Related papers: Magnetic octupole tensor decomposition and second-…
In this paper, we explore magneteoelectricity of rare earth orthochromites from the symmetry point of view. We determine the principal structural order parameters and find their couplings with ferroelectric and magnetic orderings. Our…
Multipole moments serve as order parameters for characterizing higher-order magnetic effects in momentum space, providing a framework to describe diverse magnetic responses by extending the concept of magnetism. In this letter, we introduce…
We show that the surface of a centrosymmetric, collinear, compensated antiferromagnet, which hosts bulk ferroically ordered magnetic octupoles, exhibits a linear magnetoelectric effect, a net magnetization, and a net electric dipole moment.…
d-wave altermagnets have magnetic octupoles as their order parameters [Phys. Rev. X 14, 011019 (2024)]. We theoretically show that magnetic octupoles injected from outside generate torque on the d-wave altermagnets. The injection can be…
Recent experiments on URu2Si2 show that the low-pressure hidden order is non-magnetic but it breaks time reversal invariance. Restricting our attention to local order parameters of 5f2 shells, we find that the best candidate for hidden…
Motivated by the recent discovery of anomalously large magnetic response of chiral phonons in dipolar magnets, we explore an extension to study Einstein quantum phonon modes coupled to multipolar moments. We consider the case of non-Kramers…
We present a thorough density functional theory study of the magneto-electric (ME) effect in Cr$_{2}$O$_{3}$. The spin-lattice ME tensor $\alpha$ was determined in the low-field and spin flop (SF) phases, using the method of dynamical…
We study the multiferroic properties in the distorted tetrahedral quasi-one dimensional spin system Cu$_3$Mo$_2$O$_9$, in which the effects of the low dimensionality and the magnetic frustration are expected to appear simultaneously. We…
Using first principles calculations, we study the microscopic origin of ferroelectricity (FE) induced by magnetic order in the orthorhombic HoMnO3. We obtain the largest ferroelectric polarization observed in the whole class of improper…
Magnetoelectrics often possess ions located in noncentrosymmetric surroundings. Based on this fact we suggest a microscopic model of magnetoelectric interaction and show that the spin-orbit coupling leads to spin-dependent electric dipole…
We combine the anisotropy of magnetic interactions and the point symmetry of finite solids in the study of dipolar clusters as new basic units for multiferroics metamaterials. The hamiltonian of magnetic dipoles with an easy axis at the…
In the electromagnetic multipole expansion, magnetic octupoles are the subsequent order of magnetic multipoles allowed in centrosymmetric systems, following the more commonly observed magnetic dipoles. As order parameters in condensed…
We have investigated the dielectric anomalies associated with spin ordering transitions in the tetragonal spinel Mn$_3$O$_4$, using thermodynamic, magnetic, and dielectric measurements. We find that two of the three magnetic ordering…
We clarify that the antiferromagnetic order in the distorted tetrahedral quasi-one dimensional spin system induces electric polarizations. In this system, the effects of the low dimensionality and the magnetic frustration are expected to…
Detecting symmetry-breaking hidden orders with conventional probes has been a long-standing challenge in the field of magnetism. Higher-rank multipolar ordering $-$ anisotropic charge and magnetization distributions arising from a…
Two-dimensional (2D) multiferroic materials are ideal systems for exploring new coupling mechanisms between different ferroic orders and producing novel quantum phenomena with potential applications. We employed first-principles density…
Within Landau theory, magnetism and polarity are homotopic, displaying a one-to-one correspondence between most physical characteristics. However, despite widely reported noncollinear magnetism, spontaneous noncollinear electric dipole…
Chiral magnets, which break both spatial inversion and time reversal symmetries, carry a potential for quadratic optical responses. Despite the possibility of enhanced and controlled responses through the magnetic degree of freedom, the…
Quantum magnets with spin $J=2$, which arise in spin-orbit coupled Mott insulators, can potentially display multipolar orders. We carry out an exact diagonalization study of a simple octahedral crystal field Hamiltonian for two electrons,…
A ferroaxial ordering, which appears without mirror symmetry parallel to an electric axial moment, is described by a ferroic alignment of the electric toroidal (ET) dipole rather than the conventional electric and magnetic dipoles. Although…