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The control of spin-orbit coupling (SOC) at the microscopic level has become a major research quest within the magnetism and spintronics communities. Altering the interaction between the spin and orbital degrees of freedom can fundamentally…

Mesoscale and Nanoscale Physics · Physics 2015-06-19 James H. Atkinson , Ross Inglis , Enrique del Barco , Euan K. Brechin

Magnetism in transition metal compounds is usually considered starting from a description of isolated ions, as exact as possible, and treating their (exchange) interaction at a later stage. We show that this standard approach may break down…

Strongly Correlated Electrons · Physics 2016-10-24 S. V. Streltsov , D. I. Khomskii

Ferromagnetism in the two-dimensional CrI$_3$ has generated a lot of excitement, and it was recently proposed that the spin-orbit coupling (SOC) in Iodine may generate bond-dependent spin interactions leading to magnetic anisotropy. Here we…

Strongly Correlated Electrons · Physics 2021-03-17 P. Peter Stavropoulos , Xiaoyu Liu , Hae-Young Kee

The origin of magnetic anisotropy in magnetic compounds is a longstanding issue in solid state physics and nonmagnetic ligand ions are considered to contribute little to magnetic anisotropy. Here, we introduce the concept of ligand driven…

Magnetic anisotropy (MA) is one of the most important material properties for modern spintronic devices. Conventional manipulation of the intrinsic MA, i.e. magnetocrystalline anisotropy (MCA), typically depends upon crystal symmetry.…

Materials composed of two dimensional layers bonded to one another through weak van der Waals interactions often exhibit strongly anisotropic behaviors and can be cleaved into very thin specimens and sometimes into monolayer crystals.…

Materials Science · Physics 2017-04-28 Michael A. McGuire

We present a detailed study on the microscopic origin of magnetism in suspended and dielectrically embedded CrI$_3$ monolayer. To this end, we down-fold two distinct minimal generalized Hubbard models with different orbital basis sets from…

Strongly Correlated Electrons · Physics 2021-10-06 D. Soriano , A. N. Rudenko , M. I. Katsnelson , M. Rösner

After the discovery of magnetism in monolayer CrI3, the magnetic properties of different 2D materials from the chromium-trihalide family are intuitively assumed to be similar, yielding magnetic anisotropy from the spin-orbit coupling on…

Mesoscale and Nanoscale Physics · Physics 2021-03-24 C. Bacaksiz , D. Šabani , R. M. Menezes , M. V. Milošević

Spin-orbit coupling (SOC), the core of numerous condensed-matter phenomena such as nontrivial band gap, magnetocrystalline anisotropy, etc, is generally considered to be appreciable only in heavy elements, detrimental to the synthetization…

Materials Science · Physics 2022-02-21 Jiayu Li , Qiushi Yao , Lin Wu , Zongxiang Hu , Boya Gao , Xiangang Wan , Qihang Liu

The coexistence of the strongly correlated 3$d$ transition metal (TM) atom and the strong spin-orbit coupling (SOC) of 5$d$ TM atom is potential to host exotic physical phenomena. In the present work, we have studied the magnetism resulting…

Strongly Correlated Electrons · Physics 2020-02-19 Shreemoyee Ganguly , Sayantika Bhowal

Monolayers of molybdenum disulfide (MoS2) are the most studied two-dimensional (2D) transition-metal dichalcogenides (TMDs), due to its exceptional optical, electronic, and opto-electronic properties. Recent studies have shown the…

Based on first-principles calculations, the evolution of the electronic and magnetic properties of transition metal dihalides MX$_2$ (M= V, Mn, Fe, Co, Ni; X = Cl, Br, I) is analyzed from the bulk to the monolayer limit. A variety of…

Strongly Correlated Electrons · Physics 2019-04-17 Antia S. Botana , Michael R. Norman

We theoretically describe a mechanism of low-field linear magnetoconductivity in helical magnetic metals. Two ingredients for the mechanism in three-dimensional metals are identified to be the spin-orbit coupling and momentum-dependent…

Mesoscale and Nanoscale Physics · Physics 2022-09-28 Vladimir A. Zyuzin

Magnetism in doped transition metal dichalcogenide monolayers and van der Waals interfaced materials have motivated the search for sustainable magnetic states at the nanoscale with the prospect of building devices for spintronics…

Materials Science · Physics 2025-08-05 Rohin Sharma , Diem Thi-Xuan Dang , Lilia M. Woods

We analyze magnetic phases of monolayers of transition metal dichalcogenides that are two-valley materials with electron-electron interactions. The exchange inter-valley scattering makes two-valley systems less stable to the spin…

Strongly Correlated Electrons · Physics 2019-07-31 Dmitry Miserev , Jelena Klinovaja , Daniel Loss

A supposedly nonmagnetic 5d$^1$ double perosvkite oxide is investigated by a combination of spectroscopic and theoretical methods, namely resonant inelastic X-ray scattering, X-ray absorption spectroscopy, magnetic circular dichroism, and…

The discovery of an ever increasing family of atomic layered magnetic materials, together with the already established vast catalogue of strong spin-orbit coupling (SOC) and topological systems, calls for some guiding principles to tailor…

Materials Science · Physics 2021-10-13 Hidekazu Kurebayashi , Jose H. Garcia , Safe Khan , Jairo Sinova , Stephan Roche

Two dimensional magnetic materials, with tunable electronic properties could lead to new spintronic, magnetic and magneto-optic applications. Here, we explore intrinsic magnetic ordering in two dimensional monolayers of transition metal…

Understanding of the intimate cross-coupling between electric and magnetic degrees of freedom in solids usually requires sophisticated models and time-consuming calculation methods. Instead of macroscopic symmetry analysis, we present a…

Materials Science · Physics 2022-02-02 Maocai Pi , Xifan Xu , Mingquan He , Yisheng Chai

Magnetoelasticity plays a crucial role in numerous magnetic phenomena, including magnetocalorics, magnon excitation via acoustic waves, and ultrafast demagnetization/Einstein-de Haas effect. Despite a long-standing discussion on…

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