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Collective motion over increasing length scales is a signature of the vitrification process of liquids. We demonstrate the emergence of distinct static and dynamic length scales probed near the free surface in fully equilibrated…

Statistical Mechanics · Physics 2022-11-28 Hailong Peng , Huashan Liu , Thomas Voigtmann

The high frequency collective dynamics of liquid hydrogen fluoride is studied by inelastic x-ray scattering on the coexistence curve at T = 239 K. The comparison with existing molecular dynamics simulations shows the existence of two active…

Soft Condensed Matter · Physics 2023-08-29 R. Angelini , P. Giura , G. Monaco , G. Ruocco , F. Sette , R. Verbeni

Within the macroscopic Landau-de Gennes approach, we examine the Gaussian normal mode fluctuations of semi-infinite nematic liquid crystals in a regime of critical wetting. It is argued that surface free-energy potentials that strongly…

Soft Condensed Matter · Physics 2009-10-31 N. B. Ivanov

I use the method of classical density-functional theory in the weighted-density approximation of Tarazona to investigate the phase diagram and the interface structure of a two-dimensional lattice-gas model with three phases -- vapour,…

Statistical Mechanics · Physics 2009-11-10 S. Prestipino

When captured by a flat nematic-isotropic interface, colloidal particles can be dragged by it. As a result spatially periodic structures may appear, with the period depending on a particle mass, size, and interface…

Soft Condensed Matter · Physics 2009-11-11 J. L. West , K. Zhang , A. Glushchenko , D. Andrienko , M. Tasinkevych , Y. Reznikov

In this work, a mathematical model based on interface energy is proposed within the framework of surface continuum mechanics to study the dynamics of encapsulated bubbles. The interface model naturally induces a residual stress field into…

Fluid Dynamics · Physics 2023-06-22 Nehal Dash , Ganesh Tamadapu

The growing trend towards engineering interfacial complexion (or phase) transitions has been seen in the grain boundary and solid surface systems.Meanwhile, little attention has been paid to the chemically heterogeneous solid/liquid…

Materials Science · Physics 2023-05-10 Jiaojiao Liu , Hongtao Liang , Jinfu Li , Brian B. Laird , and Yang Y

Hypothesis: The collective dynamics and self-assembly of colloids floating at a fluid/fluid interface is a balance between deterministic lateral interaction forces, viscous resistance to colloid motion along the surface and thermal…

Soft Condensed Matter · Physics 2022-10-05 Archit Dani , Mohsen Yeganeh , Charles Maldarelli

There is mounting evidence indicating that relaxation dynamics in liquids approaching their glass transition not only becomes increasingly cooperative (1,2) but the relaxing regions also become more compact in shape(3-7). While the surface…

Statistical Mechanics · Physics 2018-02-21 Divya Ganapathi , Hima K Nagamanasa , A. K. Sood , Rajesh Ganapathy

We analyze from a far field the evolution of an interface that separates ideal incompressible fluids of different densities and has an interfacial mass flux. We develop and apply the general matrix method to rigorously solve the boundary…

Liquid-gas phase coexistence in a boundary-driven diffusive system is studied by analyzing fluctuating hydrodynamics of a density field defined on a one-dimensional lattice with a space interval $\Lambda$. When an interface width $\ell$ is…

Statistical Mechanics · Physics 2024-11-28 Shin-ichi Sasa , Naoko Nakagawa

Family of compounds CBr$_n$Cl$_{4-n}$ has been proven helpful in unraveling microscopic mechanisms responsible of glassy behavior. Some of the family members show translational ordered phases with minimal disorder which appears to reveal…

Soft Condensed Matter · Physics 2017-11-21 Nirvana B. Caballero , Mariano Zuriaga , Josep Lluis Tamarit , Pablo Serra

The rapid solidification of a binary mixture in the region of the interface velocities $V$ close to the diffusion speed in the bulk of the liquid phase $V_D$ is considered within the framework of the local nonequilibrium approach. In this…

Materials Science · Physics 2021-07-12 G. L. Buchbinder

Controlling polymorphism in molecular crystals is crucial in the pharmaceutical, dye, and pesticide industries. However, its theoretical description is extremely challenging, due to the associated long timescales ($ > 1 \, \mu s$). We…

Chemical Physics · Physics 2023-02-09 Oren Elishav , Roy Podgaetsky , Olga Meikler , Barak Hirshberg

The properties of the interface between solid and melt are key to solidification and melting, as the interfacial free energy introduces a kinetic barrier to phase transitions. This makes solidification happen below the melting temperature,…

Statistical Mechanics · Physics 2015-12-02 Bingqing Cheng , Gareth A. Tribello , Michele Ceriotti

Hypothesis: Diffusion in confinement is an important fundamental problem with significant implications for applications of supported liquid phases. However, resolving the spatially dependent diffusion coefficient, parallel and perpendicular…

This article covers thermodynamic, dynamic, and kinetic models that are suitable for the analysis of wetting, adsorption, and related interfacial phenomena in colloidal and multiphase systems. Particular emphasis is made on describing…

Soft Condensed Matter · Physics 2025-09-03 Carlos E. Colosqui

We investigate the zero-temperature properties of a dilute two-component Fermi gas with attractive interspecies interaction in the BCS-BEC crossover. We build an efficient parametrization of the energy per particle based on Monte Carlo data…

Soft Condensed Matter · Physics 2009-11-10 N. Manini , L. Salasnich

We calculate the spectrum of low-lying collective excitations in a mesoscopic cloud formed by a Bose-Einstein condensate and a spin-polarized Fermi gas as a function of the boson-fermion repulsions. The cloud is under isotropic harmonic…

Condensed Matter · Physics 2016-08-31 P. Capuzzi , A. Minguzzi , M. P. Tosi

We present a complete analysis of the dynamics of a Bose-Einstein condensate trapped in a symmetric triple-well potential. Our classical analogue treatment, based on a time-dependent variational method using SU(3) coherent states, includes…

Quantum Physics · Physics 2011-04-01 T. F. Viscondi , K. Furuya