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Different insulator phases compete with each other in strongly correlated materials with simultaneous local and non-local interactions. It is known that the homogeneous Mott insulator converts into a charge density wave (CDW) phase when the…

Compression of UV femtosecond laser pulses focused into a gas cell filled with xenon is reported numerically. With a large negative Kerr index and normal dispersion, xenon promotes temporal modulational instability (MI) which can be…

Optics · Physics 2010-02-03 L. Berge , C. Koehler , S. Skupin

The use of few-femtosecond, extreme ultraviolet (XUV) pulses, produced by high-order harmonic generation, in combination with few-femtosecond infrared (IR) pulses in pump-probe experiments has great potential to disclose ultrafast dynamics…

Non-destructive cross-sectional characterization of materials systems with a resolution in the nanometer range and the ability to allow for time-resolved in-situ studies is of great importance in material science. Here, we present such a…

Core excitons in solids have garnered increasing interest, yet their behavior and decay mechanisms are not fully understood. Here, we use attosecond extreme ultraviolet (XUV) transient absorption spectroscopy, performed with a broadband…

Materials Science · Physics 2023-11-07 Rafael Quintero-Bermudez Stephen R. Leone

Photoexcitation of van der Waals complexes can lead to several decay pathways depending on the nature of the potential energy surfaces. Upon excitation of a chromophore in a complex, ionization of its weakly bound neighbour via energy…

Chemical Physics · Physics 2022-01-14 Namitha Brijit Bejoy , Nitin. K Singh , Balanarayan Pananghat , G. Naresh Patwari

Low-energy-electron emission from resonant Auger final states via intermolecular Coulombic decay (RA-ICD) has been previously described as a promising scenario for controlling radiation damage for medical purposes, but has so far only been…

The decay of core-excited states is a sensitive probe of autoionization dynamics and correlation effects in many-electron systems, occurring on the fastest timescales. Xenon, with its dense manifold of autoionizing resonances that can be…

The goal to control short-wavelength radiation for the investigation and manipulation of ultrafast dynamics in quantum systems coevolves with the growing availability of extreme-ultraviolet (XUV) and x-ray sources from high-harmonic…

Coulomb explosion imaging (CEI) is a powerful technique for capturing the real-time motion of individual atoms during ultrafast photochemical reactions. CEI generates high-dimensional data with naturally embedded correlations that allow…

Infrared (IR) spectroscopy can be used as an important and effective tool for probing periodic networks of quantum wires or nanotubes (quantum crossbars, QCB) at finite frequencies far from the Luttinger liquid fixed point. Plasmon…

Strongly Correlated Electrons · Physics 2009-11-10 I. Kuzmenko , S. Gredeskul , K. Kikoin , Y. Avishai

We resolve the real-time electric field of a femtosecond third-order nonlinear optical signal in the molecular frame. The electric field emitted by the induced third-order polarization from impulsively pre-aligned gas-phase molecules at…

We present a method for a complete characterization of a femtosecond ultraviolet pulse when a fundamental near-infrared beam is also available. Our approach relies on generation of second harmonic from the pre-characterized fundamental,…

Optics · Physics 2009-07-09 Marcin Kacprowicz , Wojciech Wasilewski , Konrad Banaszek

Ultralight bosonic dark matter (UBDM) can be described by a classical wave-like field oscillating near the Compton frequency of the bosons. If a measurement scheme for the direct detection of UBDM interactions is sensitive to a signature…

High-resolution measurements of angular scattering distributions provide a sensitive test for theoretical descriptions of collision processes. Crossed beam experiments employing a decelerator and velocity map imaging have proven successful…

We demonstrate a femtosecond enhancement cavity with a crossed-beam geometry for efficient generation and extraction of extreme-ultraviolet (XUV) frequency combs at a 154 MHz repetition rate. We achieve a record-high out-coupled power of…

A high-performance fast response deep ultraviolet (UV) photodetectors with interdigitated Ti/Au planar electrodes using a lithography technology has fabricated on homoepitaxial diamond. The device shows a high ultraviolet photocurrent at…

Instrumentation and Detectors · Physics 2020-02-07 Le Li

Inorganic molecular materials such as tin oxo cages are a promising generation of photoresists compatible with the demands of the recently developed Extreme UltraViolet (EUV) lithography technology. Therefore, a detailed understanding of…

Photoelectron circular dichroism (PECD) is a highly sensitive enantiospecific spectroscopy for studying chiral molecules in the gas phase using either single-photon ionization or multiphoton ionization. In the short pulse limit investigated…

The dynamics of autoionizing Rydberg states of oxygen are studied using attosecond transient absorption technique, where extreme ultraviolet (XUV) initiates molecular polarization and near infrared (NIR) pulse perturbs its evolution.…

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