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The relationship between vacancy ordering and magnetism in TlFe1.6Se2 has been investigated via single crystal neutron diffraction, nuclear forward scattering, and transmission electron microscopy. The examination of chemically and…

We present a set of {\em optimum ground states} for a large class of spin-$\frac{3}{2}$ chains. Such global ground states are simultaneously ground states of the local Hamiltonian, i.e. the nearest neighbour interaction in the present case.…

Condensed Matter · Physics 2009-10-28 H. Niggemann , J. Zittartz

We study the ground state properties of the Heisenberg spin-1/2 chain with ferromagnetic nearest-neighbor and antiferromagnetic next-nearest-neighbor interactions using two approximate methods. One of them is the Jordan-Wigner mean-field…

Strongly Correlated Electrons · Physics 2009-11-11 D. V. Dmitriev , V. Ya. Krivnov

The fluctuations of the magnetic order parameter, or longitudinal spin excitations, are investigated theoretically in the ferromagnetic Fe and Ni as well as in the antiferromagnetic phase of the pnictide superconductor FeSe. The charge and…

Strongly Correlated Electrons · Physics 2020-07-01 Paweł Buczek , Nadine Buczek , Giovanni Vignale , Arthur Ernst

Exact ground state properties of antiferromagnetic Heisenberg spin rings with isotropic next neighbour interaction are presented for various numbers of spin sites and spin quantum numbers. Earlier work by Peierls, Marshall, Lieb, Schultz…

Statistical Mechanics · Physics 2009-10-31 K. Baerwinkel , H. -J. Schmidt , J. Schnack

First-principles calculations have been performed for different collinear magnetic orderings in orthorhombic manganites, such as HoMnO3, TbMnO3 and YMnO3, showing large GdFeO3-like distortions. Our results suggest that the AFM-E type…

Materials Science · Physics 2009-11-11 S. Picozzi , K. Yamauchi , G. Bihlmayer , S. Bluegel

Spin-crossover compounds, which are characterized by magnetic ions showing low-spin and high-spin states at thermally accessible energies, are ubiquitous in nature. We here focus on the effect of an exchange interaction on the collective…

Statistical Mechanics · Physics 2009-11-13 Carsten Timm , Charles J. Pye

We present a computationally efficient general first-principles based method for spin-lattice simulations for solids. Our method is based on a combination of atomistic spin dynamics and molecular dynamics, expressed through a spin-lattice…

Electronic structure calculations of the Verwey ground state of magnetite, Fe3O4, using density functional theory with treatment of on-site Coulomb interactions (DFT+U scheme) are reported. These calculations use the recently-published…

Strongly Correlated Electrons · Physics 2013-01-16 Mark Senn , Ingo Loa , Jon P. Wright , J. Paul Attfield

We study the nearest-neighbor Heisenberg antiferromagnet on a face-centered cubic lattice with arbitrary spin S. The model exhibits degenerate classical ground states including two collinear structures AF1 and AF3 described by different…

Strongly Correlated Electrons · Physics 2022-12-05 R. Schick , O. Götze , T. Ziman , R. Zinke , J. Richter , M. E. Zhitomirsky

The microscopic structure of spin-orbit fields for the technologically important Fe/GaAs interface is uncovered from first principles. A symmetry based method allows to obtain the spin-orbit fields---both their magnitude and…

Mesoscale and Nanoscale Physics · Physics 2013-09-18 Martin Gmitra , Alex Matos-Abiague , Claudia Draxl , Jaroslav Fabian

We investigated the reliability and applicability of so-called magnetic force linear response method to calculate spin-spin interaction strengths from first-principles. We examined the dependence on the numerical parameters including the…

Strongly Correlated Electrons · Physics 2018-03-28 Hongkee Yoon , Taek Jung Kim , Jae-Hoon Sim , Seung Woo Jang , Taisuke Ozaki , Myung Joon Han

Based on density functional calculations, we report on the orbital order and microscopic magnetic model of FeNCN, a prototype compound for orbital-only models. Despite having a similar energy scale, the spin and orbital degrees of freedom…

Strongly Correlated Electrons · Physics 2011-06-21 Alexander A. Tsirlin , Klaus Koepernik , Helge Rosner

We use the three-dimensional Heisenberg model with site randomness as an effective model of the compound Sr(Fe$_{1-x}$Mn$_x$)O$_2$. The model consists of two types of ions that correspond to Fe and Mn ions. The nearest-neighbor interactions…

Statistical Mechanics · Physics 2011-09-30 Ryo Tamura , Naoki Kawashima

We have found the exact ground state for a large class of antiferromagnetic spin-one chains with nearest and next-nearest neighbour interactions. The ground state is characterized as a matrix product of local site states and has the…

Condensed Matter · Physics 2009-10-22 C. Lange , A. Klümper , J. Zittartz

Recent inelastic neutron scattering (INS) measurements on FeSe and Fe(Te$_{1-x}$Se$_x$), have sparked intense debate over the nature of the ground state in these materials. Here we propose an effective bilinear-biquadratic spin model which…

Strongly Correlated Electrons · Physics 2017-11-09 Patricia Bilbao Ergueta , Wen-Jun Hu , Andriy H. Nevidomskyy

The electronic structure of the ground and some excited states of neutral atoms with the nuclear charge numbers $1\leq Z \leq 10$ and their single positive ions are investigated by means of our 2D mesh Hartree-Fock method for strong…

Atomic Physics · Physics 2009-10-31 M. V. Ivanov , P. Schmelcher

Quasiperiodic structures possess long range positional order, but are freed of constraints imposed by translational invariance. For spins interacting via Heisenberg couplings, one may expect therefore to find novel magnetic configurations…

Strongly Correlated Electrons · Physics 2008-10-15 Anuradha Jagannathan , Attila Szallas

Global minimum structures of neutral (Fe2O3)n clusters with n = 1-5 were determined employing the genetic algorithm in combination with ab initio parameterized interatomic potentials and subsequent refinement at the density functional…

Materials Science · Physics 2024-05-30 Andreas Erlebach , Carolin Hühn , Richard Jana , Marek Sierka

The ferrimagnetic phase of the sawtooth chain with mixed ferromagnetic nearest-neighbour interactions $J$ and antiferromagnetic next-nearest-neighbour interactions $J'$ (within the isotropic Heisenberg model) was previously characterized as…

Strongly Correlated Electrons · Physics 2023-04-04 Roman Rausch , Matthias Peschke , Cassian Plorin , Jürgen Schnack , Christoph Karrasch