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In CALPHAD-type thermodynamic databases, nonstoichiometric compounds are typically described by sublattice models where the sublattice site fractions represent the occupation probability of different atomic, ionic or defect species on…

Materials Science · Physics 2025-03-04 Yanzhou Ji , Yueze Tan , Long-Qing Chen

Machine learning has become a crucial tool for predicting the properties of crystalline materials. However, existing methods primarily represent material information by constructing multi-edge graphs of crystal structures, often overlooking…

Machine Learning · Computer Science 2024-11-14 Chao Huang , Chunyan Chen , Ling Shi , Chen Chen

Efficient and precise prediction of plasticity by data-driven models relies on appropriate data preparation and a well-designed model. Here we introduce an unsupervised machine learning-based data preparation method to maximize the…

The ability to understand the atomistic mechanisms that occur in the solid phase transition is of crucial importance in materials research. To investigate the displacive phase transition at the atomic scale, we have implemented a numerical…

Materials Science · Physics 2025-06-06 Qiang Zhu , Byungkyun Kang , Kevin Parrish

With the aim of future applications in quantum mechanical embedding in extended systems such as crystals, we suggest a simple and computationally efficient method which enables construction of a set of nonorthogonal highly localized…

Computational Physics · Physics 2009-11-10 Oleh Danyliv , Lev Kantorovich

This paper develops a new continuous approach to a similarity between periodic lattices of ideal crystals. Quantifying a similarity between crystal structures is needed to substantially speed up the Crystal Structure Prediction, because the…

Computational Geometry · Computer Science 2024-09-05 Marco Michele Mosca , Vitaliy Kurlin

Artificial Intelligence (AI) in materials science is driving significant advancements in the discovery of advanced materials for energy applications. The recent GNoME protocol identifies over 380,000 novel stable crystals. From this, we…

Materials Science · Physics 2025-10-01 Paolo De Angelis , Giovanni Trezza , Giulio Barletta , Pietro Asinari , Eliodoro Chiavazzo

Reliable and robust methods of predicting the crystal structure of a compound, based only on its chemical composition, is crucial to the study of materials and their applications. Despite considerable ongoing research efforts, crystal…

Materials Science · Physics 2017-07-26 Qi-Jun Hong , Joseph Yasi , Axel van de Walle

The structure-property hypothesis says that the properties of all materials are determined by an underlying crystal structure. The main obstacle was the ambiguity of conventional crystal representations based on incomplete or discontinuous…

Computational Physics · Physics 2024-05-08 Jonathan Balasingham , Viktor Zamaraev , Vitaliy Kurlin

Crystal structure prediction (CSP) has emerged as one of the most important approaches for discovering new materials. CSP algorithms based on evolutionary algorithms and particle swarm optimization have discovered a great number of new…

Materials Science · Physics 2022-04-06 Wenhui Yang , Edirisuriya M. Dilanga Siriwardane , Jianjun Hu

Subgroup discovery (SGD) is presented here as a data-mining approach to help find interpretable local patterns, correlations, and descriptors of a target property in materials-science data. Specifically, we will be concerned with data…

Materials Science · Physics 2017-02-07 B. R. Goldsmith , M. Boley , J. Vreeken , M. Scheffler , L. M. Ghiringhelli

Polynomial machine learning potentials (MLPs) based on polynomial rotational invariants have been systematically developed for various systems and applied to efficiently predict crystal structures. In this study, we propose a robust…

Materials Science · Physics 2026-03-18 Hayato Wakai , Atsuto Seko , Isao Tanaka

Crystallisation is an important phenomenon which facilitates the purification as well as structural and bulk phase material characterisation using crystallographic methods. However, different conditions can lead to a vast set of different…

Robotics · Computer Science 2024-09-10 Edward C Lee , Daniel Salley , Abhishek Sharma , Leroy Cronin

Understanding structure-property relationships is an essential yet challenging aspect of materials discovery and development. To facilitate this process, recent studies in materials informatics have sought latent embedding spaces of crystal…

Machine Learning · Computer Science 2025-06-23 Yuta Suzuki , Tatsunori Taniai , Ryo Igarashi , Kotaro Saito , Naoya Chiba , Yoshitaka Ushiku , Kanta Ono

Disordered materials such as glasses, unlike crystals, lack long range atomic order and have no periodic unit cells, yielding a high dimensional configuration space with widely varying properties. The complexity not only increases…

Computational Engineering, Finance, and Science · Computer Science 2025-11-12 Qiyuan Chen , Ajay Annamareddy , Ying-Fei Li , Dane Morgan , Bu Wang

Clustering is an unsupervised machine learning method grouping data samples into clusters of similar objects. In practice, clustering has been used in numerous applications such as banking customers profiling, document retrieval, image…

Computer Vision and Pattern Recognition · Computer Science 2021-07-06 Raphaël Couturier , Hassan N. Noura , Ola Salman , Abderrahmane Sider

Mathematical crystal chemistry views crystal structures as the optimal solutions of mathematical optimization problem formalizing inorganic structural chemistry. This paper introduces the minimum and maximum atomic radii depending on the…

Materials Science · Physics 2025-04-01 Ryotaro Koshoji

We present detailed elaboration and first generally applicable linearization routines of the \textit{Parameter Space Concept} (PSC) for determining 1-dimensionally projected structures of $m$ independent scatterers. This crystal…

Computational Physics · Physics 2024-11-14 Muthu Vallinayagam , Melanie Nentwich , Dirk C. Meyer , Matthias Zschornak

Organic molecular crystals are ideally placed to become next-generation piezoelectric materials due to their diverse chemistries that can be used to engineer tailor-made solid-state assemblies. Using crystal engineering principles, and…

Materials Science · Physics 2024-12-11 Shubham Vishnoi , Geetu Kumari , Robert Guest , Pierre-André Cazade , Sarah Guerin

De novo crystal generation, a central task in materials discovery, aims to generate crystals that are simultaneously valid, stable, unique, and novel. Existing methods mainly rely on black-box stochastic sampling, providing limited control…

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