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We study the self-assembly of colloidal microgel particles at a quasi-two-dimensional air-water interface of a drying droplet. Using bright-field microscopy, we demonstrate that increasing particle elasticity drives interfacial organization…

Soft Condensed Matter · Physics 2026-03-10 Vaibhav Raj Singh Parmar , Sayantan Chanda , Rituparno Mandal , Ranjini Bandyopadhyay

We consider gelation of colloidal particles in suspension after cessation of shear flow. Particle aggregation is driven by a temperature-tunable attractive potential which controls the growth of clusters under isothermal conditions. A…

Soft Condensed Matter · Physics 2014-02-03 Ajay Singh Negi , Carissa G. Redmon , Subramanian Ramakrishnan , Chinedum O. Osuji

We numerically study a simple model for thermo-reversible colloidal gelation in which particles can form reversible bonds with a predefined maximum number of neighbors. We focus on three and four maximally coordinated particles, since in…

We present dynamic light scattering (DLS) measurements of soft polymethyl-methacrylate (PMMA) and polyacrylamide(PA) polymer gels prepared with trapped bodies (latex spheres or maghemite nanoparticles). We show that the anomalous…

Soft Condensed Matter · Physics 2015-06-10 Alvaro V. N. C. Teixeira , Erik Geissler , Pedro Licinio

Shear flow is known to induce huge density fluctuations in otherwise clear and uniform polymer solutions. This effect is rooted in the elasticity of the entangled polymer network, and can span distances over a thousand chains wide. It has…

Computational Physics · Physics 2018-08-21 Airidas Korolkovas

Restricting the number of attractive physical "bonds" that can form between particles in a fluid suppresses the usual demixing phase transition to very low particle concentrations, allowing for the formation of open, percolated, and…

Soft Condensed Matter · Physics 2016-08-25 Beth A. Lindquist , Ryan B. Jadrich , Delia J. Milliron , Thomas M. Truskett

The swelling kinetics of charged polymer gels reflect the complex competition among elastic, mixing, and ionic contributions. Here, we used dynamic light scattering to investigate the collective diffusion coefficient of model gels, whose…

Soft Condensed Matter · Physics 2024-02-01 Shoei Sano , Takashi Yasuda , Takeshi Fujiyabu , Naoyuki Sakumichi , Takamasa Sakai

We derive the elastic field generated by multiple small-scaled inclusions distributed in a bounded set of $\mathbb{R}^3$. These inclusions are modeled with moderate values of the Lam\'e coefficients while they have a large relative mass…

Analysis of PDEs · Mathematics 2024-05-10 Durga Prasad Challa , Divya Gangadaraiah , Mourad Sini

Solutions of polymer chains are modelled using non-equilibrium Brownian dynamics simulations, with physically associative beads which form reversible crosslinks to establish a system-spanning physical gel network. Rheological properties…

Soft Condensed Matter · Physics 2024-06-19 Dominic Robe , Aritra Santra , Gareth H. McKinley , J. Ravi Prakash

The dynamics of flexible polymer molecules are often assumed to be governed by hydrodynamics of the solvent. However there is considerable evidence that internal dissipation of a polymer contributes as well. Here we investigate the dynamics…

Soft Condensed Matter · Physics 2013-05-29 J. M. Deutsch

Suspensions of colloidal microplates in contoured 2D elastic fluids sheets are dominated by the bending mechanics and shear rigidity of the plates and the contrasting in-plane shear flow of the 2D fluid. Using the phase separated…

Applied Physics · Physics 2024-02-26 Weiyue Xin , Maria M. Santore

We examine the dynamics of two-dimensional colloidal systems using numerical simulations of a system with a drive applied to a thin region in the middle of the sample to produce a local shear. For a monodisperse colloidal assembly, we find…

Soft Condensed Matter · Physics 2015-06-11 A. Libal , B. M. Csiki , C. J. Olson Reichhardt , C. Reichhardt

Gels are used to design bilayered structures with high residual stresses. The swelling of a thin layer on a compliant substrate leads to compressive stresses. The post-buckling of this layer is investigated experimentally; the wavelengths…

Soft Condensed Matter · Physics 2015-06-25 Eric Sultan , Arezki Boudaoud

Colloidal molecules are designed to mimic their molecular analogues through their anisotropic shape and interactions. However, current experimental realizations are missing the structural flexibility present in real molecules thereby…

Cellulose nanocrystals (CNC) are naturally-derived nanostructures of growing importance for the production of composites having attractive mechanical properties, and offer improved sustainability over purely petroleum-based alternatives.…

Soft Condensed Matter · Physics 2019-01-15 Abhinav Rao , Thibaut Divoux , Gareth H. McKinley , A. John Hart

Molecular clouds (MCs) are stellar nurseries, however, formation of stars within MCs depends on the ambient physical conditions. MCs, over a free-fall time are exposed to numerous dynamical phenomena, of which, the interaction with a thin,…

Astrophysics of Galaxies · Physics 2015-05-20 S. Anathpindika , H. C. Bhatt

Mesoscale behavior of polymers is frequently described by universal laws. This physical property motivates us to propose a new modeling concept, grouping polymers into classes with a common long-wavelength representation. In the same class…

Soft Condensed Matter · Physics 2016-10-25 Guojie Zhang , Torsten Stuehn , Kostas Ch. Daoulas , Kurt Kremer

We present a multichannel model for elastic interactions, comprised of an arbitrary number of coupled finite square-well potentials, and derive semi-analytic solutions for its scattering behavior. Despite the model's simplicity, it is…

Atomic Physics · Physics 2018-12-11 Nirav P. Mehta , Kaden R. A. Hazzard , Christopher Ticknor

The behavior of particles driven through a narrow constriction is investigated in experiment and simulation. The system of particles adapts to the confining potentials and the interaction energies by a self-consistent arrangement of the…

Soft Condensed Matter · Physics 2008-10-15 P. Henseler , A. Erbe , M. Köppl , P. Leiderer , P. Nielaba

Despite intense research, methods for controlling soft matter's spontaneous self-assembly in-to well-defined layers remain a significant challenge. We observed ion-induced structural disconti-nuities of phospholipid vesicles that can be…

Soft Condensed Matter · Physics 2024-04-01 Judith U. De Mel , Sudipta Gupta , Gerald J. Schneider