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Strong coupling of molecular vibrations with light creates polariton states, enabling control over many optical and chemical properties. However, the near-field signatures of strong coupling are difficult to map as most cavities are closed…

The possibility of strong coupling between a single molecule and surface plasmons is analyzed on the basis of a microscopic classical description. It is predicted that strong single molecule - plasmon coupling can happen for a silver…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Mykhaylo M. Dvoynenko

Here we study subwavelength gratings for coupling into graphene plasmons by means of an an- alytical model based on transformation optics that is not limited to very shallow gratings. We consider gratings that consist of a periodic…

Mesoscale and Nanoscale Physics · Physics 2016-05-04 Paloma A. Huidobro , Matthias Kraft , Ren Kun , Stefan A. Maier , John B. Pendry

Graphene can support surface plasmons with higher confinement, lower propagation loss, and substantially more tunable response compared to usual metal-based plasmonic structures. Interestingly, plasmons in graphene can strongly couple with…

Optics · Physics 2023-08-03 Tianjing Guo , Christos Argyropoulos

We study the strong coupling between the molecular excited state and the plasmonic modes of silver hole arrays with a resonant frequency very close to the asymptotic line of the plasmonic dispersion relation, at the nonlinear regime. We…

Mesoscale and Nanoscale Physics · Physics 2017-01-26 Lihi Efremushkin , Maxim Sukharev , Adi Salomon

Strongly coupled plasmon-exciton systems offer promising applications in nanooptics. The classification of the coupling regime is currently debated both from experimental and theoretical perspectives. We present a method to unambiguously…

Mesoscale and Nanoscale Physics · Physics 2023-07-19 Felix Stete , Wouter Koopman , Matias Bargheer

The interaction between excited states of a molecule and excited states of metal nanostructure (e.g. plasmons) leads to hybrid states with modified optical properties. When plasmon resonance is swept through molecular transition frequency…

Chemical Physics · Physics 2022-05-04 Monosij Mondal , Maicol A. Ochoa , Maxim Sukharev , Abraham Nitzan

We extend the model of exciton-plasmon materials to include a ro-vibrational structure of molecules using wave-packet propagations on electronic potential energy surfaces. The new model replaces conventional two-level emitters with more…

Mesoscale and Nanoscale Physics · Physics 2017-08-18 Maxim Sukharev , Eric Charron

Here we present the theoretical foundation of the strong coupling phenomenon between quantum emitters and propagating surface plasmons observed in two-dimensional metal surfaces. For that purpose, we develop an ab-initio quantum framework…

Mesoscale and Nanoscale Physics · Physics 2013-04-11 A. Gonzalez-Tudela , P. A. Huidobro , L. Martin-Moreno , C. Tejedor , F. J. Garcia-Vidal

We demonstrate strong coupling between molecular excited states and surface plasmon modes of a slit array in a thin metal film. The coupling manifests itself as an anti-crossing behavior of the two newly formed polaritons. As the coupling…

Mesoscale and Nanoscale Physics · Physics 2012-08-17 Adi Salomon , Robert J. Gordon , Yehiam Prior , Tamar Seideman , Maxim Sukharev

In this review we look at the concepts and state-of-the-art concerning the strong coupling of surface plasmon-polariton modes to states associated with quantum emitters such as excitons in J-aggregates, dye molecules and quantum dots. We…

Optics · Physics 2015-01-19 P. Törmä , W. L. Barnes

The resonant scattering of surface plasmon-polariton waves by embedded semiconductor quantum dots above the dielectric/metal interface is explored in the strong-coupling regime. In contrast to non-resonant scattering by a localized…

Mesoscale and Nanoscale Physics · Physics 2015-06-19 Danhong Huang , Michelle Easter , Godfrey Gumbs , A. A. Maradudin , Shawn-Yu Lin , Dave Cardimona , Xiang Zhang

Strong coupling between light and molecular matter is currently attracting interest both in chemistry and physics, in the fast-growing field of molecular polaritonics. The large near-field enhancement of the electric field of plasmonic…

Mesoscale and Nanoscale Physics · Physics 2024-10-03 Álvaro Buendía , Jose A. Sánchez-Gil , Vincenzo Giannini , William L. Barnes , Marie S. Rider

Guided-mode resonances in diffraction gratings are manifested as peaks (dips) in reflection (transmission) spectra. Smaller resonance line widths (higher Q-factors) ensure stronger light-matter interactions and are beneficial for…

Molecular polaritons are hybrid states of photonic and molecular character that form when molecules strongly interact with light. Strong coupling tunes energy levels and importantly, can modify molecular properties (e.g. photoreaction…

Chemical Physics · Physics 2023-02-14 Francesca Fassioli , Kyu Hyung Park , Sarah E. Bard , Gregory D. Scholes

We use molecules to couple light into and out of microscale plasmonic waveguides. Energy transfer, mediated by surface plasmons, from donor molecules to acceptor molecules over ten micrometer distances is demonstrated. Also surface plasmon…

We examine the coupling of electromagnetic waves incident normal to a thin silver film that forms an oscillatory grating embedded between two otherwise uniform, semi-infinite half spaces. Two grating structures are considered, in one of…

Optics · Physics 2009-07-23 M. Sukharev , P. R. Sievert , T. Seideman , J. B. Ketterson

We present a quantum theory for the interaction of a two level emitter with surface plasmon polaritons confined in single-mode waveguide resonators. Based on the Green's function approach, we develop the conditions for the weak and strong…

Mesoscale and Nanoscale Physics · Physics 2015-03-20 T. Hümmer , F. J. García-Vidal , L. Martín-Moreno , D. Zueco

The ability of curved gratings as sectors of concentric circular gratings to couple linearly polarized light into focused surface plasmons is investigated by theory, simulation and experiment. Curved gratings, as sectors of concentric…

We theoretically investigate dispersion of plasma waves propagating in a lateral plasmonic crystal based on a two-dimensional electron system with grating gates. Two specific configurations are analyzed: a system with single grating gate…

Mesoscale and Nanoscale Physics · Physics 2026-01-27 I. V. Gorbenko , P. A. Gusikhin , V. Yu. Kachorovskii , V. M. Muravev
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