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We employ nonlinear autocorrelation measurements to investigate plasmon-assisted hot carrier dynamics generated in optical gold antennas. We demonstrate that surface plasmons enable a nonlinear formation of hot carriers, providing thus a…

Promoting performance of generation, transport and injection of hot carriers in metal/semiconductor junctions is critical for harvesting energy of hot carriers. However, the injection efficiency of hot carriers in the commonly used noble…

Materials Science · Physics 2025-02-26 Tingting Liu , QianJun Wang , Cheng Zhang , Xiaofeng Li , Jun Hu

The scaling of Si transistor technology has resulted in a remarkable improvement in the performance of integrated circuits over the last decades. However, scaled transistors also require reduced electrical interconnect dimensions, which…

A wide range of unconventional transport phenomena have recently been observed in single-crystal delafossite metals. Here, we present a theoretical framework to elucidate electron transport using a combination of first-principles…

Materials Science · Physics 2022-08-17 Georgios Varnavides , Yaxian Wang , Philip J. W. Moll , Polina Anikeeva , Prineha Narang

Oscillations of conductance observed in strong magnetic fields are a striking manifestation of the quantum dynamics of charge carriers in solids. The large charge carrier density in typical metals sets the scale of oscillations in both…

When plasmonic nanoparticles are coupled with semiconductors, highly energetic hot carriers can be extracted from the metal-semiconductor interface for various applications in light energy conversion. Hot charge-carrier extraction upon…

We developed and tested an approach for predicting trends for efficient hot carrier generation among disordered metal alloys. We provide a simple argument for the importance of indirect transitions in the presence of disorder, thus…

Materials Science · Physics 2024-06-11 Eklavya Thareja , Kevin M. McPeak , Phillip T. Sprunger , Ilya Vekhter , William A. Shelton

We used high resolution angle-resolved photoemission spectroscopy to reveal the Fermi surface and key transport parameters of the metallic state of the layered Colossal Magnetoresistive (CMR) oxide La1.2Sr1.8Mn2O7. With these parameters the…

Strongly Correlated Electrons · Physics 2009-11-07 Y. -D. Chuang , A. D. Gromko , D. S. Dessau , T. Kimura , Y. Tokura

Hot carriers are energetic photo-excited carriers driving a large range of chemico-physical mechanisms. At the nanoscale, an efficient generation of these carriers is facilitated by illuminating plasmonic antennas. However, the ultrafast…

We present anisotropic transport and optical spectroscopy studies on EuCd_2As_2. The measurements reveal that EuCd_2As_2 is a low carrier density semimetal with moderate anisotropic resistivity ratio. The charge carriers experience very…

Strongly Correlated Electrons · Physics 2016-07-15 H. P. Wang , D. S. Wu , Y. G. Shi , N. L. Wang

Fermi liquid theory is remarkably successful in describing the transport and optical properties of metals; at frequencies higher than the scattering rate, the optical conductivity adopts the well-known power law behavior $\sigma_1(\omega)…

Superconductivity · Physics 2013-12-17 C. C. Homes , J. J. Tu , J. Li , G. D. Gu , A. Akrap

We highlight a new metal-molecule charge transfer process by tuning the Fermi energy of plasmonic silver nanoparticles (AgNPs) in-situ. The strong adsorption of halide ions upshifts the Fermi level of AgNPs by up to ~0.3 eV in the order:…

The presence of hot carriers is presented in the operational properties of an (FA,Cs)Pb(I, Br, Cl)3 solar cell at ambient temperatures and under practical solar concentration. At 100 K, clear evidence of hot carriers is observed in both the…

The interband optical absorption of linearly polarised light by two-dimensional (2D) semimetals hosting tilted and anisotropic Dirac cones in the bandstructure is analysed theoretically. Super-critically tilted (type-II) Dirac cones are…

Mesoscale and Nanoscale Physics · Physics 2022-06-09 A. Wild , E. Mariani , M. E. Portnoi

Hot electrons and holes generated from the decay of localized surface plasmons (LSPs) in aluminum nanostructures have significant potential for applications in photocatalysis, photodetection and other optoelectronic devices. Here, we…

Optics · Physics 2025-11-03 Gengyue Dong , Simão João , Hanwen Jin , Johannes Lischner

We briefly review some basic aspects of transport in clean metals focusing on the role of electron-electron interactions and neglecting the effects of impurities, phonons and interband transitions. Both for small Fermi surfaces of two and…

Strongly Correlated Electrons · Physics 2007-05-23 A. Rosch

The collective oscillations of surface charges (surface plasmons) induced by light-matter interactions were predicted in the 1950s to influence electrical conduction in 2D noble metals. Primarily two mechanisms were predicted and later by…

Mesoscale and Nanoscale Physics · Physics 2020-06-19 Suresh C Sharma , Vivek Khichar , Hussein Akafzade , Nader Hozhabri

Quantum transport properties in molecularly thin perovskite/graphene heterostructure are experimentally investigated by Shubnikov-de Hass (SdH) oscillation and photo-resistance spectroscopy. We find an efficient charge transfer between the…

Mesoscale and Nanoscale Physics · Physics 2023-12-22 Yan Sun , C. Morice , D. Garrot , R. Weil , K. Watanabe , T. Taniguchi , M. Monteverde , A. D. Chepelianskii

Topological nodal-line semimetals are characterized by symmetry-protected one-dimensional band-touching lines or loops, which give rise to their peculiar Fermi surfaces at low energies. Furthermore, if time-reversal or inversion symmetry…

Mesoscale and Nanoscale Physics · Physics 2024-01-17 Hamid Rahimpoor , Saeed H. Abedinpour

Hot carrier-based energy conversion systems could double the efficiency of conventional solar energy technology or drive photochemical reactions that would not be possible using fully thermalized, ``cool'' carriers, but current strategies…