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We show that circularly polarized femtosecond laser pulses produce field-free alignment in linear and planar molecules. We study the rotational wavepacket evolution of O$_2$ and benzene created by circularly polarized light. For benzene, we…

Chemical Physics · Physics 2014-06-06 C T L Smeenk , P B Corkum

Frequency-angular distributions for THz emission in the range of 0.1 - 3 THz generated in a single-color laser filament plasma situated both under and without electrostatic field are for the first time experimentally studied. The angular…

A recent expansion of cold and ultracold molecule applications has led to renewed focus on molecular species preparation under ultrahigh vacuum conditions. Meanwhile, molecular beams have been used to study gas phase chemical reactions for…

Atomic Physics · Physics 2016-02-23 M. G. Kokish , V. Rajagopal , J. P. Marler , B. C. Odom

Short laser pulses are widely used for controlling molecular rotational degrees of freedom and inducing molecular alignment, orientation, unidirectional rotation and other types of coherent rotational motion. To follow the ultra-fast…

A new phenomenon of enhancing the relativistic transparency of overdense plasmas by the influence of hot-electron refluxing has been found via particle-in-cell simulations. When a p-polarized laser pulse, with intensity below the…

Plasma Physics · Physics 2019-02-20 Yong Yu , Xiao-Ya Li , Zi-Yu Chen , Jia-Xiang Wang , Wen-Jun Zhu

While many-particle entanglement can be found in natural solids and strongly interacting atomic and molecular gases, generating highly entangled states between weakly interacting particles in a controlled and scalable way presents a…

Atomic Physics · Physics 2013-02-27 Felipe Herrera , Sabre Kais , K. Birgitta Whaley

Due to electronic many-body effects, the ionization of a molecule can trigger ultrafast electron dynamics appearing as a migration of the created hole charge throughout the system. Here we propose a scheme for control of the charge…

Chemical Physics · Physics 2015-06-11 Nikolay V. Golubev , Alexander I. Kuleff

We provide a theory of the deflection of polar and non-polar rotating molecules by inhomogeneous static electric field. Rainbow-like features in the angular distribution of the scattered molecules are analyzed in detail. Furthermore, we…

Chemical Physics · Physics 2015-05-20 E. Gershnabel , I. Sh. Averbukh

We report the observation of macroscopic field-free orientation, i.e. more than 73 % of CO molecules pointing in the same direction. This is achieved through an all-optical scheme operating at high particle densities ($>10^{17}$cm$^{-3}$)…

Chemical Physics · Physics 2014-07-09 P. M. Kraus , D. Baykusheva , H. J. Wörner

Broadband ultrashort terahertz (THz) pulses can be produced using plasma generation in a noble gas ionized by femtosecond two-color pulses. Here we demonstrate that, by using multiple-frequency laser pulses, one can obtain a waveform which…

We demonstrate a scheme for enhanced proton acceleration from near-critical-density targets by splitting a laser pulse into a linearly and a circularly polarized laser pulse. The combination of two laser pulses generates a shock wave as…

Plasma Physics · Physics 2025-02-25 D N Gupta , Saurabh Kumar , S Kar

The field-free alignment and orientation of the linear molecule by the two-color trapezoidal laser pulses were theoretically investigated. The trapezoidal shape of a laser pulse allows to enhance the maximum alignment degree for the same…

Quantum Physics · Physics 2024-01-11 Eugene A. Koval

Mountain echoes are a well-known phenomenon, where an impulse excitation is mirrored by the rocks to generate a replica of the original stimulus, often with reverberating recurrences. For spin echoes in magnetic resonance and photon echoes…

The generation of ultrashort pulses hinges on the careful management of dispersion. Traditionally, this has exclusively involved second-order dispersion, while higher-order dispersion was treated as a nuisance to be minimized. Here we show…

We present a combined analytical and numerical investigation to show how an optimal control field can be designed to generate maximum field-free orientation of molecules for three populated rotational states. Based on a model involving pure…

Quantum Physics · Physics 2021-07-28 Qian-Qian Hong , Li-Bao Fan , Chuan-Cun Shu , Niels E. Henriksen

Utilizing ultrafast light-matter interaction to manipulate electronic states of quantum materials is an emerging area of research in condensed matter physics. It has significant implications for the development of future ultrafast…

Photoexcitation of metallic nanostructures with short optical pulses can drive non-thermal electronic states, which, upon decay, lead to elevated electronic temperatures ($T_e \gtrapprox 1000\,\mathrm{K}$) eventually equilibrating with the…

Mesoscale and Nanoscale Physics · Physics 2025-01-07 Qian Ye , Stephen K. Sanders , Andrea Schirato , Alessandro Alabastri

We propose a method of stimulated laser cooling of diatomic molecules by counter-propagating $\pi$-trains of ultrashort laser pulses. The cooling cycles occur on the rovibrational transitions inside the same ground electronic manifold, thus…

Atomic Physics · Physics 2015-03-13 Ekaterina Ilinova , Jonathan Weinstein , Andrei Derevianko

Given the wide range of applications of time-domain spectroscopy, and particularly THz time-domain spectroscopy, the modelling of a probe pulse propagating through a multilayered structure is often required. Due to the fact that the…

Optics · Physics 2021-11-23 Yingshu Yang , Stefano Dal Forno , Marco Battiato

Localized heating of a gas by intense laser pulses leads to interesting acoustic, hydrodynamic and optical effects with numerous applications in science and technology, including controlled wave guiding and remote atmosphere sensing.…

Optics · Physics 2015-09-30 A. A. Milner , A. Korobenko , K. Rezaiezadeh , V. Milner
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