Related papers: A new standard in high-field terahertz generation:…
Organic nonlinear optical (NLO) crystals have emerged as efficient room-temperature emitters of broadband THz radiation with high electric field strengths. Although initially confined to high-pulse-energy excitation in the millijoule range…
We characterize the terahertz (THz) generation of N-benzyl-2-methyl-4-nitroaniline (BNA), with crystals ranging in thickness from 123-700 {\mu}m. We compare excitation using 800-nm and 1250 to 1500-nm wavelengths. Pumping BNA with 800-nm…
The rapid advancement of communication technology necessitates the development of hybrid optical modulators that integrate silicon photonics with electro-optic (EO) materials to enable ultrafast, low-power, and compact photonic devices.…
The generation of tunable narrowband pulses is increasingly being pursued in terahertz science, for example to study the nonlinear response of individual modes of solids and molecules. Here, we extend the chirp-and-delay method to achieve…
We report on high energy terahertz pulses by optical rectification (OR) in the organic crystal N-benzyl-2-methyl-4-nitroaniline (BNA) directly pumped by a conventional Ti:Sapphire (Ti:Sa) amplifier. The simple scheme provides an optical to…
Increasing the average power of broadband, few-cycle terahertz (THz) sources is currently a topic of intense investigation, fueled by recent immense progress in high average power femtosecond laser driving sources at 1030 nm. However, many…
The organic terahertz (THz) generation crystal BNA has recently gained traction as a valuable source to produce broadband THz pulses. Even when pumped with 800-nm light, thin BNA crystals can produce relatively high electric fields with…
We are reporting on terahertz generation from organic crystal BNA using a 1.15 to 1.55 um near infrared pump. We observed a very large emission spectrum extending up to 7 THz, compared to 2.5 THz from Ti:Sa pump in previous reports. The…
We demonstrate record conversion efficiencies of up to 0.9 percent for narrowband (1 percent relative bandwidth) THz generation by strongly-cascaded difference frequency generation. These results are achieved using a novel laser source,…
As high-average power ultrafast lasers become increasingly available for nonlinear conversion, the temperature dependence of the material properties of nonlinear crystals becomes increasingly relevant. Here, we present temperature-dependent…
We present a high power and broadband THz-TDS setup utilizing the nonlinear organic crystal MNA both as emitter and detector. The THz source is based on optical rectification of near infra-red laser pulses at a central wavelength of 1036 nm…
Highly efficient terahertz (THz) wave sources based on difference frequency generation (DFG) process in nonlinear optical crystals play an important role for the applications of THz wave. In order to find more novel nonlinear crystals, here…
We demonstrate a data mining approach to discover and develop new organic nonlinear optical crystals that produce intense pulses of terahertz radiation. We mine the Cambridge Structural Database for non-centrosymmetric materials and use…
We demonstrate a 13.3 MHz repetition rate, broadband THz source with milliwatt-average power, obtained by collinear optical rectification of a high-power Yb-doped thin-disk laser in the organic crystal BNA…
We demonstrate efficient optical rectification in the organic crystal BNA (N-benzyl-2-methyl-4-nitroaniline), driven by a temporally compressed, commercially available industrial Yb-laser system operating at 540 kHz repetition rate. Our THz…
Sensitive detection of terahertz (THz) radiation is fundamental to progress in spectroscopy, advanced wireless communication, and the realization of emerging quantum technologies. However, the intrinsically low photon energies in the THz…
A highly efficient, practical approach to high-energy terahertz (THz) generation based on spectrally cascaded optical parametric amplification (THz-COPA) is introduced. The THz wave initially generated by difference frequency generation…
High-energy terahertz pulses are challenging to produce due to the low conversion efficiency and limited optical damage threshold of nonlinear crystals. Here, we describe the high-efficiency generation of terahertz radiation pulses with…
In this work, the polar tetrahedron [PN$_2$O$_2$] was revealed as a new deep-ultraviolet (deep-UV) nonlinear optically active unit. Accordingly, a thermodynamically stable compound (PNO) consisting of the polar [PN$_2$O$_2$] units was…
The intense terahertz (THz) pulses facilitate the observation of various nonlinear optical effects and manipulation of material properties. In this work, we report a convenient approach that can produce strong broadband terahertz pulses…