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We demonstrate the ability to control and shape the spectro-temporal content of extreme-ultraviolet (XUV) pulses produced by a seeded free-electron laser (FEL). The control over the spectro-temporal properties of XUV light was achieved by…

New experimental techniques based on non-linear ultrafast spectroscopies have been developed over the last few years, and have been demonstrated to provide powerful probes of quantum dynamics in different types of molecular aggregates,…

We describe an experiment to measure the emitted real-time electric field from an ultrafast third-order nonlinear optical interaction in molecules, using a phase-tracked spectral interferometry scheme. By combining a software lock-in…

Optics · Physics 2025-03-11 Siddhant Pandey , Francis Walz , Niranjan Shivaram

We report on the implementation of a time-multiplexed click detection scheme to probe quantum correlations between different spatial optical modes. We demonstrate that such measurement setups can uncover nonclassical correlations in…

Quantum Physics · Physics 2015-07-08 J. Sperling , M. Bohmann , W. Vogel , G. Harder , B. Brecht , V. Ansari , C. Silberhorn

Fourier synthesis is one of the foundations of physical optics. Spatial Fourier optics is a basis for understanding optical imaging, microscopy, and holography. In conventional Fourier optics, the complex spatial field distribution in the…

Optics · Physics 2025-04-29 Murat Yessenov , Ayman F. Abouraddy

Suppose we measure the time-dependent spectrum of a single photon. That is, we first send the photon through a set of frequency filters (which we assume to have different filter frequencies but the same finite bandwidth $\Gamma$), and then…

Quantum Physics · Physics 2017-09-27 S. J. van Enk

We introduce the concept of coherent temporal imaging and its combination with the anamorphic stretch transform. The new system can measure both temporal profile of fast waveforms as well as their spectrum in real time and at…

Optics · Physics 2013-11-05 Mohammad H. Asghari , Bahram Jalali

We propose, analyze, and evaluate a technique for the joint measurement of time-frequency entanglement between two photons. In particular, we show that the frequency sum and time difference of two photons could be simultaneously measured…

Quantum Physics · Physics 2020-06-15 Han Liu , Amr S. Helmy

We present a sensing scheme for estimating the frequency difference of two non-entangled photons. The technique consists of time-resolving sampling measurements at the output of a beam splitter. With this protocol, the frequency shift…

Quantum Physics · Physics 2025-12-10 Luca Maggio , Danilo Triggiani , Paolo Facchi , Vincenzo Tamma

Quantum mechanics ascribes to the ground state of the electromagnetic radiation zero-point electric field fluctuations that permeate empty space at all frequencies. No energy can be extracted from the ground state of a system and,…

We study light absorption in many-electron interacting systems beyond the linear regime by using a {\em single} broadband impulse of an electric field in the instantaneous limit. We determine non-pertubatively the absorption cross section…

Chemical Physics · Physics 2021-04-20 Alberto Guandalini , Caterina Cocchi , Stefano Pittalis , Alice Ruini , Carlo Andrea Rozzi

In recent years, electro-optic sampling, which is based on Pockel's effect between an electromagnetic mode and a copropagating, phase-matched ultrashort probe, has been largely used for the investigation of broadband quantum states of…

Quantum Physics · Physics 2023-10-03 Francesca Fabiana Settembrini , Alexa Herter , Jèrôme Faist

Measuring an electric field waveform beyond radio frequencies is often accomplished via a second-order nonlinear interaction with a laser pulse shorter than half of the field's oscillation period. However, synthesizing such a gate pulse is…

The novel camera architecture facilitates the development of machine vision. Instead of capturing frame sequences in the temporal domain as traditional video cameras, FourierCam directly measures the pixel-wise temporal spectrum of the…

Image and Video Processing · Electrical Eng. & Systems 2020-11-02 Chengyang Hu , Honghao Huang , Minghua Chen , Sigang Yang , Hongwei Chen

The characterization of the complex spectral amplitude that is, the spectrum and spectral phase, of single-photon-level light fields is a crucial capability for modern photonic quantum technologies. Since established pulse characterisation…

Combined spectrally and time resolved measurements provide information not otherwise available if performed in either domain alone. We demonstrate a new approach to Four Wave Mixing spectroscopy, where spectral selectivity is achieved by…

Optics · Physics 2015-05-13 Yuri Paskover , Andrey Shalit , Yehiam Prior

We consider ramifications of the use of high speed light modulators to questions of correlation and measurement of time-energy entangled photons. Using phase modulators, we find that temporal modulation of one photon of an entangled pair,…

Quantum Physics · Physics 2009-11-13 S. E. Harris

A quantum memory for light is expected to play a crucial role in quantum communication protocols and distributed quantum computing. In addition to storage and buffering, a quantum memory can be used for manipulations of stored states to…

Quantum Physics · Physics 2025-10-09 Ankit Papneja , Jesse Everett , Cameron Trainor , Aaron D. Tranter , Ben C. Buchler

Ultrafast processes in matter, such as the electron emission following light absorption, can now be studied using ultrashort light pulses of attosecond duration ($10^{-18}$s) in the extreme ultraviolet spectral range. The lack of spectral…

We study the fundamental limits of the precision of estimating parameters of a quantum matter system when it is probed by a travelling pulse of quantum light. In particular, we focus on the estimation of the interaction strength between the…

Quantum Physics · Physics 2023-06-05 Francesco Albarelli , Evangelia Bisketzi , Aiman Khan , Animesh Datta
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