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Enormous enhancement in the viscosity of a liquid near its glass transition is generally connected to the growing many-body static correlations near the transition, often coined as `amorphous ordering'. Estimating the length scales of such…

For thin films of superfluid adsorbed on a disordered substrate, we derive the equation of motion for a vortex in the presence of a random potential within a mean field (Hartree) description of the condensate. The compressible nature of the…

Statistical Mechanics · Physics 2009-10-31 H. H. Lee , J. M. F. Gunn

We study supercooled dynamics in quantum hard-sphere liquid using quantum mode-coupling formulation. In the moderate quantum regime, classical cage effects lead to slower dynamics compared to strongly quantum regime, where tunneling…

Statistical Mechanics · Physics 2021-02-03 Ankita Das , Eran Rabani , Kunimasa Miyazaki , Upendra Harbola

The properties of nanoconfined fluids can be strikingly different from those of bulk liquids. A basic unanswered question is whether the equilibrium and dynamic consequences of confinement are related to each other in a simple way. We study…

Soft Condensed Matter · Physics 2013-12-17 Trond S. Ingebrigtsen , Jeffrey R. Errington , Thomas M. Truskett , Jeppe C. Dyre

In this article we study in detail the Q-vector dependence of the collective dynamics in simulated deeply supercooled SPC/E water. The evolution of the system has been followed for 250 ns at low T, allowing a clear identification of a two…

Soft Condensed Matter · Physics 2009-10-30 Francesco Sciortino , Linda Fabbian , Sow-Hsin Chen , Piero Tartaglia

Low Reynolds number direct simulations of large populations of hydrodynamically interacting swimming particles confined between planar walls are performed. The results of simulations are compared with a theory that describes dilute…

Fluid Dynamics · Physics 2015-05-13 Juan P. Hernandez-Ortiz , Patrick T. Underhill , Michael D. Graham

We theoretically study the effect of external deformation on activated structural relaxation and elementary aspects of the nonlinear mechanical response of glassy hard sphere fluids in the context of the nonequilibrium version of the…

Soft Condensed Matter · Physics 2021-02-03 Ashesh Ghosh , Kenneth S. Schweizer

A possible role of quantum effects, such as tunneling and zero-point energy, in the structural dynamics of supercooled liquids is studied by dielectric spectroscopy. Presented results demonstrate that the liquids, bulk 3-methylpentane 3MP…

Soft Condensed Matter · Physics 2017-01-04 A. Agapov , V. N. Novikov , A. Kisliuk , R. Richert , A. P. Sokolov

Pinning particles at the equilibrium configuration of the liquid is expected not to affect the structure and any property that depends on the structure while slowing down the dynamics. This leads to a breakdown of the structure dynamics…

Chemical Physics · Physics 2024-04-24 Palak Patel , Sarika Maitra Bhattacharyya

We generalize the force-level Nonlinear Langevin Equation theory of single particle hopping to include collective effects associated with long range elastic distortion of the liquid. The activated alpha relaxation event is of a mixed…

Disordered Systems and Neural Networks · Physics 2015-06-18 Stephen Mirigian , Kenneth S. Schweizer

We use molecular dynamics computer simulations to investigate the relaxation dynamics of a binary Lennard-Jones liquid confined in a narrow pore. We find that the average dynamics is strongly influenced by the confinement in that time…

Statistical Mechanics · Physics 2009-10-31 Peter Scheidler , Walter Kob , Kurt Binder

We study numerically the crystallization of a hard-sphere mixture with 8\% polydispersity. Although often used as a model glass former, for small system sizes we observe crystallization in molecular dynamics simulations. This opens the…

Soft Condensed Matter · Physics 2016-09-05 Matteo Campo , Thomas Speck

One of the hallmarks of molecular dynamics in deeply supercooled liquids is the non-exponential character of the relaxation functions. It has been a long standing issue if 'universal' features govern the lineshape of glassy dynamics…

We present a quantitative theory for a relaxation function in a simple glass-forming model (binary mixture of particles with different interaction parameters). It is shown that the slowing down is caused by the competition between locally…

Materials Science · Physics 2009-11-13 Edan Lerner , Itamar Procaccia

When an ensemble of particles interact hydrodynamically, they generically display large-scale transient structures such as swirls in sedimenting particles [1], or colloidal strings in sheared suspensions [2]. Understanding these…

Soft Condensed Matter · Physics 2013-01-24 Nicolas Desreumaux , Jean-Baptiste Caussin , Raphael Jeanneret , Eric Lauga , Denis Bartolo

Structural alpha relaxation in liquid orthoterphenyl is studied by means of coherent neutron time-of-flight and backscattering spectroscopy over a large temperature range. Not only amplitude and relaxation time but also the spectral line…

Statistical Mechanics · Physics 2011-04-05 A. Toelle , H. Schober , J. Wuttke , F. Fujara

In this paper, we consider some aspects of the physics of the partly pinned (PP) systems obtained by freezing in place particles in equilibrium bulk fluid configurations in the normal (nonglassy) state. We first discuss the configurational…

Disordered Systems and Neural Networks · Physics 2014-09-11 Vincent Krakoviack

We formulate a microscopic, no adjustable parameter, theory of activated relaxation in supercooled liquids directly in terms of the repulsive and attractive forces within the framework of pair correlations. Under isochoric conditions,…

Statistical Mechanics · Physics 2016-07-18 Zachary E. Dell , Kenneth S. Schweizer

An accurate prediction of the translational and rotational motion of particles suspended in a fluid is only possible if a complete set of correlations for the force coefficients of fluid-particle interaction is known. The present study is…

Fluid Dynamics · Physics 2020-09-24 Martyna Minakowska , Thomas Richter , Sebastian Sager

Motivated by a number of recent experimental and computational studies of the dynamics of fluids plunged in quenched-disordered external fields, we report on a theoretical investigation of this topic within the framework of the…

Soft Condensed Matter · Physics 2018-10-05 Thomas Konincks , Vincent Krakoviack