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Aqueous solutions of LiCl are probably the most studied electrolyte solutions related to the complexity of liquid water at low temperatures. Despite the large amount of available experimental data hardly any computational studies were…

Soft Condensed Matter · Physics 2020-04-29 Philip H. Handle

We studied the liquid-glass transition of $SiO_2$ by means of replica theory, utilizing an effective pair potential which was proved to reproduce a few experimental features of silica. We found a finite critical temperature $T_0$, where the…

Condensed Matter · Physics 2009-11-07 B. Coluzzi , P. Verrocchio

Liquid crystals are phases of matter intermediate between crystals and liquids. Whereas classical liquid crystals have been known for a long time and are used in electro-optical displays, much less is known about their quantum counterparts.…

Quantum Gases · Physics 2016-01-12 Zhigang Wu , Jens K. Block , Georg M. Bruun

Liquid-gas phase transition in statistical mechanics is a long-standing dilemma not yet well explained. In this paper we propose a novel approach to this dilemma, by: 1). Putting forth a new space homogeneity assumption. 2). Giving a new…

Statistical Mechanics · Physics 2007-05-23 Yuan-Xing Gui

In equilibrium and supercooled liquids, polymorphism is manifested by thermodynamic regions defined in the phase diagram, which are predominantly of different short- and medium-range order (local structure). It is found that on the phase…

Soft Condensed Matter · Physics 2024-03-19 Anatolii V. Mokshin , Roman V. Vlasov

Demixing of binary liquids is a ubiquitous transition, which is explained using a well-established thermodynamic formalism that requires equality of intensive thermodynamics parameters across the phase boundaries. Demixing transitions also…

Two-dimensional (2D) solid-liquid transition (SLT)~\cite{Mermin1966Absence,Mermin1968Crystalline,Kosterlitz1972Long} concerns fundamental concepts of long-range correlations vital to magnetism, superconductivity, superfluidity, and…

Strongly Correlated Electrons · Physics 2018-02-28 Jian Huang , Talbot Knighton , Zhe Wu , Alessandro Serafin , J. S. Xia L. N. Pfeiffer , K. W. West

Recent imaging experiments show a surprisingly robust regime of liquid-solid phase coexistence in a 2D electron system near the quantum melting/freezing transition, with the two phases mixed in mesoscopic domains. Strikingly, the…

Strongly Correlated Electrons · Physics 2025-02-18 Sandeep Joy , Brian Skinner

The study of liquid-liquid phase transition has attracted considerable attention. One interesting example of such phenomenon is phosphorus for which the existence a first-order phase transition between a low density insulating molecular…

Soft Condensed Matter · Physics 2021-08-25 Manyi Yang , Tarak Karmakar , Michele Parrinello

We studied dielectric properties of nano-sized liquid water samples confined in polymerized silicates MCM-41 characterized by the porous sizes \sim 3-10nm. We report the direct measurements of the dielectric constant by the dielectric…

Soft Condensed Matter · Physics 2015-05-27 P. O. Fedichev , L. I. Menshikov , G. S. Bordonskiy , A. O. Orlov

Effect of confinement on the liquid-liquid transition of water are studied by simulations in the Gibbs ensemble. Upon cooling along the liquid-vapor coexistence curve, confined water undergoes transition from normal to strongly tetrahedral…

Soft Condensed Matter · Physics 2007-05-23 Ivan Brovchenko , Alla Oleinikova

We find that a system of particles interacting through a simple isotropic potential with a softened core is able to exhibit a rich phase behavior including: a liquid-liquid phase transition in the supercooled phase, as has been suggested…

Soft Condensed Matter · Physics 2009-10-31 G. Malescio , G. Pellicane

We have developed a scaled parametric equation of state to describe and predict thermodynamic properties of supercooled water. The equation of state, built on the growing evidence that the critical point of supercooled liquid-liquid water…

Soft Condensed Matter · Physics 2007-05-23 M. A. Anisimov , D. A. Fuentevilla

The overlap, or similarity, between liquid configurations is at the core of the mean-field description of the glass transition, and remains a useful concept when studying three-dimensional glass-forming liquids. In liquids, however, the…

Statistical Mechanics · Physics 2021-01-05 Benjamin Guiselin , Gilles Tarjus , Ludovic Berthier

The thermodynamic properties of the supercooled liquid state of the mW model of water show anomalous behavior. Like in real water, the heat capacity and compressibility sharply increase upon supercooling. One of the possible explanations of…

Chemical Physics · Physics 2013-05-02 Vincent Holten , David T. Limmer , Valeria Molinero , Mikhail A. Anisimov

A revised phase diagram for water shows three distinct fluid phases. There is no continuity of liquid and gas and no critical point on Gibbs density surface. A liquid state, water, spans all temperatures. A thermodynamic rigidity function,…

Statistical Mechanics · Physics 2013-08-22 Leslie V. Woodcock

Structurally disordered materials continue to pose fundamental questions, including that of how different disordered phases ("polyamorphs") can coexist and transform from one to another. As a widely studied case, amorphous silicon (a-Si)…

Using molecular dynamics simulations we analyze the dynamics of two atomic liquids that display a liquid-liquid phase transition (LLPT): Si described by the Stillinger-Weber potential and Ga as modeled by the modified embedded-atom model…

Statistical Mechanics · Physics 2015-06-17 Samuel Cajahuaringa , Maurice de Koning , Alex Antonelli

We show that the existence of an intermediate phase between the Fermi liquid and the Wigner crystal phases is a generic property of the two-dimensional pure electron liqd in MOSFET's at zero temperature. The physical reason for the…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 B. Spivak

Twenty years ago Poole et al. (Nature 360, 324, 1992) suggested that the anomalous properties of supercooled water may be caused by a critical point that terminates a line of liquid-liquid separation of lower-density and higher-density…

Chemical Physics · Physics 2017-08-14 V. Holten , M. A. Anisimov