Related papers: High-Resolution Quantum Cascade Laser Dual-Comb Sp…
Broadband dual-comb spectroscopy has attracted increasing interests due to its unique advantages in high spectral resolution, fast detection, and so on. Although the dual-comb technique is relatively mature in the infrared wavelengths, it…
We report the upgrade and operation of a frequency-comb-assisted high-resolution mid-infrared molecular spectrometer allowing us to combine high spectral purity, SI-traceability, wide tunability and high sensitivity. An optical frequency…
The road towards the realization of quantum cascade laser (QCL) frequency combs (QCL-combs) has undoubtedly attracted ubiquitous attention from the scientific community, as these devices promise to deliver all-in-one (i.e. a single,…
Due to its fast and high resolution characteristics, dual-comb spectroscopy has attracted an increasing amount of interest since its first demonstration. In the terahertz frequency range where abundant absorption lines (finger prints) of…
Mid infrared (MIR) photonics is a key region for molecular physics [1]. High-resolution spectroscopy in the 1--10 {\mu}m region, though, has never been fully tackled for the lack of widely-tunable and practical light sources. Indeed, all…
Quantum cascade lasers are compact sources capable of generating frequency combs. Yet key characteristics - such as optical bandwidth and power-per-mode distribution - have to be improved for better addressing spectroscopy applications.…
A novel study on harmonic frequency combs emitted by Quantum Cascade Lasers (QCLs) is here presented, demonstrating the presence of intensity correlations between twin modes characterising the emission spectra. These originate from a…
Dual-comb spectroscopy has been proven a powerful tool in molecular characterization, which remains challenging to implement in the mid-infrared region due to difficulties in the realization of two mutually locked comb sources and efficient…
Mid-infrared (mid-IR) spectroscopy offers unparalleled sensitivity for the detection of trace gases, solids and liquids, which is based on the existence of strong telltale vibrational bands in this part of the spectrum. It was shown more…
We demonstrate a robust and simple method for measurement, stabilization and tuning of the frequency of cw mid-infrared (MIR) lasers, in particular of quantum cascade lasers. The proof of principle is performed with a quantum cascade laser…
We have built a frequency chain which enables to measure the absolute frequency of a laser emitting in the 28-31 THz frequency range and stabilized onto a molecular absorption line. The set-up uses an optical frequency comb and an…
Historically, there has been a trade-off in spectroscopic measurements between high spectral resolution, broadband coverage, and acquisition time. Optical frequency combs, initially envisioned for precision spectroscopy of the hydrogen atom…
The femtosecond laser frequency comb has enabled the 21st century revolution in optical synthesis and metrology. A particularly compelling technique that relies on the broadband coherence of two laser frequency combs is dual-comb…
Optical frequency combs enable all-solid-state spectrometers that will trigger a breakthrough in miniaturization and on-chip integration of mid-infrared sensing technology. Interband cascade lasers (ICLs) are an ideal candidate for…
Laser spectroscopy and interferometry have provided an unparalleled view into the fundamental nature of matter and the universe through ultra-precise measurements of atomic transition frequencies and gravitational waves. Optical frequency…
Mid-infrared microscopy is an important tool for biological analyses, allowing a direct probe of molecular bonds in their low energy landscape. In addition to the label-free extraction of spectroscopic information, the application of…
Dual-frequency comb spectroscopy permits broadband precision spectroscopic measurements with short acquisition time. A dramatic improvement of the maximal spectral bandwidth and the minimal measurement time can be expected when the lasers'…
The major development recently undergone by quantum cascade lasers has effectively extended frequency comb emission to longer-wavelength spectral regions, i.e. the mid and far infrared. Unlike classical pulsed frequency combs, their…
We describe a possible new technique for precise wavelength calibration of high-resolution astronomical spectrographs using femtosecond-pulsed mode-locked lasers controlled by stable oscillators such as atomic clocks. Such `frequency combs'…
A fully stabilized mid-infrared optical frequency comb spanning from 2.9 to 3.4 um is described. The comb is based on half-harmonic generation in a femtosecond optical parametric oscillator, which transfers the high phase coherence of a…