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Efficiently detecting and characterizing individual spins in solid-state hosts is an essential step to expand the fields of quantum sensing and quantum information processing. While selective detection and control of a few 13C nuclear spins…

Quantum Physics · Physics 2020-10-22 Hyunseok Oh , Jiwon Yun , M. H. Abobeih , Kyung-Hoon Jung , Kiho Kim , T. H. Taminiau , Dohun Kim

We analytically calculate the nuclear-spin interactions of a single electron confined to a carbon nanotube or graphene quantum dot. While the conduction-band states in graphene are p-type, the accordant states in a carbon nanotube are…

Mesoscale and Nanoscale Physics · Physics 2009-10-02 Jan Fischer , Bjoern Trauzettel , Daniel Loss

Precise characterization of a hyperfine interaction is a prerequisite for high fidelity manipulations of electron and nuclear spins belonging to a hybrid qubit register in diamond. Here, we demonstrate a novel scheme for determining a…

Quantum Physics · Physics 2013-09-11 J. H. Shim , B. Nowak , I. Niemeyer , J. Zhang , F. D. Brandao , D. Suter

Quantum spin networks having engineered geometries and interactions are eagerly pursued for quantum simulation and access to emergent quantum phenomena such as spin liquids. Spin-1/2 centers are particularly desirable because they readily…

An electron density functional approach for the calculation of the nuclear multipole moments is presented. The electronic matrix elements entering the experimentally observed hyperfine electron-nucleus interaction constants in atoms are…

Nuclear Theory · Physics 2007-05-23 R. L. Pavlov , P. P. Raychev , V. P. Garistov , M. Dimitrova-Ivanovich , J. Maruani

The detection of nuclear spins using individual electron spins has enabled new opportunities in quantum sensing and quantum information processing. Proof-of-principle experiments have demonstrated atomic-scale imaging of nuclear-spin…

Nanoscale nuclear magnetic resonance (NMR) signals can be measured through hyperfine interaction to paramagnetic electron sensor spins. A heterodyne approach is widely used to overcome the electron spin lifetime limit in spectral…

We study the hyperfine interaction between the nuclear spins and the electrons in a HgTe quantum well, which is the prime experimentally realized example of a two-dimensional topological insulator. The hyperfine interaction is a naturally…

Mesoscale and Nanoscale Physics · Physics 2013-09-06 Anders Mathias Lunde , Gloria Platero

We employ collisions of individual atomic cesium (Cs) impurities with an ultracold rubidium (Rb) gas to probe atomic interaction with hyperfine- and Zeeman-state sensitivity. Controlling the Rb bath's internal state yields access to novel…

We review recent theoretical developments about the role of spins, electron-electron interactions, and spin-orbit coupling in metal nanoparticles and semiconductor quantum dots. For a closed system, in the absence of spin-orbit coupling or…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Yuval Oreg , P. W. Brouwer , X. Waintal , Bertrand I. Halperin

Rare-earth spin ensembles are a promising platform for microwave quantum memory applications due to their hyperfine transitions, which can exhibit exceptionally long coherence times when using an operation point with zero first-order Zeeman…

We present a rigorous quantum scattering study of the effects of hyperfine and Zeeman interactions on cold Li - H$_{2}$ collisions in the presence of an external magnetic field using a recent ab initio potential energy surface. We find that…

Chemical Physics · Physics 2024-03-06 Hubert Jóźwiak , Timur V. Tscherbul , Piotr Wcisło

We experimentally demonstrate the use of a single electronic spin to measure the quantum dynamics of distant individual nuclear spins from within a surrounding spin bath. Our technique exploits coherent control of the electron spin,…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Shimon Kolkowitz , Quirin P. Unterreithmeier , Steven D. Bennett , Mikhail D. Lukin

Electrically detected electron spin resonance (ESR) is used to study the hyperfine interaction of the two-dimensional electrons and the nuclei of the host lattice in a GaAs/AlGaAs heterostructure. Under the microwave and radio- frequency…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Chris Hillman , H. W. Jiang

We report a systematic study of the hyperfine interaction between the electron spin of a single nitrogen-vacancy (NV) defect in diamond and nearby $^{13}$C nuclear spins, by using pulsed electron spin resonance spectroscopy. We isolate a…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 A. Dréau , J. -R. Maze , M. Lesik , J. -F. Roch , V. Jacques

The transferred hyperfine interaction between nuclear and electron spins in an heavy fermion material depends on the hybridization between the $f$-electron orbitals and those surrounding a distant nucleus. In CeMIn$_5$ (M=Rh, Ir, Co), both…

Strongly Correlated Electrons · Physics 2021-08-04 P. Menegasso , J. C. Souza , I. Vinograd , Z. Wang , S. P. Edwards , P. G. Pagliuso , N. J. Curro , R. R. Urbano

Magnetic resonance imaging (MRI) revolutionized diagnostic medicine and biomedical research by allowing a noninvasive access to spin ensembles. To enhance MRI resolution to the nanometer scale, new approaches including scanning probe…

Mesoscale and Nanoscale Physics · Physics 2019-10-23 Philip Willke , Kai Yang , Yujeong Bae , Andreas J. Heinrich , Christopher P. Lutz

We study Si:P donor electron spin decoherence due to anisotropic hyperfine (AHF) interaction with the surrounding nuclear spin bath. In particular, we clarify the electron spin echo envelope modulation (ESEEM) in the Si:P system and the…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 W. M. Witzel , Xuedong Hu , S. Das Sarma

With a view towards implementation in microscopic transport simulations of heavy-ion collisions, the properties of spin-isospin modes are studied in nuclear matter consisting of nucleons and Delta isobars that interact by the exchange of pi…

Nuclear Theory · Physics 2015-06-26 J. Helgesson , J. Randrup

We review and summarize recent theoretical and experimental work on electron spin dynamics in quantum dots and related nanostructures due to hyperfine interaction with surrounding nuclear spins. This topic is of particular interest with…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 John Schliemann , Alexander Khaetskii , Daniel Loss