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We present a theoretical framework to describe polarons from first principles within a many-body Green's function formalism. Starting from a general electron-phonon Hamiltonian, we derive a self-consistent Dyson equation in which the…

The Allen-Heine-Cardona theory allows us to calculate phonon-induced electron self-energies from first principles without resorting to the adiabatic approximation. However, this theory has not been able to account for the change of the…

Materials Science · Physics 2024-10-17 Jae-Mo Lihm , Cheol-Hwan Park

The electronic structure of condensed matter can be significantly affected by the electron-phonon interaction, leading to important phenomena such as electrical resistance, superconductivity or the formation of polarons. This interaction is…

We develop a theoretical and computational framework to study polarons in semiconductors and insulators from first principles. Our approach provides the formation energy, excitation energy, and wavefunction of both electron and hole…

Materials Science · Physics 2019-06-21 Weng Hong Sio , Carla Verdi , Samuel Ponce , Feliciano Giustino

The single-polaron band structure of the Holstein model in one and two dimensions is studied using a new form of resummed strong-coupling perturbation theory. Well converged results are obtained for phonon frequencies of the order of the…

Condensed Matter · Physics 2007-05-23 Walter Stephan

The renormalization of electronic eigenenergies due to electron-phonon coupling is sizable in many materials with light atoms. This effect, often neglected in ab-initio calculations, can be computed using the perturbation-based…

We develop a theory for the electron-phonon interaction effects on the electronic properties of graphene. We analytically calculate the electron self-energy, spectral function and band velocity renormalization due to phonon-mediated…

Materials Science · Physics 2009-11-13 Wang-Kong Tse , S. Das Sarma

We present a theory of electronic excitation energies and optical absorption spectra which incorporates energy-level renormalization and phonon-assisted optical absorption within a unified framework. Using time-independent perturbation…

Materials Science · Physics 2016-07-28 Christopher E. Patrick , Feliciano Giustino

We investigate the spinless Anderson-Holstein model routinely employed to describe the basic physics of phonon-assisted tunneling in molecular devices. Our focus is on small to intermediate electron-phonon coupling; we complement a recent…

Strongly Correlated Electrons · Physics 2017-11-30 A. Khedri , T. A. Costi , V. Meden

In compound semiconductors and insulators, the polar electron-phonon coupling diverges at long range, known as the Fr\"ohlich interaction. Modern first-principles electron-phonon calculations treat the Fr\"ohlich interaction in a…

\ni We develop a simple method to study the zero-point and thermally renormalized electron energy $\varepsilon_{\mathbf{k}n}(T)$ for $\mathbf{k}n$ the conduction band minimum or valence maximum in polar semiconductors. We use the adiabatic…

Materials Science · Physics 2016-09-21 Jean Paul Nery , Philip B. Allen

Starting from recent advances in the first-principles modeling of polarons, variational polaron equations in the strong-coupling adiabatic approximation are formulated in Bloch space. In this framework, polaron formation energy as well as…

Materials Science · Physics 2022-06-09 Vasilii Vasilchenko , Andriy Zhugayevych , Xavier Gonze

Partial summing of infinite range of diagrams for the two-phonon mass operator of polaron described by Fr\"{o}hlich Hamiltonian is performed using the Feynman-Pines diagram technique. Renormalized spectral parameters of ground and first…

Mesoscale and Nanoscale Physics · Physics 2015-10-26 M. V. Tkach , Ju. O. Seti , O. M. Voitsekhivska , O. Yu. Pytiuk

We present a novel approach to electron-lattice interaction beyond the linear-coupling regime. Based on the solution of a Holstein-Peierls-type model, we derive explicit analytical expressions for the eigenvalue spectrum of the Hamiltonian,…

Materials Science · Physics 2018-12-13 Pablo García Risueño , Dmitrii Nabok , Qiang Fu , Claudia Draxl

Path-integral approach to the tight-binding polaron is extended to multiple optical phonon modes of arbitrary dispersion and polarization. The non-linear lattice effects are neglected. Only one electron band is considered. The…

Strongly Correlated Electrons · Physics 2009-11-11 Pavel Kornilovitch

An impurity immersed in a Bose-Einstein condensate is no longer accurately described by the Fr\"ohlich Hamiltonian as the coupling between the impurity and the boson bath gets stronger. We study the dominant effects of the two-phonon terms…

Quantum Gases · Physics 2019-10-28 Timour Ichmoukhamedov , Jacques Tempere

A new method for calculation of band structure has been proposed based on the Green's function theory and local sampling. Potential energy in the Hamiltonian of Schrodinger's equation is approximated with a series of sampled Dirac delta…

Mesoscale and Nanoscale Physics · Physics 2010-02-24 Milad Khoshnegar , Sina Khorasani , Amirhossein Hosseinnia

We present a novel, highly efficient yet accurate analytical approximation for the Green's function of a Holstein polaron. It is obtained by summing all the self-energy diagrams, but with each self-energy diagram averaged over the momenta…

Strongly Correlated Electrons · Physics 2009-11-11 Glen L. Goodvin , Mona Berciu , George A. Sawatzky

The description of an impurity atom in a Bose-Einstein condensate can be cast in the form of Frohlich's polaron Hamiltonian, where the Bogoliubov excitations play the role of the phonons. An expression for the corresponding polaronic…

Quantum Gases · Physics 2014-03-26 J. Tempere , W. Casteels , M. K. Oberthaler , E. Timmermans , J. T. Devreese

The Fr\"ohlich model describes the interaction of a mobile impurity with a surrounding bath of phonons which leads to the formation of a quasiparticle, the polaron. In this article an efficient renormalization group approach is presented…

Quantum Gases · Physics 2016-04-27 Fabian Grusdt
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