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We analyze fermionic entanglement and correlation measures in the ground and the low temperature thermal state of the water molecule as a function of the internuclear distance in the context of the full configuration interaction approach.…

Quantum Physics · Physics 2026-04-10 J. Garcia , J. A. Cianciulli , R. Rossignoli

Practical measures of electronic decoherence, called distilled purities, that are applicable to many-body systems are introduced. While usual measures of electronic decoherence such as the purity employ the full $N$-particle density matrix…

Quantum Physics · Physics 2017-06-07 Arnab Kar , Ignacio Franco

We present a quantum Monte Carlo method capable of sampling the full density matrix of a many-particle system at finite temperature. This allows arbitrary reduced density matrix elements and expectation values of complicated non-local…

Computational Physics · Physics 2015-06-15 N. S. Blunt , T. W. Rogers , J. S. Spencer , W. M. C. Foulkes

At present, there are many methods of quantum entanglement of particles with an electromagnetic field. Most methods have a low probability of quantum entanglement and not an exact theoretical apparatus based on an approximate solution of…

Quantum Physics · Physics 2017-09-15 Dmitry Makarov

Properties that are necessarily formulated within pure (symmetric) expectation values are difficult to calculate for projector quantum Monte Carlo approaches, but are critical in order to compute many of the important observable properties…

Computational Physics · Physics 2015-06-23 Catherine Overy , George H. Booth , N. S. Blunt , James Shepherd , Deidre Cleland , Ali Alavi

The exact study of small systems can guide us toward measures for extracting information about many-body physics as we move to more complex systems capable of quantum information processing or quantum analog simulation. We use exact…

Mesoscale and Nanoscale Physics · Physics 2021-06-10 Emily Townsend , Tomáš Neuman , Alex Debrecht , Javier Aizpurua , Garnett W. Bryant

Reduced density-matrix functional theory (RDMFT) is a promising alternative approach to the problem of electron correlation. Like standard density functional theory, it contains an unknown exchange-correlation functional, for which several…

Chemical Physics · Physics 2017-03-03 N. N. Lathiotakis , Miguel A. L. Marques

In electronic structure calculations, the correlation energy is defined as the difference between the mean field and the exact solution of the non relativistic Schr\"odinger equation. Such an error in the different calculations is not…

Quantum Physics · Physics 2022-04-04 Kumar J. B. Ghosh , Sabre Kais , Dudley R. Herschbach

Studies of one-body density matrices (ODM) are performed in various correlation methods, such as the Jastrow method, the correlated basis function method, the Green's function method and the generator coordinate method aiming to extract the…

Nuclear Theory · Physics 2007-05-23 A. N. Antonov , M. K. Gaidarov , M. V. Ivanov , K. A. Pavlova , C. Giusti

The many-body Coulomb repulsive energy of strictly correlated electrons provides direct information of the exact Hohenberg-Kohn exchange-correlation functional in the strong interaction limit. Until now the treatment of strictly correlated…

Chemical Physics · Physics 2013-03-13 Christian B. Mendl , Lin Lin

A quantum mechanical system of two coupled rotors (particles constrained to move on a circle) is studied from an open quantum systems point of view. One of the rotors is integrated out and the reduced density operator of the other rotor is…

Quantum Physics · Physics 2025-05-21 V V Sreedhar , Ankit Yadav

The Bures-Hall distance metric between quantum states is a unique measure that satisfies various useful properties for quantum information processing. In this work, we study the statistical behavior of quantum entanglement over the…

Mathematical Physics · Physics 2021-01-04 Lu Wei

We present a measurement-cost efficient implementation of Strongly-Contracted $N$-Electron Valence Perturbation Theory (SC-NEVPT2) for use on near-term quantum devices. At the heart of our algorithm we exploit the properties of adaptive…

Quantum Physics · Physics 2024-05-27 Aaron Fitzpatrick , N. Walter Talarico , Roberto Di Remigio Eikås , Stefan Knecht

Ab initio calculations play an essential role in our fundamental understanding of quantum many-body systems across many subfields, from strongly correlated fermions to quantum chemistry and from atomic and molecular systems to nuclear…

We investigate the efficiency of the recently proposed Restricted Boltzmann Machine (RBM) representation of quantum many-body states to study both the static properties and quantum spin dynamics in the two-dimensional Heisenberg model on a…

Strongly Correlated Electrons · Physics 2019-07-10 G. Fabiani , J. H. Mentink

In this paper we propose an ab initio method to solve quantum many-body problems of molecular dynamics where both the electronic and the nuclear degrees are represented by ensembles of trajectories and guiding waves in physical space. Both…

Atomic Physics · Physics 2025-01-28 Ivan P. Christov

We investigate the accuracy and efficiency of the semiclassical Frozen Gaussian method in describing electron dynamics in real time. Model systems of two soft-Coulomb-interacting electrons are used to study correlated dynamics under…

Chemical Physics · Physics 2015-05-30 Peter Elliott , Neepa T. Maitra

Operationally accessible entanglement in bipartite systems of indistinguishable particles could be reduced due to restrictions on the allowed local operations as a result of particle number conservation. In order to quantify this effect,…

Quantum Gases · Physics 2018-10-17 Hatem Barghathi , C. M. Herdman , Adrian Del Maestro

We present and motivate an efficient way to include orbital dependent many--body correlations in trial wave function of real--space Quantum Monte Carlo methods for use in electronic structure calculations. We apply our new…

Computational Physics · Physics 2019-10-17 Markus Holzmann , Saverio Moroni

Entanglement entropy encodes important features of strongly interacting quantum many-body systems and gauge theories, but its analytical study is still limited to systems with high level of symmetry. This motivates the search for efficient…

High Energy Physics - Lattice · Physics 2023-09-28 Andrea Bulgarelli , Marco Panero