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Motivated by recent experimental measurement of the intrinsic excitonic wave-function in 2D Transition-metal dichalcogenides (TMDs) by angle-resolved photoemission spectroscopy (ARPES), we developed a theoretical study to resolve some…

Mesoscale and Nanoscale Physics · Physics 2021-09-01 Nizar Chaouachi , Sihem Jaziri

Coherent dynamics of coupled molecules are effectively characterized by the two-dimensional (2D) electronic coherent spectroscopy. Depending on the coupling between electronic and vibrational states, oscillating signals of purely…

Chemical Physics · Physics 2013-10-17 Vytautas Butkus , Donatas Zigmantas , Darius Abramavicius , Leonas Valkunas

Coherent spin dynamics in colloidal CdSe quantum dots (QDs) typically show two spin components with different Larmor frequencies, whose origin is an open question. We exploit the photocharging approach to identify their origin and find that…

Mesoscale and Nanoscale Physics · Physics 2019-06-24 Rongrong Hu , Dmitri R. Yakovlev , Pan Liang , Gang Qiang , Cong Chen , Tianqing Jia , Zhenrong Sun , Manfred Bayer , Donghai Feng

We study the quantum beats in the polarization of the photon echo from donor-bound exciton ensembles in semiconductor quantum wells. To induce these quantum beats, a sequence composed of a circularly polarized and a linearly polarized…

Mesoscale and Nanoscale Physics · Physics 2020-02-26 S. V. Poltavtsev , I. A. Yugova , Ya. A. Babenko , I. A. Akimov , D. R. Yakovlev , G. Karczewski , S. Chusnutdinow , T. Wojtowicz , M. Bayer

We perform two-dimensional coherent spectroscopy on CdSe/CdZnS core/shell colloidal quantum dots at cryogenic temperatures. In the two-dimensonal spectra, sidebands due to electronic coupling with CdSe lattice LO-phonon modes are observed…

Materials Science · Physics 2019-08-16 A. Liu , D. B. Almeida , W. K. Bae , L. A. Padilha , S. T. Cundiff

We study experimentally time-resolved emission of CdSe quantum dots in an environment with a controlled local density of states (LDOS). The decay rate is measured versus frequency and as a function of distance to a mirror. We observe a…

Optics · Physics 2009-01-13 M. D. Leistikow , J. Johansen , A. J. Kettelarij , P. Lodahl , W. L. Vos

The excitation and detection of coherent phonons has given unique insights into condensed matter, in particular for materials with strong electron-phonon coupling. We report a study of coherent phonons in the layered charge density wave…

The noise spectra associated with correlations of the current through a single level quantum dot, and with the charge fluctuations on the dot, are calculated for a finite bias voltage. The results turn out to be sensitive to the asymmetry…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 E. A. Rothstein , O. Entin-Wohlman , A. Aharony

Long-lived beatings in two-dimensional electronic spectroscopy (2DES) remain difficult to interpret within standard excitonic open-system models, which typically assume factorized initialization and predict rapid coherence decay. We show…

Quantum Physics · Physics 2026-02-05 Sirui Chen , Dragomir Davidović

We propose phonon spectroscopy by electric measurements of the low-temperature conductance of coupled-quantum dots, specifically employing dephasing of the quantum electronic transport by the phonons. The setup we consider consists of a…

Mesoscale and Nanoscale Physics · Physics 2013-05-29 A. Ueda , O. Entin-Wohlman , M. Eto , A. Aharony

The coherent two-dimensional (2D) electronic spectra with respect to the singlet fission (SF) process in organic molecular aggregates are simulated by the Davydov ansatz combined with the Frenkel-Dirac time-dependent variational algorithm.…

Mesoscale and Nanoscale Physics · Physics 2018-01-17 Ke-Wei Sun , Yao Yao

Luminescence spectroscopy experiments were realized for single colloidal quantum dots CdSe/ZnS in a broad temperature range above room temperature in a nitrogen atmosphere. Broadening and shifts of spectra due to the temperature change as…

Spin relaxation in undoped quasi-spherical CdS quantum dots at zero magnetic fields is investigated using time- and polarization-resolved transient absorption measurements. Unlike in previous studies of these systems, the measured signals…

Mesoscale and Nanoscale Physics · Physics 2007-09-27 P. Nahálková , D. Sprinzl , P. Malý , P. Němec , V. N. Gladilin , J. T. Devreese

We perform a nonperturbative analysis of a charge qubit in a double quantum dot structure coupled to its detector. We show that strong detector-dot interaction tends to slow down and halt coherent oscillations. The transitions to a…

Mesoscale and Nanoscale Physics · Physics 2013-05-29 Udo Hartmann , Frank K. Wilhelm

The problem of continuous quantum measurement of coherent oscillations in an individual quantum two-state system is studied for a generic model of the measuring device. It is shown that for a symmetric detector, the signal-to-noise ratio of…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 D. V. Averin

Designing coherent processes is essential for developing quantum information technologies. We study coherent dynamics of two spatially separated electrons in a coupled semiconductor double quantum dot (DQD), in which various two-qubit…

Mesoscale and Nanoscale Physics · Physics 2009-05-09 Gou Shinkai , Toshiaki Hayashi , Takeshi Ota , Toshimasa Fujisawa

We study the noise spectra of a many-level quantum dot coupled to two electron reservoirs, when interactions are taken into account only on the dot within the Hartree-Fock approximation. The dependence of the noise spectra on the…

Mesoscale and Nanoscale Physics · Physics 2015-05-30 N. Gabdank , E. A. Rothstein , O. Entin-Wohlman , A. Aharony

The complex phase diagram of 1T-TiSe2 consists of a charge density wave (CDW) below 200 K, and CDW fluctuations of still unknown origin at higher temperatures. Here, we use time-resolved extreme ultraviolet momentum microscopy and density…

We investigate carrier and collective mode dynamics in 2H-NbSe$_2$ using time-resolved optical pump-probe spectroscopy and compare the results with first-principle calculations. Broadband ultrafast reflectivity studies of 2H-NbSe$_2$ in a…

Strongly Correlated Electrons · Physics 2020-12-30 A. Anikin , R. D. Schaller , G. P. Wiederrecht , E. R. Margine , I. I. Mazin , G. Karapetrov

Quantum bit or qubit is a two-level system, which builds the foundation for quantum computation, simulation, communication and sensing. Quantum states of higher dimension, i.e., qutrits (D = 3) and especially qudits (D = 4 or higher), offer…

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