room temperature for the…

Ultrafast optical control of ferroelectricity using intense terahertz fields has attracted significant interest. Here we show that the nonlinear interactions between two optical phonons in SnTe, a two-dimensional in-plane ferroelectric…

Theory of the Linear photogalvanic effect is developed for direct optical transitions between surface states of three-dimensional topological insulators. The photocurrent governed by the orientation of the polarization plane of light and…

Mesoscale and Nanoscale Physics · Physics 2023-04-10 N. V. Leppenen , L. E. Golub

We report the optical excitation-dependent output photocurrent characteristics of GaN-based polariton diode lasers operated under reverse-bias at room temperature. The photocurrent demonstrates a non-linear enhancement at an incident…

Solid systems with strong correlations and interactions under light illumination have the potential for exhibiting interesting bulk photovoltaic behavior in the non-perturbative regime, which has remained largely unexplored in the past…

Strongly Correlated Electrons · Physics 2022-04-06 Sangeeta Rajpurohit , C. Das Pemmaraju , Tadashi Ogitsu , Liang Z Tan

Amplification of light through stimulated emission or nonlinear optical interactions has had a transformative impact on modern science and technology. The amplification of other bosonic excitations, like phonons in solids, is likely to open…

Materials Science · Physics 2022-06-01 Andrea Cartella , Tobia Federico Nova , Michael Fechner , Roberto Merlin , Andrea Cavalleri

Electronic transport in a model molecular device coupled to local phonon modes is theoretically analyzed. The method allows for obtaining an accurate approximation of the system's quantum state irrespective of the electron and phonon energy…

Mesoscale and Nanoscale Physics · Physics 2007-10-10 Antonino La Magna , Ioannis Deretzis

The bulk photovoltaic effect (BPVE) has attracted an increasing interest due to its potential to overcome the efficiency limit of traditional photovoltaics, and much effort has been devoted to understanding its underlying physics. However,…

Materials Science · Physics 2022-01-05 Zhenbang Dai , Andrew M. Rappe

We explore a novel coupling mechanism of electrons with the transverse optical (TO) phonon branch in a regime when the TO mode becomes highly anharmonic and drives the ferroelectric phase transition. We show that this anharmonicity, which…

Strongly Correlated Electrons · Physics 2020-03-04 P. Chudzinski

The correlation between the shift current mechanism for the bulk photovoltaic effect (BPVE) and the structural and electronic properties of ferroelectric perovskite oxides is not well understood. Here, we study and engineer the shift…

Materials Science · Physics 2015-03-03 Fenggong Wang , Steve M. Young , Fan Zheng , Ilya Grinberg , Andrew M. Rappe

Steady current in metals induces a thermal gradient, a phenomenon known as the Peltier effect. The Peltier effect is one of the fundamental phenomena in the thermoelectric properties of materials and is also used in applications such as…

Mesoscale and Nanoscale Physics · Physics 2024-08-15 Hiroaki Ishizuka , Masahiro Sato

We introduce a variational wave-function to study the polaron formation when the electronic transfer integral depends on the relative displacement between nearest-neighbor sites giving rise to a non-local electron-phonon coupling with…

Strongly Correlated Electrons · Physics 2009-11-10 C. A. Perroni , E. Piegari , M. Capone , V. Cataudella

Photogalvanic effect (PGE) occurring in noncentrosymmetric materials enables the generation of the open-circuit voltage that is much larger than the bandgap, making it rather attractive in solar cells. However, the magnitude of the PGE…

Applied Physics · Physics 2020-08-11 Juan Zhao , Yibin Hu , Yiqun Xie , Lei Zhang , Yin Wang

We report a comprehensive study of polarized infrared/terahertz photocurrents in bulk tellurium crystals. We observe different photocurrent contributions and show that, depending on the experimental conditions, they are caused by the…

Mesoscale and Nanoscale Physics · Physics 2023-12-07 M. D. Moldavskaya , L. E. Golub , S. N. Danilov , V. V. Bel'kov , D. Weiss , S. D. Ganichev

Nonlinear phononics provides a route to control crystal structures through light-induced phonon excitation. In this study, we apply nonlinear phononics to an iron-based superconductor, LaFeAsO, with the aim of tuning its crystal structure…

Superconductivity · Physics 2026-04-09 Shu Kamiyama , Tatsuya Kaneko , Kazuhiko Kuroki , Masayuki Ochi

Nonlinear phononics play important role in strong laser-solid interactions. We discuss nonlinear dynamical protocols which allow for efficient excitation and control of nonlinear phonons. We consider recent inspiring proposals: inducing…

Other Condensed Matter · Physics 2018-05-16 A. P. Itin , M. I. Katsnelson
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