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We study the multiorder coherent Raman scattering of a quantum probe field in a far-off-resonance medium with a prepared coherence. Under the conditions of negligible dispersion and limited bandwidth, we derive a Bessel-function solution…

Quantum Physics · Physics 2009-11-10 Fam Le Kien , Anil K. Patnaik , K. Hakuta

The remarkable progress in the field of laser spectroscopy induced by the invention of the frequency-comb laser has enabled many new high-precision tests of fundamental theory and searches for new physics. Extending frequency-comb based…

Atomic Physics · Physics 2021-01-20 L. S. Dreissen , C. Roth , E. L. Gründeman , J. J. Krauth , M. G. J. Favier , K. S. E. Eikema

Optical frequency-comb-based-high-resolution spectrometers offer enormous potential for spectroscopic applications. Although various implementations have been demonstrated, the lack of suitable mid-infrared comb sources has impeded…

Optical frequency combs are one of the most remarkable inventions of the last decades. Originally conceived as the spectral counterpart of the train of short pulses emitted by mode-locked lasers, frequency combs have also been subsequently…

The optical microresonator-based frequency comb (microcomb) provides a versatile platform for nonlinear physics studies and has wide applications ranging from metrology to spectroscopy. Deterministic quantum regime is an unexplored aspect…

Fourier transform spectroscopy based on incoherent light sources is a well-established tool in research fields from molecular spectroscopy and atmospheric monitoring to material science and biophysics. It provides broadband molecular…

We discuss a simple, linear, zero-delay implementation of spectral shearing interferometry for amplitude and phase characterization of optical frequency comb sources and arbitrary waveforms. We demonstrate this technique by characterizing…

We determine the frequency of the Yb I $^1S_0 - ^1P_1$ transition at 399 nm using an optical frequency comb. Although this transition was measured previously using an optical transfer cavity [D. Das et al., Phys. Rev. A 72, 032506 (2005)],…

Atomic Physics · Physics 2016-12-05 Michaela Kleinert , M. E. Gold Dahl , Scott D. Bergeson

Stimulated Raman scattering (SRS) has played an increasingly pivotal role in chemistry and photonics. Recently, understanding of light-molecule interaction during SRS was brought to a new quantitative level through the introduction of…

Chemical Physics · Physics 2023-12-13 Wei Min , Xin Gao

Optical frequency comb, as a spectrum made of discrete and equally spaced spectral lines, is a light source with essential applications in modern technology. Cavity optomechanical systems were found to be a feasible candidate for realizing…

Optics · Physics 2024-08-13 Xin Gu , Jinlian Zhang , Shulin Ding , Xiaoshun Jiang , Bing He , Qing Lin

Multi-spectral frequency combs provide frontier architectures for laser standoff spectroscopy, optical clockwork, and high-capacity optical communications. Frequency microcombs, aided by their high-quality resonances and inherent…

Quantum cascade laser (QCL) frequency combs are a promising candidate for chemical sensing and biomedical diagnostics, requiring only milliseconds of acquisition time to record absorption spectra without any moving parts. They are…

Frequency combs are light sources with coherent evenly-spaced lines. It has been observed that in certain laser systems, combs can form whose output is frequency-modulated (FM) in time. In this state, they produce an output whose frequency…

Optics · Physics 2020-06-23 David Burghoff

Non-perturbative and phase-sensitive light-matter interactions have led to the generation of attosecond pulses of light and the control electrical currents on the same timescale. Traditionally, probing these effects via high harmonic…

Optics · Physics 2022-05-17 Daniel M. B. Lesko , Kristina F. Chang , Scott A. Diddams

We present a quantum-mechanical model that describes fiber-based frequency conversion by four-wave-mixing Bragg scattering in the presence of Raman interactions. In the case of continuous-wave pumps we find closed-form expressions for the…

Quantum Physics · Physics 2024-06-06 Mathias Linde Holst Korsgaard , Jacob Gade Koefoed , Karsten Rottwitt

Frequency combs have triggered an impressive evolution of optical metrology across diverse regions of the electromagnetic spectrum, from the ultraviolet to the terahertz frequencies. An unexplored territory, however, remains in the region…

We demonstrate the acquisition of stimulated Raman scattering spectra with the use of a single femtosecond pulse. High resolution vibrational spectra are obtained by shifting the phase of a narrow band of frequencies in the broadband input…

Optics · Physics 2015-05-20 Hadas Frostig , Ori Katz , Adi Natan , Yaron Silberberg

Optical frequency combs, with precise control of repetition rate and carrier-envelope-offset frequency, have revolutionized many fields, such as fine optical spectroscopy, optical frequency standards, ultra-fast science research,…

Optics · Physics 2018-02-14 Y. Zhang , L. Yan , X. F. Zhang , L. Zhang , W. Han , W. Guo , H. Jiang , S. Zhang

We show experimentally and theoretically that the spectral components of a multi-octave frequency comb spontaneously created by stimulated Raman scattering in a hydrogen-filled hollow-core photonic crystal fiber exhibit strong self…

Quantum Physics · Physics 2015-05-19 Y. Y. Wang , Chunbai Wu , F. Couny , M. G. Raymer , F. Benabid

Ring quantum cascade lasers (QCLs) proved to be a versatile tool for generating tunable and stable frequency combs in the mid infrared range in the form of quantum walk combs. By homogeneously integrating a racetrack QCL with a passive…

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