Related papers: Shells in CO$_2$ Clusters
The mass spectra of gas-phase clusters in cluster beams have a rich structure where the relative heights of the peaks compared to peaks corresponding to clusters of neighbor sizes reveal the stability of the clusters as a function of the…
Together with the second generation REBO reactive potential, replica-exchange molecular dynamics simulations coupled with systematic quenching were used to generate a broad set of isomers for neutral C$_n$ clusters with $n=24$, 42, and 60.…
Size and composition of clusters produced by adiabatic expansion of binary gas mixtures (Ar-Kr, Kr-Xe, and N2-Ar) with various component concentrations are studied by using electron-diffraction technique. The resulting homogeneous and…
Influence of surrounding matter on the properties of clusters is considered by an approach combining the methods of statistical and quantum mechanics. A cluster is treated as a bound N-particle system and surrounding matter as thermostat.…
We investigate the dependence of cluster abundance $n(>M,r_{cl})$, i.e., the number density of clusters with mass larger than $M$ within radius $r_{cl}$, on scale parameter $r_{cl}$. Using numerical simulations of clusters in the CDM…
An ab initio density functional study was performed investigating the adsorption of CO$_2$ on the neutral boron B$_{n}$ ($n = 10-13$) clusters, characterized by planar and quasiplanar ground-state atomic structures. For all four clusters,…
We have carried out extensive density functional calculations for series of sodium clusters $Na$$_{N}$ ranging from $N$=10 to 147 and have obtained $\approx$ 13000 distinct isomers. We unravel a number of striking features of the growth…
A variable combination of realistic and random two-body interactions allows the study of collective properties, such as the energy spectra and B(E2) transition strengths in 44Ti, 48Cr and 24Mg. It is found that the average energies of the…
An expansion of energy characteristics of wide thin slab of thickness L in power of 1/L is constructed using the free-electron approximation and the model of a potential well of finite depth. Accuracy of results in each order of the…
Dynamics of coarsening of a statistically homogeneous fractal cluster, created by a morphological instability of diffusion-controlled growth, is investigated theoretically. An exact mathematical setting of the problem is presented that…
Two exponents, $\delta$, for size distribution of $n$-atom clusters, $Y(n)\sim n^{-\delta}$, have been found in Au clusters sputtered from embedded Au nanoparticles under swift heavy ion irradiation. For small clusters, below 12.5 nm in…
Cluster growth in a coagulating system of active particles (such as microswimmers in a solvent) is studied by theory and simulation. In contrast to passive systems, the net velocity of a cluster can have various scalings dependent on the…
We numerically investigate the vibrational spectra of single-component clusters in two-dimensions. Stable configurations of clusters at local energy minima are obtained, and for each the hessian matrix is evaluated and diagonalized to…
We measured the binding energy of N$_2$, CO, O$_2$, CH$_4$, and CO$_2$ on non-porous (compact) amorphous solid water (np-ASW), of N$_2$ and CO on porous amorphous solid water (p-ASW), and of NH$_3$ on crystalline water ice. We were able to…
The existence of shell structure and the accompanying high degeneracy of electronic levels leads to the possibility of strong superconducting pairing in metallic nanoclusters with N~100-1000 delocalized electrons. The most favorable cases…
The exponential sensitivity of cluster number counts to the properties of the dark energy implies a comparable sensitivity to not only the mean but also the actual_distribution_ of an observable mass proxy given the true cluster mass. For…
We propose a model of mass-conserving heterogeneous nucleation to describe the dynamics of ligand-receptor binding in closed cellular compartments. When the ligand dissociation rate is small, competition among receptors for free ligands…
Although globular clusters are generally chemically homogeneous, substantial abundance variations are sometimes seen even among unevolved main sequence stars, especially for the CNO group of elements. Multi-object intermediate-dispersion…
We examine the classic problem of homogeneous nucleation and growth by deriving and analyzing a fully discrete stochastic master equation. Upon comparison with results obtained from the corresponding mean-field Becker-D\"{o}ring equations…
This Article presents a nonequilibrium thermodynamic theory for the mean-field precipitation, aggregation and pattern formation of colloidal clusters. A variable gradient energy coefficient and the arrest of particle diffusion upon…