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We study non-perturbatively the anomalous Hall current and its high harmonics generated in Weyl and Dirac semimetals by strong elliptically polarized laser fields, in the context of kinetic theory. We find a novel crossover between…

Mesoscale and Nanoscale Physics · Physics 2021-05-12 Renato M. A. Dantas , Zhe Wang , Piotr Surówka , Takashi Oka

Strong light-matter coupling within electromagnetic environments provides a promising path to modify and control chemical and physical processes. The origin of the enhancement of nonlinear optical processes such as second-harmonic and…

Optics · Physics 2022-03-03 Davis M. Welakuh , Prineha Narang

To clarify the microscopic origin of chirality-induced optical effect, we develop an analytical method that extracts the chiral part of the Hamiltonian of molecular electronic states. We demonstrate this method in a model chiral molecule…

Materials Science · Physics 2024-09-04 Akihito Kato , Nobuhiko Yokoshi

The emerging possibilities to steer and control electronic motion on subcycle time scales with strong electric fields enable studying the nonperturbative optical response and Bloch bands' topological properties, originated from Berry's…

Mesoscale and Nanoscale Physics · Physics 2021-01-12 Hamed Koochaki Kelardeh

High order harmonic generation from clusters is a controversial topic: conflicting theories exist, with different explanations for similar experimental observations. From an experimental point of view, separating the contributions from…

Atomic and Molecular Clusters · Physics 2015-06-12 H. Ruf , C. Handschin , R. Cireasa , N. Thiré , A. Ferré , S. Petit , D. Descamps , E. Mével , E. Constant , V. Blanchet , B. Fabre , Y. Mairesse

High-harmonic generation (HHG) in two-dimensional materials offers a compelling route toward compact extreme ultraviolet sources and probing electron dynamics on the attosecond scale. However, achieving precise control over the emission and…

Computational Physics · Physics 2026-05-19 Zhenjiang Zhao , Zhihua Zheng , Zhiyi Xu , Xing Ran , Xiaolong Yao , Fangping Ouyang

Optical modulation of high-harmonics generation in solids enables the detection of material properties such as the band structure and promising new applications such as super-resolution imaging in semiconductors. Various recent studies have…

This Letter brings together two topics that, until now, have been the focus of intense but non-overlapping research efforts. The first concerns high harmonic generation in solids, which occurs when intense light field excites highly…

Strongly Correlated Electrons · Physics 2022-04-06 R. E. F. Silva , Igor V. Blinov , Alexey N. Rubtsov , O. Smirnova , M. Ivanov

High harmonic generation is a convenient way to obtain extreme ultraviolet light from table-top laser systems and the experimental tools to exploit this simple and powerful light source for time-resolved spectroscopy are being developed by…

Atomic and Molecular Clusters · Physics 2013-12-20 Jakob Grilj , Emily Sistrunk , Markus Koch , Markus Gühr

Using a high-frequency field superposed to a linearly polarized bichromatic laser field composed by a wave with frequency $\omega $ and a wave with frequency $2\omega $, we show it is possible to enhance the intensity of a group of high…

Atomic Physics · Physics 2009-11-06 C. Figueira de Morisson Faria , M. L. Du

The first high harmonic spectrum, containing only the odd orders, was observed in experiments 30 years ago (1987). However, a spectrum containing pure even harmonics has never been observed. We investigate the generation of pure even…

Optics · Physics 2017-11-22 Hongtao Hu , Na Li , Peng Liu , Ruxin Li , Zhizhan Xu

Thermotropic liquid crystals are versatile optical materials that exhibit a state of matter intermediate between liquids and solids. Their properties can change significantly with temperature, pressure, or other external factors, leading to…

We study a certain type of anomalous Hall current in magnetically- and electrically-biased bulk GaAs samples under the formation of Landau levels. The currents are generated by ultrafast optical excitation of spin-polarized carriers and…

Mesoscale and Nanoscale Physics · Physics 2025-03-28 Christoph Dresler , Shekhar Priyadarshi , Mark Bieler

We experimentally explore the fingerprint of the microscopic electron dynamics in second-order harmonic generation (SHG). It is shown that the interbond electron hopping induces a novel source of nonlinear polarization and plays an…

The Hall effect, in which current flows perpendicular to an applied electrical bias, has played a prominent role in modern condensed matter physics over much of the subject's history. Appearing variously in classical, relativistic and…

Materials Science · Physics 2021-07-08 Libor Smejkal , Allan H. MacDonald , Jairo Sinova , Satoru Nakatsuji , Tomas Jungwirth

We study numerically the Bloch electron wave-packet dynamics in periodic potentials to simulate laser-solid interactions. We introduce a quasi-classical model in the \emph{k} space combined with the energy band structure to understand the…

Optics · Physics 2017-01-05 Tao-Yuan Du , Xue-Bin Bian

High harmonic generation (HHG) in solids has emerged as a powerful spectroscopic method for resolving ultrafast electron dynamics and band structure properties across a wide range of materials. However, quantitative HHG studies require…

Optics · Physics 2025-12-16 S. Mandal , P. Kumar , Z. Pi , H. Y. Kim , M. Zhan , E. Goulielmakis

We observe enhanced second-harmonic generation in monolayer graphene in the presence of an ultra-strong terahertz field pulse with a peak amplitude of 250 kV/cm. This is a strongly nonperturbative regime of light-matter interaction in which…

High-harmonic generation (HHG) in liquids is opening new opportunities for attosecond light sources and attosecond time-resolved studies of dynamics in the liquid phase. In gas-phase HHG, few-cycle pulses are routinely used to create…

We report measurements and theoretical simulations of high-order harmonic generation (HHG) in aligned N$_2$ molecules using a 1200-nm intense laser field when the generating pulse is perpendicular to the aligning one. With increasing laser…

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