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While many-body systems can host long-ranged entangled quantum spin liquids (QSLs), the ingredients for realizing these as ground states can be prohibitively difficult. In many circumstances, one requires (i) a constrained Hilbert space and…

Strongly Correlated Electrons · Physics 2023-02-14 Rahul Sahay , Ashvin Vishwanath , Ruben Verresen

We have performed thermodynamic and neutron scattering measurements on the S=1/2 kagome lattice antiferromagnet Zn Cu_3 (OH)_6 Cl_2. The susceptibility indicates a Curie-Weiss temperature of ~ -300 K; however, no magnetic order is observed…

Strongly Correlated Electrons · Physics 2007-05-23 J. S. Helton , K. Matan , M. P. Shores , E. A. Nytko , B. M. Bartlett , Y. Yoshida , Y. Takano , A. Suslov , Y. Qiu , J. -H. Chung , D. G. Nocera , Y. S. Lee

Quantum spin liquid (QSL) is a disordered state of quantum-mechanically entangled spins commonly arising from frustrated magnetic dipolar interactions. However, QSL in some pyrochlore magnets can also come from frustrated magnetic octupolar…

In condensed matter physics, there is a novel phase termed "quantum spin liquid", in which strong quantum fluctuations prevent the long-range magnetic order from being established, and so the electron spins do not form an ordered pattern…

Strongly Correlated Electrons · Physics 2019-04-10 Jinsheng Wen , Shun-Li Yu , Shiyan Li , Weiqiang Yu , Jian-Xin Li

Quantum spin ice is an appealing proposal of a quantum spin liquid - systems where the magnetic moments of the constituent electron spins evade classical long-range order to form an exotic state that is quantum entangled and coherent over…

Quantum spin liquid (QSL) state in rare-earth triangular lattice has attracted much attention recently due to its potential application in quantum computing and communication. Here we report the single-crystal growth synthesis, crystal…

Strongly Correlated Electrons · Physics 2021-11-16 Jie Xing , Liurukara D. Sanjeewa , Andrew F. May , Athena S. Sefat

Recent studies have revealed that the randomness-induced quantum spin liquid (QSL)-like state is stabilized in certain frustrated quantum magnets in two and three dimensions. In order to clarify the nature of this gapless QSL-like state, we…

Strongly Correlated Electrons · Physics 2021-11-24 Kazuki Uematsu , Toshiya Hikihara , Hikaru Kawamura

Quantum spin liquids are exotic Mott insulators that carry extraordinary spin excitations and thus, when doped, expected to afford novel metallic states coupled to the unconventional magnetic excitations. The organic triangular-lattice…

Strongly Correlated Electrons · Physics 2025-01-07 H. Oike , Y. Suzuki , H. Taniguchi , K. Miyagawa , K. Kanoda

Quantum spin liquids (QSL) have generated considerable excitement as phases of matter with emergent gauge structures and fractionalized excitations. In this context, phase transitions out of QSLs have been widely discussed as Higgs…

Strongly Correlated Electrons · Physics 2021-09-15 Hyeok-Jun Yang , Nic Shannon , SungBin Lee

The quasi two-dimensional Mott insulator $\alpha$-RuCl$_3$ is proximate to the sought-after Kitaev quantum spin liquid (QSL). In a layer of $\alpha$-RuCl$_3$ on graphene the dominant Kitaev exchange is further enhanced by strain. Recently,…

Strongly Correlated Electrons · Physics 2021-03-24 V. Leeb , K. Polyudov , S. Mashhadi , S. Biswas , Roser Valenti , M. Burghard , J. Knolle

Recent advances in material synthesis made it possible to realize two-dimensional monolayers of candidate materials for a quantum spin liquid (QSL) such as $\alpha$-RuCl$_3$,1T-TaSe$_2$ and 1T-TaS$_2$. In this work, we propose an…

Strongly Correlated Electrons · Physics 2023-07-27 Raffaele Mazzilli , Alex Levchenko , Elio J. König

Organic solids host various electronic phases. Especially, a milestone compound of organic solid, $\beta'$-$X$[Pd(dmit)$_2$]$_2$ with $X$=EtMe$_3$Sb shows quantum spin-liquid (QSL) properties suggesting a novel state of matter. However,…

Strongly Correlated Electrons · Physics 2022-04-29 Kota Ido , Kazuyoshi Yoshimi , Takahiro Misawa , Masatoshi Imada

Continuous spin excitations are widely recognized as one of the hallmarks of novel spin states in quantum magnets, such as quantum spin liquids (QSLs). Here, we report the observation of such kind of excitations in K2Ni2(SO4)3, which…

Kitaev magnets are materials with bond-dependent Ising interactions between localized spins on a honeycomb lattice. Such interactions could lead to a quantum spin-liquid (QSL) ground state at zero temperature. Recent theoretical studies…

The possible existence of a quantum spin liquid (QSL) phase, an exotic state of matter with long-range quantum entanglement and fractionalized excitations, in $\alpha$-RuCl$_3$ has sparked widespread interests in exploring QSLs in various…

Strongly Correlated Electrons · Physics 2023-04-04 Shun-Yao Yu , Han Li , Qi-Rong Zhao , Yuan Gao , Xiao-Yu Dong , Zheng-Xin Liu , Wei Li , Shou-Shu Gong

The search for the experimental evidence of quantum spin liquid (QSL) states is critical but extremely challenging, as the quenched interaction randomness introduced by structural imperfection is usually inevitable in real materials.…

Strongly Correlated Electrons · Physics 2022-11-08 Fangjun Lu , Long Yuan , Jian Zhang , Boqiang Li , Yongkang Luo , Yuesheng Li

By using a high pressure, high temperature (HPHT) technique, the antiferromagnetically ordered ($T_N$ = 13.5 K) 6H-A phase of Ba$_3$NiSb$_2$O$_9$ was transformed into two new gapless quantum spin liquid(QSL) candidates with S=1 (Ni$^{2+}$)…

Strongly Correlated Electrons · Physics 2011-11-08 J. G. Cheng , G. Li , L. Balicas , J. S. Zhou , J. B. Goodenough , Cenke Xu , H. D. Zhou

A new quantum spin liquid (QSL) candidate material H$_{3}$LiIr$_{2}$O$_{6}$ was synthesized recently and was found not to show any magnetic order or phase transition down to low temperatures. In this work, we study the quantum dynamics of…

Strongly Correlated Electrons · Physics 2020-08-17 Shuai Wang , Long Zhang , Fa Wang

Quantum spin liquids are long-range entangled states of matter with emergent gauge fields and fractionalized excitations. While candidate materials, such as the Kitaev honeycomb ruthenate $\alpha$-RuCl$_3$, show magnetic order at low…

Strongly Correlated Electrons · Physics 2019-07-16 I. Rousochatzakis , S. Kourtis , J. Knolle , R. Moessner , N. B. Perkins

Arguably the most favorable situation for spins to enter the long-sought quantum spin liquid (QSL) state is when they sit on a kagome lattice. No consensus has been reached in theory regarding the true ground state of this promising…

Strongly Correlated Electrons · Physics 2022-01-05 Y. Y. Huang , Y. Xu , Le Wang , C. C. Zhao , C. P. Tu , J. M. Ni , L. S. Wang , B. L. Pan , Ying Fu , Zhanyang Hao , Cai Liu , Jia-Wei Mei , S. Y. Li