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Within the nuclear DFT framework, employing the Skyrme UNEDF1 functional and incorporating pairing correlations, we determined the spectroscopic electric quadrupole and magnetic dipole moments of the $\nu11/2^{-}$ and $\pi7/2^{+}$…

Duo is a general, user-friendly program for computing rotational, rovibrational and rovibronic spectra of diatomic molecules. Duo solves the Schr\"{o}dinger equation for the motion of the nuclei not only for the simple case of uncoupled,…

Computational Physics · Physics 2016-07-05 Sergei N. Yurchenko , Lorenzo Lodi , Jonathan Tennyson , Andrey V. Stolyarov

Ultracold LiCs molecules in the absolute ground state X$^1\Sigma^+$, v"=0, J"=0 are formed via a single photo-association step starting from laser-cooled atoms. The selective production of v"=0, J"=2 molecules with a 50-fold higher rate is…

Quantum Physics · Physics 2010-08-09 J. Deiglmayr , A. Grochola , M. Repp , K. Mörtlbauer , C. Glück , J. Lange , O. Dulieu , R. Wester , M. Weidemüller

The lower moments of the unpolarized and polarized deep-inelastic structure functions of the nucleon are calculated on the lattice. The calculation is done with Wilson fermions and for three values of the hopping parameter $\kappa$, so that…

High Energy Physics - Lattice · Physics 2008-11-26 M. Göckeler , R. Horsley , E. -M. Ilgenfritz , H. Oelrich , H. Perlt , P. Rakow , G. Schierholz , A. Schiller

Electric dipole moments of diamagnetic atoms of experimental interest are calculated using the relativistic Hartree-Fock and random-phase approximation methods, the many-body perturbation theory and configuration interaction technique. We…

Atomic Physics · Physics 2009-10-12 V. A. Dzuba , V. V. Flambaum , S. G. Porsev

We present here the MsSpec Dielectric Function module (MsSpec-DFM), which generates dielectric functions in an electron gas or a liquid, either isolated or embedded into an environment. In addition to standard models such as the plasmon…

Other Condensed Matter · Physics 2022-07-21 Aditi Mandal , Sylvain Tricot , Rakesh Choubisa , Didier Sebilleau

We present a novel energy-based localization procedure able to localize molecular orbitals into specific spatial regions. The method is applied to several cases including both conjugated and non-conjugated systems. The obtained localized…

Chemical Physics · Physics 2022-09-13 Tommaso Giovannini , Henrik Koch

Using a counting scheme which treats pseudoscalar and vector mesons on equal footing, the decays of the narrow light vector mesons omega and phi into a dilepton and a pseudoscalar pi-meson or eta-meson, respectively, are calculated.…

High Energy Physics - Phenomenology · Physics 2015-06-03 Carla Terschlüsen , Stefan Leupold

We revisited the electronic structure parameters used to interpret the hyperfine structure of neutral polonium. We used a computational scheme that treats relativistic and high-order electronic correlation effects within the coupled cluster…

Atomic Physics · Physics 2024-03-08 Leonid V. Skripnikov , Anatoly E. Barzakh

The obtention of ultracold samples of dipolar molecules is a current challenge which requires an accurate knowledge of their electronic properties to guide the ongoing experiments. In this paper, we systematically investigate the ground…

Quantum Physics · Physics 2009-11-11 Mireille Aymar , Olivier Dulieu

Single molecule rotational correlation functions are analyzed for several reorientation geometries. Even for the simplest model of isotropic rotational diffusion our findings predict non-exponential correlation functions to be observed by…

Other Condensed Matter · Physics 2016-08-16 G. Hinze , G. Diezemann , Th. Basché

PyCharge is a computational electrodynamics Python simulator that can calculate the electromagnetic fields and potentials generated by moving point charges and can self-consistently simulate dipoles modeled as Lorentz oscillators. To…

Computational Physics · Physics 2022-03-02 Matthew J. Filipovich , Stephen Hughes

Molecular hydrogen ions are of metrological relevance due to the possibility of precise theoretical evaluation of their spectrum and of external-field-induced shifts. In homonuclear molecular ions the electric dipole $E1$ transitions are…

Atomic Physics · Physics 2021-01-20 P. Danev , D. Bakalov , V. I. Korobov , S. Schiller

The synergy between high-resolution rotational spectroscopy and quantum-chemical calculations is essential for exploring future detection of molecules, especially when spectroscopy parameters are not available yet. By using highly…

Instrumentation and Methods for Astrophysics · Physics 2023-11-16 Natalia Inostroza-Pino , Valerio Lattanzi , C. Zachary Palmer , Ryan C. Fortenberry , Diego Mardones , Paola Caselli , Oko E. Godwin , Timothy J. Lee

We trap atoms in versatile two-dimensional (2D) arrays of optical potentials, prepare flexible 2D spin configurations, perform site-selective coherent manipulation, and demonstrate the implementation of simultaneous measurements of…

Quantum Physics · Physics 2011-02-18 Jens Kruse , Christian Gierl , Malte Schlosser , Gerhard Birkl

RaOCH$_3$ molecule is one of the most sensitive systems for the electron electric dipole moment ($e$EDM) searches. Its hyperfine and $K-$doubling structure in the external electric field is of key importance for preparing and interpreting…

Atomic Physics · Physics 2025-08-12 Alexander Petrov

We introduce four new molecules -- YbRb, YbCs, YbSr$^+$, and YbBa$^+$ -- that may prove fruitful in experimental searches for the electric dipole moment (EDM) of the electron. These molecules can, in principle, be prepared at extremely low…

Atomic Physics · Physics 2015-05-13 Edmund R. Meyer , John L. Bohn

We present a theoretical approach for ab initio calculations of the one-loop QED corrections to energy levels of heavy diatomic quasimolecules. This approach is based on the partial-wave expansion of the molecular wave and Green functions…

Atomic Physics · Physics 2022-07-27 A. N. Artemyev , A. Surzhykov , V. A. Yerokhin

The multiconfiguration Dirac-Hartree-Fock (MCDHF) method has been employed to calculate atomic electric dipole moments (EDM) of 225^Ra, 199^Hg, and 171^Yb. For the calculations of the matrix elements we extended the relativistic atomic…

Atomic Physics · Physics 2013-12-24 Laima Radziute , Gediminas Gaigalas , Per Jonsson , Jacek Biero

Vibrational overtones in deeply bound molecules are sensitive probes for variation of the proton-to-electron mass ratio $\mu$. In nonpolar molecules, these overtones may be driven as two-photon transitions. Here, we present procedures for…

Atomic Physics · Physics 2019-01-03 Ryan Carollo , Alexander Frenett , David Hanneke
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