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We have developed an extreme ultraviolet (XUV) frequency comb for performing ultra-high precision spectroscopy on the many XUV transitions found in highly charged ions (HCI). Femtosecond pulses from a 100 MHz phase-stabilized near-infrared…

The remarkable precision of frequency comb (FC) lasers is transferred to the extreme ultraviolet (XUV, wavelengths shorter than 100 nm), a frequency region previously not accessable to these devices. A frequency comb at XUV wavelengths near…

High speed optical telecommunication is enabled by wavelength division multiplexing, whereby hundreds of individually stabilized lasers encode the information within a single mode optical fiber. In the seek for larger bandwidth the optical…

Optical frequency combs allow for precise measurement of optical frequencies and are used in a growing number of applications beyond spectroscopy and optical frequency metrology. A class of compact microresonator based frequency comb…

The major development recently undergone by quantum cascade lasers has effectively extended frequency comb emission to longer-wavelength spectral regions, i.e. the mid and far infrared. Unlike classical pulsed frequency combs, their…

We report on the generation of frequency combs from the recently-discovered phenomenon of high-order sideband generation (HSG). A near-band gap continuous-wave (cw) laser with frequency $f_\text{NIR}$ was transmitted through an epitaxial…

Optical frequency combs (FCs), that establish a rigid phase-coherent link between the microwave and optical domains of the electromagnetic spectrum, are emerging as a key high-precision tools for the development of quantum technology…

We report measurements of absolute transition frequencies and hyperfine coupling constants for the 8S_{1/2}, 9S_{1/2}, 7D_{3/2}, and 7D_{5/2} states in ^{133}Cs vapor. The stepwise excitation through either the 6P_{1/2} or 6P_{3/2}…

We describe a possible new technique for precise wavelength calibration of high-resolution astronomical spectrographs using femtosecond-pulsed mode-locked lasers controlled by stable oscillators such as atomic clocks. Such `frequency combs'…

Mid-infrared optical frequency combs are of significant interest for molecular spectroscopy due to the large absorption of molecular vibrational modes on one hand, and the ability to implement superior comb-based spectroscopic modalities…

The broadband, coherent nature of narrow-linewidth fiber frequency combs is exploited to measure the full complex spectrum of a molecular gas through multi-heterodyne spectroscopy. We measure the absorption and phase shift experienced by…

Optics · Physics 2009-11-13 Ian Coddington , William C. Swann , Nathan R. Newbury

Mid-infrared (mid-IR) spectroscopy provides a way to study structures and dynamics of complicated molecules in condensed phases. Therefore, developing compact and broadband mid-IR spectrometer has been a long-standing challenge. Here, we…

Optics · Physics 2020-01-16 Noh Soo Han , JunWoo Kim , Tai Hyun Yoon , Minhaeng Cho

Optical frequency combs [1-8] have resulted in significant advances in optical frequency metrology and found wide application to precise physical measurements [1-4, 9] and molecular fingerprinting [8]. A direct analogue of frequency combs…

Pattern Formation and Solitons · Physics 2017-01-25 Adarsh Ganesan , Cuong Do , Ashwin A. Seshia

The classic self-referenced frequency comb acts as an unrivaled ruler for precision optical metrology in both time and frequency. Two decades after its invention, the frequency comb is now used in numerous active sensing applications. Many…

Frequency combs, spectra of evenly-spaced narrow phase-coherent laser lines, have revolutionized precision measurements. On-chip frequency comb generators hold much promise for fully-integrated instruments of time and frequency metrology.…

High harmonic spectra generated in condensed matter carry the fingerprints of sub-cycle electronic motion and the energy structure of the studied system. Here we show that tailoring the waveform of mid-infrared driving light by using a…

State-of-the-art experiments employ strong ultrafast optical fields to study the nonlinear response of electrons in solids on an attosecond time-scale. Notably, a recent experiment retrieved a 3rd order nonlinear susceptibility by comparing…

While mid-infrared optical frequency combs have been widely utilized in areas such as trace gas sensing, chemical kinetics, and combustion science, the relatively low power per comb tooth has limited acquisition times and sensitivities. We…

Optics · Physics 2023-09-28 Adam T. Heiniger , Matthew J. Cich , David A. Long

Attosecond metrology sensitive to sub-optical-cycle electronic and structural dynamics is opening up new avenues for ultrafast spectroscopy of condensed matter. Using intense lightwaves to precisely control the extremely fast carrier…

We propose a new approach to near-infrared molecular spectroscopy, harnessing advanced concepts of optical telecommunications and supercontinuum photonics. We generate, without mode-locked lasers, two frequency combs of slightly different…

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