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Despite the enormous interest in the properties of graphene and the potential of graphene nanostructures in electronic applications, the study of quantum confined states in atomically well-defined graphene nanostructures remains an…

We extend our recently developed sparse-stochastic fragmented exchange formalism for ground-state hybrid DFT (ngH-DFT) to calculate absorption spectra within linear-response time-dependent Generalized Kohn-Sham DFT (LR-GKS-TDDFT), for…

Chemical Physics · Physics 2025-03-11 Mykola Sereda , Tucker Allen , Nadine C. Bradbury , Khaled Z. Ibrahim , Daniel Neuhauser

DFT calculation of various atomic species on graphene sheet is investigated as prototypes for formation of nano-structures on carbon nanotube (CNT) wall. We investigate computationally adsorption energies and adsorption sites on graphene…

Materials Science · Physics 2009-11-13 Akira Ishii , Masana Yamamoto , Hiroki Asano , Katsutoshi Fujiwara

We theoretically investigate the effects of long-range disorder and electron-electron interactions on the optical properties of hexagonal armchair graphene quantum dots consisting of up to 10806 atoms. The numerical calculations are…

Mesoscale and Nanoscale Physics · Physics 2017-02-08 A. Altıntaş , K. E. Çakmak , A. D. Güçlü

A few years ago, by means of first-principles calculations, Enyashin et al.(2011) proposed several novel monolayers of carbon containing rings other than hexagons. One of those monolayers containing tetragons and octagons was investigated…

Materials Science · Physics 2025-06-26 Arifa Nazir , Alok Shukla

The electronic absorption (EA), circular dichroism (ECD), and anisotropy spectra of the L-valine zwitterion and D-glyceraldehyde are calculated by time-dependent density functional theory (TDDFT) with the M06-2X and B3LYP functionals. It is…

Chemical Physics · Physics 2021-01-27 Jie Su , Bingbing Suo , Patrick Cassam-Chenaï

When calculating the optical absorption spectra of molecular crystals from first principles, the influence of the crystalline environment on the excitations is of significant importance. For such systems, however, methods to describe the…

Materials Science · Physics 2021-08-17 Joseph C. A. Prentice , Arash A. Mostofi

We employ the first-principles GW+Bethe Salpeter equation approach to study the electronic structure and optical absorption spectra of uniaxial strained graphene with many-electron effects included. Applied strain not only induces an…

Materials Science · Physics 2015-05-30 Yufeng Liang , Shouting Huang , Li Yang

Density functional theory (DFT) and many body perturbation theory at the G$_0$W$_0$ level are employed to study the electronic properties of polythiophene (PT) adsorbed on graphene surface. Analysis of charge density difference shows the…

Mesoscale and Nanoscale Physics · Physics 2017-09-07 F. Marsusi , I. A. Fedorov , S. Gerivani

Efficient identification of promising drug candidates for nanomaterial-based delivery systems is essential for advancing next-generation therapeutics. In this work, we present a synergistic framework combining density functional theory…

Computational Physics · Physics 2025-11-07 Chaithanya Purushottam Bhat , Pranav Suryawanshi , Aditya Guneja , Debashis Bandyopadhyay

Absorption of terahertz waves by a metasurface comprising a biperiodic array of pixellated meta-atoms on top of a dielectric substrate backed by a perfect electric conductor was simulated using a commercial software, with either all or a…

Optics · Physics 2019-11-12 Pankaj Kumar , Akhlesh Lakhtakia , Pradip K. Jain

We determine the optical properties of gated bilayer graphene quantum dots with trigonal warping (TW) of single-particle energy spectra. The lateral structure of metallic gates confines electrons and holes in a quantum dot (QD)…

Mesoscale and Nanoscale Physics · Physics 2025-06-03 Matthew Albert , Daniel Miravet , Yasser Saleem , Katarzyna Sadecka , Marek Korkusinski , Gabriel Bester , Pawel Hawrylak

We have recently developed a method based on relativistic time-dependent density functional theory (TD-DFT) that allows the calculation of electronic spectra in solution (Creutzberg, Hedeg{\aa}rd, J. Chem. Theory Comput.18, 2022, 3671).…

Chemical Physics · Physics 2023-04-04 Joel Creutzberg , Erik Donovan Hedegård

We investigate a quantum dot (QD) system coupled to a vibrational environment with a super-Ohmic spectral density and weakly to a leaky cavity mode, a model relevant for semiconductor-based single-photon sources. The phonon coupling induces…

Mesoscale and Nanoscale Physics · Physics 2024-12-31 Sebastian Toivonen , Kimmo Luoma

We present a density-functional theory (DFT) approach to the study of the phase diagram of the maximum density droplet (MDD) in two-dimensional quantum dots in a magnetic field. Within the lowest Landau level (LLL) approximation, analytical…

Mesoscale and Nanoscale Physics · Physics 2009-10-30 M. Ferconi , G. Vignale

Graphene layers grown by chemical vapour deposition (CVD) method and transferred from Cu-foils to the oxidized Si-substrates were investigated by spectroscopic ellipsometry (SE), Raman and X-Ray Photoelectron Spectroscopy (XPS) methods. The…

Materials Science · Physics 2018-02-23 Aarne Kasikov , Tauno Kahro , Leonard Matisen , Margus Kodu , Aivar Tarre , Helina Seemen , Harry Alles

Time-dependent density functional theory (TDDFT) is presently enjoying enormous popularity in quantum chemistry, as a useful tool for extracting electronic excited state energies. This article explains what TDDFT is, and how it differs from…

Materials Science · Physics 2007-05-23 Peter Elliott , Kieron Burke , Filipp Furche

Ab-initio density functional perturbation theory (DFPT) has been employed to study thermodynamical properties of pure and doped graphene sheet and the results have been compared with available theoretical and experimental data. The…

Mesoscale and Nanoscale Physics · Physics 2020-05-22 Sarita Mann , Pooja Rani , Ranjan Kumar , Girija S. Dubey , V. K. Jindal

We compare the performance of an approach using real frequency dependent polarizability to compute optical absorption spectra to linear-response time-dependent density functional theory (TD-DFT) for small organic dyes, oligomers of…

Materials Science · Physics 2018-05-22 Ang Siong Tuan , Amrita Pal , Sergei Manzhos

Microscopic quantum theory of nonlinear stimulated scattering of 2D Dirac particles in doped graphene on Coulomb field of impurity ions at the presence of an external strong coherent electromagnetic radiation is developed. We consider high…

Mesoscale and Nanoscale Physics · Physics 2017-10-27 A. K. Avetissian , A. G. Ghazaryan , Kh. V. Sedrakian , B. R. Avchyan