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Free energies of molecules can be calculated by quantum computations or by normal mode classical calculations. However, the first can be computationally impractical for large molecules and the second is based on the assumption of harmonic…

Chemical Physics · Physics 2016-03-23 Asaf Farhi

This article explores the van der Waals gas model proposed to describe the hadronic stages of nuclear fireball evolution during the cooling stage. Two different models were proposed for the early and late stages of hadronization. At the…

High Energy Physics - Phenomenology · Physics 2023-05-18 Yaroslav D. Krivenko-Emetov , Andriy I. Smetana

A new molecular simulation method for the calculation of vapour-liquid equilibria of mixtures is presented. In this method, the independent thermodynamic variables are temperature and liquid composition. In the first step, one isobaric…

Chemical Physics · Physics 2009-05-06 J. Vrabec , H. Hasse

Many liquids have curves (isomorphs) in their phase diagrams along which structure, dynamics, and some thermodynamic quantities are invariant in reduced units. A substantial part of their phase diagrams is thus effectively one dimensional.…

Soft Condensed Matter · Physics 2016-08-22 Arno A. Veldhorst , Thomas B. Schrøder , Jeppe C. Dyre

We study the relations among the chemical potentials of paired and unpaired particles in a cold asymmetrical fermionic mixed phase in thermodynamical equilibrium. We show how the chemical potentials are expressed in terms of the parameters…

Superconductivity · Physics 2011-11-09 Heron Caldas

We formulate a method for calculating the hadron-hadron scattering amplitudes at nonzero chemical potential ($\mu$) in the hadronic phase at zero temperature, where the baryon number symmetry remains to be violated. Although it is widely…

High Energy Physics - Lattice · Physics 2024-02-01 Kotaro Murakami , Etsuko Itou , Kei Iida

We propose a new method to compute the free energy or enthalpy of fluids or disordered solids by computer simulation . The main idea is to construct a reference system by freezing one representative configuration, and then carry out a…

Computational Physics · Physics 2011-03-16 Friederike Schmid , Tanja Schilling

We study the chemical potential of D-instantons in c=0 noncritical string theory. In a recent work(hep-th/0405076), it was shown that the chemical potential can be calculated using the one matrix model. The calculation was done using the…

High Energy Physics - Theory · Physics 2009-11-11 Nobuyuki Ishibashi , Atsushi Yamaguchi

The shift in chemical equilibria due to isotope substitution is often exploited to gain insight into a wide variety of chemical and physical processes. It is a purely quantum mechanical effect, which can be computed exactly using…

Statistical Mechanics · Physics 2014-07-04 Michele Ceriotti , Thomas E. Markland

Solvation free energy is an important quantity in Computational Chemistry with a variety of applications, especially in drug discovery and design. The accurate prediction of solvation free energies of small molecules in water is still a…

Biological Physics · Physics 2007-05-23 A. Hildebrandt , O. Kohlbacher , R. Blossey , H. -P. Lenhof

We present a molecular dynamics simulation method for the computation of the solubility of organic crystals in solution. The solubility is calculated based on the equilibrium free energy difference between the solvated solute and its…

Statistical Mechanics · Physics 2021-04-23 Zoran Bjelobrk , Dan Mendels , Tarak Karmakar , Michele Parrinello , Marco Mazzotti

Mesoscopic molecular dynamics simulations are used to determine the large scale structure of several binary polymer mixtures of various chemical architecture, concentration, and thermodynamic conditions. By implementing an analytical…

Soft Condensed Matter · Physics 2010-04-05 J. McCarty , I. Y. Lyubimov , M. G. Guenza

In this work the free energy of solid phases is computed for the Lennard-Jones potential and for a model of NaCl. The free energy is evaluated through the Einstein crystal/molecule methodologies using the Molecular Dynamics programs:…

Soft Condensed Matter · Physics 2012-10-16 J. L. Aragones , C. Valeriani , C. Vega

We propose a numerical technique to compute the equilibrium free energy of glasses that cannot be prepared quasi-reversibly. For such systems, standard techniques for estimating the free energy by extrapolation, cannot be used. Instead, we…

Statistical Mechanics · Physics 2021-01-04 H. A. Vinutha , Daan Frenkel

A general set of methods is presented for calculating chemical potentials in solid and liquid mixtures using {\em ab initio} techniques based on density functional theory (DFT). The methods are designed to give an {\em ab initio} approach…

Materials Science · Physics 2009-11-07 D. Alfe` , M. J. Gillan , G. D. Price

Calculating free energy differences is a topic of substantial interest and has many applications including molecular docking and hydration, solvation, and binding free energies which is used in computational drug discovery. However, in…

Chemical Physics · Physics 2013-10-16 Asaf Farhi

We present an analytical method to estimate the condensate fraction $n_0/n$ in strongly correlated systems for which the zero-temperature static structure factor $S({\bf p})$ is known. The advantage of the proposed method is that it allows…

Quantum Gases · Physics 2021-04-08 Yu. E. Lozovik , I. L. Kurbakov , G. E. Astrakharchik , J. Boronat

Different computational techniques in combination with molecular dynamics computer simulation are used to to determine the wall-liquid and the wall-crystal interfacial free energies of a modified Lennard-Jones (LJ) system in contact with a…

Statistical Mechanics · Physics 2015-06-16 Ronald Benjamin , Jürgen Horbach

Isothermal-isobaric molecular dynamics simulations are used to examine the microscopic structure and some properties of water-methanol liquid mixture. The TIP4P/2005 and SPC/E water models are combined with the united atom TraPPE and the…

Soft Condensed Matter · Physics 2019-03-28 M. Cruz Sanchez , H. Dominguez , O. Pizio

In this review we focus on the determination of phase diagrams by computer simulation with particular attention to the fluid-solid and solid-solid equilibria. The calculation of the free energy of solid phases using the Einstein crystal and…

Statistical Mechanics · Physics 2009-01-14 C. Vega , E. Sanz , J. L. F. Abascal , E. G. Noya