Related papers: Molecular magnetism in the multi-configurational s…
We report the development of a hybrid numerical / analytical model capable of mapping the spatially-varying distributions of the local ferromagnetic resonance (FMR) frequency and dynamic magnetic susceptibility in a wide class of patterned…
Single-molecule magnets (SMMs) are promising elements for quantum informatics. In the presence of strong magnetic anisotropy, they exhibit magnetization blocking - a magnetic memory effect at the level of a single molecule. Recent studies…
We present a study of systems of single-molecule magnets using a semiclassical analysis and catastrophe theory. Separatrices in parameter space are constructed which are useful to determine the structure of the Hamiltonians energy levels.…
The giant $\{ \mathrm{Mn}_{70} \}$ and $\{ \mathrm{Mn}_{84} \}$ wheels are the largest nuclearity single-molecule magnets synthesized to date and understanding their magnetic properties poses a challenge to theory. Starting from first…
We present a microscopic description of molecular magnets by the multi-orbital Hubbard model, which includes the correlated hopping term, i.e. the dependence of electron hopping amplitude between orbitals on the degree of their occupancy.…
The correct interpretation of magnetic properties in the weak-exchange regime has remained a challenging task for several decades. In this regime, the effective exchange interaction between local spins is quite weak, of the same order of…
We investigate how different chemical environment influences magnetic properties of terbium(III) (Tb)-based single-molecule magnets (SMMs), using first-principles relativistic multireference methods. Recent experiments showed that Tb-based…
In this paper detailed neutron scattering measurements of the magnetic excitation spectrum of CuCrO$_2$ in the ordered state below $T_{\rm{N1}}=24.2$ K are presented. The spectra are analyzed using a model Hamiltonian which includes…
This study examines the increasing complexity in the magnetic properties of small $n$ = 3, 4, 5, 6 spin-1/2 quantum rings. Using an exact diagonalization of the isotropic Heisenberg Hamiltonian with nearest and next-nearest neighbor…
The theoretical treatment of homogeneous static magnetic fields in periodic systems is challenging, as the corresponding vector potential breaks the translational invariance of the Hamiltonian. Based on density operators and perturbation…
We study the magnetization and the spin dynamics of the Cr$_7$Ni ring-shaped magnetic cluster. Measurements of the magnetization at high pulsed fields and low temperature are compared to calculations and show that the spin Hamiltonian…
The peculiarities of coherent spin radiation by magnetic nanomolecules is investigated by means of numerical simulation. The consideration is based on a microscopic Hamiltonian taking into account realistic dipole interactions.…
We investigate the magnetic field behaviour of an antiferromagnetic Heisenberg spin-1 chain with the most general single-ion anisotropy. We discuss the regime in which the magnetic field is below the transition value. The splitting of the…
We identify a magnetoelectric correction that completes the theoretical description of spin splitting (SS) in magnetic systems. Derived from the Dirac equation, this term couples local magnetic moments to the scalar electric potential,…
In the presence of a strong magnetic field, the effective action of a composite scalar field in an scalar O(N) model is derived using two different methods. First, in the framework of worldline formalism, the 1PI n-point vertex function for…
We investigated the reliability and applicability of so-called magnetic force linear response method to calculate spin-spin interaction strengths from first-principles. We examined the dependence on the numerical parameters including the…
The effect of orbital magnetism on the chemical bonding of lateral, two-dimensional artificial molecules is studied in the case of a 2e double quantum dot (artificial molecular hydrogen). It is found that a perpendicular magnetic field…
We present an extension of our one-body M{\o}ller-Plesset second-order perturbation (OBMP2) method for open-shell systems. We derived the OBMP2 Hamiltonian through the canonical transformation followed by the cumulant approximation to…
We present a comprehensive analysis of the magnetic excitations and electronic properties of fully quantum double-exchange ferromagnets, i.e., systems where ferromagnetic ordering emerges from the competition between spin, charge, and…
Using molecular orbital theory, we introduce magnetism in pure-carbon, charge-neutral fullerene monolayers which are otherwise non-magnetic. By controlling either molecular or lattice symmetry, we can realise highly-tuneable magnetic…