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We introduce a method for determining the sensitivity of any given Entangled Two-Photon Absorption (ETPA) measurement. By modeling all signal and noise contributions to the measurement, we derive a single numerical value that describes the…

Quantum Physics · Physics 2025-12-23 René Pollmann , Franz Roeder , Christine Silberhorn , Benjamin Brecht

We draw an intuitive picture of the spatio-temporal properties of the entangled state of twin photons, where they are described as classical wave-packets. This picture predicts a precise relation between their temporal and transverse…

Quantum Physics · Physics 2014-05-29 Alessandra Gatti , Lucia Caspani , Tommaso Corti , Enrico Brambilla , Ottavia Jedrkiewicz

It is well known that photons can carry a spatial structure akin to a "twisted" or "rippled" wavefront. Such structured light fields have sparked significant interest in both classical and quantum physics, with applications ranging from…

The ability to use the temporal and spatial degrees of freedom of quantum states of light to encode and transmit information is crucial for the implementation of a robust and efficient quantum network. In particular, the large…

Quantum Physics · Physics 2023-10-31 Gaurav Nirala , Siva T. Pradyumna , Ashok Kumar , Alberto M. Marino

We experimentally demonstrate amplitude and phase modulation of a time-energy entangled two-photon wave function. The entangled photons are produced by spontaneous parametric down-conversion, spectrally dispersed in an prism compressor,…

Quantum Physics · Physics 2009-01-23 F. Zäh , M. Halder , T. Feurer

Sources of photons with controllable quantum properties such as entanglement and squeezing are desired for applications in quantum information, metrology, and sensing. However, fine-grained control over these properties is hard to achieve,…

We experimentally demonstrate two-photon absorption (TPA) with broadband down-converted light (squeezed vacuum). Although incoherent and exhibiting the statistics of a thermal noise, broadband down-converted light can induce TPA with the…

Quantum Physics · Physics 2011-12-06 Barak Dayan , Avi Pe'er , Asher A. Friesem , Yaron Silberberg

We investigate one- and two-photon absorption in twisted bilayer graphene (TBLG) by examining the effects of tuning the twist angle $ \theta $ and the excitation energy $ E_l $ on its absorption coefficients $ \alpha_{i=1,2}$. We find that…

Mesoscale and Nanoscale Physics · Physics 2024-12-25 Disha Arora , Deepanshu Aggarwal , Sankalpa Ghosh , Rohit Narula

Quantum light spectroscopy, providing novel molecular information non-accessible by classical light, necessitates new computational tools when applied for complex molecular systems. We introduce two computational protocols for the molecular…

Chemical Physics · Physics 2021-09-14 Bing Gu , Daniel Keefer , Shaul Mukamel

Nonlinear absorption can limit the efficiency of nonlinear optical devices. However, it can also be exploited for optical limiting or switching applications. Thus, characterization of nonlinear absorption in photonic devices is imperative.…

A quantum system composed of two or more subsystems can be in an entangled state, i.e. a state in which the properties of the global system are well defined but the properties of each subsystem are not. Entanglement is at the heart of…

Despite the now vast body of two-dimensional materials under study, bilayer graphene remains unique in two ways: it hosts a simultaneously tunable band gap and electron density; and stems from simple fabrication methods. These two…

Mesoscale and Nanoscale Physics · Physics 2016-07-19 M. K. Brinkley , D. S. L. Abergel , B. D. Clader

We present an analytical quantum theoretic model for non-resonant molecular two-photon absorption (TPA) of broadband, spectrally multi-mode squeezed vacuum, including low-gain (isolated entangled photon pairs or EPP) and high-gain (bright…

Quantum Physics · Physics 2022-08-10 Michael G. Raymer , Tiemo Landes

We explore, both experimentally and theoretically, the propagation dynamics of spatially entangled photon pairs (biphotons). Characterization of entanglement is done via the Schmidt number, which is a universal measurement of the degree of…

Optics · Physics 2017-06-28 Matthew Reichert , Xiaohang Sun , Jason W. Fleischer

We study theoretically the strong-field absorption of an ultrafast optical pulse by a gapped graphene monolayer. At low field amplitudes, the absorbance in the pristine graphene is equal to the universal value of $2.3$ percent. Although the…

Mesoscale and Nanoscale Physics · Physics 2020-05-06 S. Azar Oliaei Motlagh , Ahmal Jawad Zafar , Aranyo Mitra , Vadym Apalkov , Mark I. Stockman

We implement a double-pixel, compressive sensing camera to efficiently characterize, at high resolution, the spatially entangled fields produced by spontaneous parametric downconversion. This technique leverages sparsity in spatial…

Quantum Physics · Physics 2013-02-25 Gregory A. Howland , John C. Howell

We report on the dynamics of photodegradation and subsequent recovery of two-photon fluorescence in a dye-doped polymer. The energy dependence suggests that photo-degradation is a linear process while recovery is entropic. Such recovery…

Optics · Physics 2009-11-13 Ye Zhu , Juefei Zhou , Mark G. Kuzyk

We use a non-perturbative theoretical approach to the parametric down-conversion (PDC) process, which generates entangled-photon field for an arbitrarily strong pump-pulse. This approach can be used to evaluate multi-point field correlation…

Chemical Physics · Physics 2025-10-22 Deependra Jadoun , Upendra Harbola , Vladimir Y. Chernyak , Shaul Mukamel

Ultrafast optical spectroscopy is a powerful technique for studying the dynamic processes of molecular systems in condensed phases. However, in molecular systems containing many dye molecules, the spectra can become crowded and difficult to…

Chemical Physics · Physics 2025-02-05 Yuta Fujihashi , Akihito Ishizaki , Ryosuke Shimizu

We formulate a theory for entangled imaging, which includes also the case of a large number of photons in the two entangled beams. We show that the results for imaging and for the wave-particle duality features, which have been demonstrated…

Quantum Physics · Physics 2009-11-07 A. Gatti , E. Brambilla , L. A. Lugiato