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We study the influence of a linear energy bias on a non-equilibrium excitation on a chain of molecules coupled to local phonons (a tilted Holstein model) using both a random-walk rate kernel theory and a nonperturbative, massively…

Quantum Physics · Physics 2022-07-29 R. Kevin Kessing , Pei-Yun Yang , Salvatore R. Manmana , Jianshu Cao

Interacting electrons in a semiconductor quantum dot at strong magnetic fields exhibit a rich set of states, including correlated quantum fluids and crystallites of various symmetries. We develop in this paper a perturbative scheme based on…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Gun Sang Jeon , Chia-Chen Chang , Jainendra K. Jain

This paper describes a simple and general method for deriving the inelastic collision term in the electron Boltzmann equation for scattering from a coupled electron-phonon system, and applies the method to the case of doped polar…

Condensed Matter · Physics 2016-08-31 B. A. Sanborn

Phonon-related decoherence effects in a quantum double-well two-level subsystem coupled to a solid are studied theoretically by the example of deformation phonons. Expressions for the reduced density matrix at T=0 are derived beyond the…

Other Condensed Matter · Physics 2009-11-13 L. A. Openov

Density matrix perturbation theory [Niklasson and Challacombe, Phys. Rev. Lett. 92, 193001 (2004)] is generalized to canonical (NVT) free energy ensembles in tight-binding, Hartree-Fock or Kohn-Sham density functional theory. The canonical…

Chemical Physics · Physics 2015-12-09 Anders M. N. Niklasson , Marc J. Cawkwell , Emanuel H. Rubensson , Elias Rudberg

We investigate the influence of electron-phonon interactions on the dynamical properties of a quantum-dot-cavity QED system. We show that non-Markovian effects in the phonon reservoir lead to strong changes in the dynamics, arising from…

Mesoscale and Nanoscale Physics · Physics 2010-04-29 P. Kaer , T. R. Nielsen , P. Lodahl , A. -P. Jauho , J. Mork

We propose a fast and non-destructive spectroscopic method for single molecular ions that implements quantum logic schemes between an atomic ion and the molecular ion of interest. Our proposal relies on a hybrid coherent manipulation of the…

In this work, we investigate dispersion interactions in a selection of atomic, molecular, and molecule-surface systems, comparing high-level correlated methods with empirically-corrected density functional theory (DFT). We assess the…

Chemical Physics · Physics 2021-01-27 Tyler J. Hughes , Robert A. Shaw , Salvy P. Russo

Phonon anharmonicity is ubiquitous in real materials and is crucial for understanding thermal properties and phase stability. In this work, we show that anharmonic phonon modes can be obtained by maximizing their vibration stability during…

Materials Science · Physics 2026-05-15 Wenjing Li , Yong Lu , Fawei Zheng

We present an accurate and efficient formulation for the calculation of phonons in real-space Kohn-Sham density functional theory. Specifically, employing a local exchange-correlation functional, norm-conserving pseudopotential in the…

Chemical Physics · Physics 2023-03-30 Abhiraj Sharma , Phanish Suryanarayana

High-resolution electron energy loss spectroscopy measurements have been carried out on an optimally doped cuprate Bi2Sr2CaCu2O8+{\delta}. The momentum-dependent linewidth and the dispersion of an A1 optical phonon are obtained. Based on…

Strongly Correlated Electrons · Physics 2015-05-18 Huajun Qin , Junren Shi , Yanwei Cao , Kehui Wu , Jiandi Zhang , E. W. Plummer , J. Wen , Z. J. Xu , G. D. Gu , Jiandong Guo

The theory of the interaction of electrons with acoustic phonons in multilayer nitride-based AlN/GaN nanostructures was developed for the first time at $T\geqslant 0$ using the method of finite-temperature Green's functions and Dyson…

Mesoscale and Nanoscale Physics · Physics 2021-01-20 I. V. Boyko , M. R. Petryk

Exposing a molecule to intense light pulses may bring this molecule to a nonstationary quantum state, thus launching correlated dynamics of electronic and nuclear subsystems. Although much had been achieved in the understanding of…

Chemical Physics · Physics 2024-04-11 Nikolay V. Golubev , Jiří Vaníček

Optically active quantum dot molecules (QDMs) can host multi-spin quantum states with the potential for the deterministic generation of photonic graph states with tailored entanglement structures. Their usefulness for the generation of such…

We present an ab initio method for eletcronic structure calculations, which accounts for the interaction of electrons and magnons in ferromagnets. While it is based on a many body perturbation theory we approximate numerically complex…

Materials Science · Physics 2023-04-19 S. Paischer , G. Vignale , M. I. Katsnelson , A. Ernst , P. Buczek

Molecular polaritons have gained considerable attention due to their potential to control nanoscale molecular processes by harnessing electromagnetic coherence. Although recent experiments with liquid-phase vibrational polaritons have shown…

We investigate interactions between the proton spin, the deuteron spin, and the orbital angular momentum in the electronic ground state of the HD molecule. These interactions lead to hyperfine splittings of molecular energy levels. Our…

Chemical Physics · Physics 2020-07-29 Jacek Komasa , Mariusz Puchalski , Krzysztof Pachucki

We here introduce a Fortran code that computes anharmonic free energy of solids from first-principles based on our phonon quasiparticle approach. In this code, phonon quasiparticle properties, i.e., renormalized phonon frequencies and…

Materials Science · Physics 2019-06-19 Zhen Zhang , Dong-Bo Zhang , Tao Sun , Renata Wentzcovitch

We study theoretically the quantum optical properties of hybrid molecules composed of an individual quantum dot and a metallic nanoparticle. We calculate the resonance fluorescence of this hybrid system. Its incoherent part, the one arising…

Quantum Physics · Physics 2010-04-12 A. Ridolfo , O. Di Stefano , N. Fina , R. Saija , S. Savasta

In this work we describe a model for the exchange interaction of electrons, as it follows from the Pauli exclusion principle. Starting from Hartree-Fock theory and making use of the free electron-gas model we propose a simple scheme to…

Materials Science · Physics 2025-06-11 G. Schiwietz , P. L. Grande