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Conical intersections play a pivotal role in excited-state quantum dynamics. Capturing transient molecular structures near conical intersections remains challenging due to the rapid timescales and subtle structural changes involved. We…

Electronic charge transfer at the atomic scale can reveal fundamental information about chemical bonding, but is far more challenging to directly image than the atomic structure. The charge density is dominated by the atomic nuclei, with…

Materials Science · Physics 2025-05-01 Christoph Hofer , Jacob Madsen , Toma Susi , Timothy J. Pennycook

Melting is an everyday phase transition that is determined by thermodynamic parameters like temperature and pressure. In contrast, ultrafast melting is governed by the microscopic response to a rapid energy input and, thus, can reveal the…

Laser-assisted electron scattering (LAES), a light-matter interaction process that facilitates energy transfer between strong light fields and free electrons, has so far been observed only in gas phase. Here we report on the observation of…

The collision of two ultra-cold atoms results in a quantum-mechanical superposition of two outcomes: each atom continues without scattering and each atom scatters as a spherically outgoing wave with an s-wave phase shift. The magnitude of…

Quantum Physics · Physics 2007-05-23 Russell A. Hart , Xinye Xu , Ronald Legere , Kurt Gibble

We investigate the quantum dynamics of fermionic particles interacting with a laser field in a gaseous medium, in the regime of inelastic diffraction scattering on the phase lattice of a slowed travelling wave, below the critical field of…

Optics · Physics 2025-07-04 H. K. Avetissian , G. F. Mkrtchian

Streaking of photoelectrons has long been used for the temporal characterization of attosecond extreme ultraviolet pulses. When the time-resolved photoelectrons originate from a coherent superposition of electronic states, they carry an…

Chemical Physics · Physics 2016-07-27 Markus Kowalewski , Kochise Bennett , Jérémy R. Rouxel , Shaul Mukamel

The tunnelling of an electron through a suppressed atomic potential followed by its motion in the continuum, is the fundamental mechanism underlying strong-field laser-atom/molecule interactions. Due to its quantum nature, the interaction…

In experimental physics, it is essential to understand electromagnetic (EM) wave scattering across EM spectrum, from radio waves to X-rays, and is pivotal in driving photonics innovations. Recent advancements have uncovered phenomena like…

Optics · Physics 2024-02-23 Deepanshu Trivedi , Arjuna Madanayake , Alex Krasnok

Four-dimensional scanning transmission electron microscopy (4D-STEM) of local atomic diffraction patterns is emerging as a powerful technique for probing intricate details of atomic structure and atomic electric fields. However, efficient…

Image and Video Processing · Electrical Eng. & Systems 2019-01-15 Xin Li , Ondrej E. Dyck , Mark P. Oxley , Andrew R. Lupini , Leland McInnes , John Healy , Stephen Jesse , Sergei V. Kalinin

Laser photons carrying non-zero orbital angular momentum are known and exploited during the last twenty years. Recently it has been demonstrated experimentally that such (twisted) electrons can be produced and even focused to a subnanometer…

Quantum Physics · Physics 2016-09-15 D. V. Karlovets , G. L. Kotkin , V. G. Serbo

The interaction of swift, free-space electrons with confined optical near fields has recently sparked much interest. It enables a new type of photon-induced near-field electron microscopy, mapping local optical near fields around…

Quantum Physics · Physics 2021-10-27 Germann Hergert , Andreas Woeste , Petra Gross , Christoph Lienau

Development of experimental techniques for characterization of magnetic properties at high spatial resolution is essential for progress in miniaturization of magnetic devices, for example, in data storage media. Inelastic scattering of…

Materials Science · Physics 2014-04-02 Jan Rusz , Somnath Bhowmick

Future ultrafast x-ray light sources might image ultrafast coherent electron motion in real-space and in real-time. For a rigorous understanding of such an imaging experiment, we extend the theory of non-resonant x-ray scattering to the…

Atomic Physics · Physics 2015-06-19 Gopal Dixit , Jan Malte Slowik , Robin Santra

We study the effects of strong inter-particle interaction on diffraction of a Bose-Einstein condensate of $^6Li_2$ molecules from a periodic potential created by pulses of a far detuned optical standing wave. For short pulses we observe the…

Quantum Gases · Physics 2022-05-11 Qi Liang , Chen Li , Sebastian Erne , Pradyumna Paranjape , RuGway Wu , Jörg Schmiedmayer

Inelastic scattering of electrons incident on a solid surface is determined by the two properties: (i) electronic response of the target system and (ii) the detailed quantum-mechanical motion of the projectile electron inside and in the…

Materials Science · Physics 2016-01-06 V. U. Nazarov , V. M. Silkin , E. E. Krasovskii

Recent advancements in abilities to create and manipulate the electron's transverse wave function within the transmission electron microscope (TEM) and scanning TEM (STEM) have enabled vectorially-resolved electron energy loss (EEL) and…

Mesoscale and Nanoscale Physics · Physics 2024-03-12 Austin G. Nixon , Matthieu Chalifour , Marc R. Bourgeois , Michael Sanchez , David J. Masiello

Sub-angstrom spatial resolution of electron density coupled with sub-femtosecond temporal resolution is required to directly observe the dynamics of the electronic structure of a molecule after photoinitiation or some other ultrafast…

The non-linear coupled particle light dynamics of an ultracold gas in the field of two independent counter-propagating laser beams can lead to the dynamical formation of a self-ordered lattice structure as presented in Phys. Rev. X 6,…

Quantum Physics · Physics 2018-01-17 Stefan Ostermann , Francesco Piazza , Helmut Ritsch

Ultrafast electron diffraction using MeV energy beams(MeV-UED) has enabled unprecedented scientific opportunities in the study of ultrafast structural dynamics in a variety of gas, liquid and solid state systems. Broad scientific…