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Mercury (Hg) and superheavy element copernicium (Cn) are investigated using equation-of-motion relativistic coupled-cluster (EOM-RCC) and configuration interaction plus many-body perturbation theory (CI+MBPT) methods. Key atomic properties…

Atomic Physics · Physics 2025-07-25 Hongxu Liu , Jize Han , Yanmei Yu , Yanfeng Ge , Yong Liu , Zhiguo Huang

In this work, we propose a multi-scale protocol for routine theoretical studies of chemical reaction mechanisms. The initial reaction paths of our investigated systems are sampled using the Nudged-Elastic Band (NEB) method driven by a cheap…

Chemical Physics · Physics 2023-07-26 Tomislav Piskor , Peter Pinski , Thilo Mast , Vladimir V. Rybkin

We report the result of our calculation of the nuclear spin-independent parity violating electric dipole transition amplitude ($E1_{PV}$) for the $6s ~ ^2S_{1/2} - 7s ~ ^2S_{1/2}$ transition in $^{133}$Cs to an accuracy of 0.3\% using a…

High Energy Physics - Phenomenology · Physics 2020-09-01 B. K. Sahoo , B. P. Das

The low-lying n(=3,4,5)d $^2D_{5/2}$ states alkaline earth ions are of vital importance in a number of different physical applications. The hyperfine structure constants of these states are characterized by unusually strong electron…

Atomic Physics · Physics 2015-06-26 B. K. Sahoo , C. Sur , T. Beier , B. P. Das , R. K. Chaudhuri , D. Mukherjee

Excited-state electronic structure in strongly correlated systems remains challenging due to the exponential scaling of the many-body Hilbert space and the difficulty of constructing systematically controlled active spaces. Building on the…

Chemical Physics · Physics 2026-05-05 Annabelle Canestraight , Russell Miller , Libor Veis , Vojtech Vlcek

We describe our efforts of the past few years to create a large set of more than 500 highly-accurate vertical excitation energies of various natures ($\pi \to \pi^*$, $n \to \pi^*$, double excitation, Rydberg, singlet, doublet, triplet,…

Passivity-based control (PBC) for port-Hamiltonian systems provides an intuitive way of achieving stabilization by rendering a system passive with respect to a desired storage function. However, in most instances the control law is obtained…

Systems and Control · Computer Science 2019-03-29 Olivier Sprangers , Gabriel A. D. Lopes , Robert Babuska

We present excitation energies for molecular doublets from a spin-adapted formulation of coupled cluster singles and doubles theory. The entanglement coupled cluster approach represents an unconventional take on the notorious problem of…

Chemical Physics · Physics 2025-04-08 Sarai Dery Folkestad , Kristine Lauvstad Kruken , Henrik Koch

We perform a global sensitivity analysis of the binding energy and the charge radius of the nucleus $^{16}$O to identify the most influential low-energy constants in the next-to-next-to-leading order chiral Hamiltonian with two- and…

Nuclear Theory · Physics 2019-12-25 Andreas Ekström , Gaute Hagen

A comparative study of two earlier three-state and fifteen-state [Chaudhuri et al., Pramana- J. Phys., 43, 175 (1994); ibid., Phys. Rev. A, 52, 1137 (1995)] close-coupled treatments of He2+-He single and double charge transfer collisions is…

Atomic and Molecular Clusters · Physics 2009-10-05 Chanchal Chaudhuri

A method and codes for two-step correlation calculation of heavy-atom molecules have been developed, employing the generalized relativistic effective core potential and relativistic coupled cluster (RCC) methods at the first step, followed…

Chemical Physics · Physics 2009-11-07 A. N. Petrov , N. S. Mosyagin , T. A. Isaev , A. V. Titov , V. F. Ezhov , E. Eliav , U. Kaldor

Variational, nonrelativisitic energies have been calculated for the ground state ($^3P_g$) and the lowest quintuplet state ($^5S_u$) of the carbon atom, with wavefunctions expressed in the basis of symmetry-projected, explicitly correlated…

Chemical Physics · Physics 2020-09-21 Krzysztof Strasburger

Energies for the lowest 56 levels, belonging to the 3s$^2$3p, 3s3p$^2$, 3p$^3$, 3s$^2$3d, 3s3p3d, 3s$^2$4$\ell$ and 3s$^2$5$\ell$ configurations of Si II, are calculated using the {\sc grasp} (General-purpose Relativistic Atomic Structure…

Instrumentation and Methods for Astrophysics · Physics 2015-06-19 KM Aggarwal , FP Keenan

The molecular ion H$_2^+$ is studied under strong confinement conditions produced by a spherical barrier centered in the gravity center of the molecule. Results for the potential curves are obtained by diffusion Monte Carlo methods for the…

Chemical Physics · Physics 2019-04-03 Gaia Micca Longo , Savino Longo , Domenico Giordano

The effective electric field experienced by the unpaired electron in the ground state of PbF, which is a potential candidate in the search of electron electric dipole moment due to some special characteristics, is calculated using Z-vector…

Atomic Physics · Physics 2015-08-28 Sudip Sasmal , Himadri Pathak , Malaya K. Nayak , Nayana Vaval , Sourav Pal

The polarizabilities and hyperpolarizabilities of the Be$^+$ ion in the $2^2S$ state and the $2^2P$ state are determined. Calculations are performed using two independent methods: i) variationally determined wave functions using Hylleraas…

Atomic Physics · Physics 2009-10-21 Li-Yan Tang , Jun-Yi Zhang , Zong-Chao Yan , Ting-Yun Shi , James F. Babb , J. Mitroy

In the present study, the newly established preformation formula is applied for the first time to study the kinematics of the cluster emission from various radioactive nuclei, especially those decaying to the double-shell closure $^{208}$Pb…

Nuclear Theory · Physics 2023-06-28 Joshua T. Majekodunmi , M. Bhuyan , K. Anwar , N. Abdullah , Raj Kumar

The random-phase approximation to the ground state correlation energy (RPA) in combination with exact exchange (EX) has brought Kohn-Sham (KS) density functional theory one step closer towards a universal, "general purpose first principles…

When the number of strongly correlated electrons becomes larger, the single-reference coupled-cluster (CC) CCSD, CCSDT, etc. hierarchy displays an erratic behavior, while traditional multi-reference approaches may no longer be applicable…

Chemical Physics · Physics 2025-12-12 Ilias Magoulas , Jun Shen , Piotr Piecuch

The open-shell reference relativistic equation-of-motion coupled-cluster method within its four-component description is successfully implemented with the consideration of single- and double- excitation approximation. The one-body and…

Atomic Physics · Physics 2016-09-21 Himadri Pathak , Sudip Sasmal , Malaya K. Nayak , Nayana Vaval , Sourav Pal